Coordination of Lewis Acids to Transition Metals: Z-Type Ligands

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• 关键词：Ambiphilic ligands ; Boranes ; Lewis acids ; M→Lewis acid interactions ; M→Z interactions ; Polyfunctional ligands ; σ ; acceptor ligands
• 刊名：Structure & Bonding
• 出版年：2017
• 出版时间：2017
• 年：2017
• 卷：171
• 期：1
• 页码：141-201
• 全文大小：5,451 KB
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• 作者单位：Ghenwa Bouhadir (3) (4)
  Didier Bourissou (3) (4)
  
  3. Université de Toulouse, UPS, Laboratoire Hétérochimie Fondamentale Appliquée, 118 route de Narbonne, 31062, Toulouse, France
  4. CNRS, LHFA UMR 5069, 31062, Toulouse, France
  
• 丛书名：The Chemical Bond III
• ISBN：978-3-319-35146-9
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Inorganic Chemistry
  
• 出版者：Springer Berlin / Heidelberg
• ISSN：1616-8550
• 卷排序：171

文摘

This chapter provides a comprehensive review of M→Z complexes, that is to say complexes featuring Lewis acids coordinated as σ-acceptor ligands. The preparation, structure and bonding, as well as the characteristic features of M→Z complexes are discussed. Only Lewis acids derived from the p-block elements are considered, with a focus on two-center M→Z interactions supported by donor sidearms. The chapter is organized according to (1) the nature of the Lewis acid moiety (based on group 13, 14, 15 or 16 elements), (2) the way the M→Z interaction is formed (by B–H activation of pro-ligands or direct coordination of preformed ambiphilic ligands) and (3) the type of complexes (M→Z interactions supported by 3, 2 or 1 donor sidearms, unsupported M→Z interactions).