Excellent photothermal conversion of core/shell CdSe/Bi2Se3 quantum dots
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- 作者：Guo Zhi Jia ; Wen Kai Lou ; Fang Cheng ; Xiong Long Wang ; Jiang Hong Yao…
- 关键词：cation exchange ; quantum dots ; photothermal ; type ; II heterostructure ; CdSe/Bi2Se3
- 刊名：Nano Research
- 出版年：2015
- 出版时间：May 2015
- 年：2015
- 卷：8
- 期：5
- 页码：1443-1453
- 全文大小：2,176 KB
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Wen Kai Lou (1)
Fang Cheng (3)
Xiong Long Wang (4)
Jiang Hong Yao (4)
Ning Dai (5)
Hai Qing Lin (6)
Kai Chang (1)
1. Institute of Semiconductors, Chinese Academy of Sciences, P.O. Box 912, Beijing, 100083, China
2. Tianjin Chengjian University, Tianjin, 300384, China
3. Department of Physics and Electronic Science, Changsha University of Science and Technology, Changsha, 410004, China
4. Key Laboratory of Weak-Light Nonlinear Photonics, Ministry of Education, School of Physics and TEDA Applied Physics School, Nankai University, Tianjin, 300457, China
5. Inst Tech Phys, Nat Lab Infrared Phys, Chinese Academy of Sciences, Shanghai, 200083, China
6. Beijing Computational Science Research Center, Beijing, 100084, China - 刊物类别：Chemistry and Materials Science
- 刊物主题：Chinese Library of Science
Chemistry
Nanotechnology - 出版者：Tsinghua University Press, co-published with Springer-Verlag GmbH
- ISSN：1998-0000
文摘
Water-dispersed CdSe/Bi2Se3 core/shell QDs with a photothermal conversion coefficient of 27.09% have been synthesized by a cation exchange reaction. The microstructure and crystal structure of the QDs, which were confirmed by TEM and XRD, showed that partial cation exchange occurred inside the CdSe QDs. Two main mechanisms are responsible for the excellent photothermal conversion: inhibition of radiative recombination of carriers due to the formation of type-II semiconductor heterostructures, and the large surface-to-volume ratio of the QDs. Photothermal conversion experiments indicated that the CdSe/Bi2Se3 QDs showed high photothermal conversion efficiency and excellent NIR photostability.