类石墨相氮化碳的复合研究进展
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摘要
类石墨相氮化碳(g-C_3N_4)是一种可见光响应的有机聚合物半导体催化材料,因比表面积小和吸附性能差等缺点限制了其实际应用。对g-C_3N_4的各种掺杂、复合、负载等改性研究一直是材料化学研究领域的热点之一,分类总结了近几年国内外文献报道的关于g-C_3N_4多孔材料负载、与半导体材料形成同型或异型异质结复合物等研究,以探讨g-C_3N_4今后的改性研究方向。
Graphite-like carbon nitride(g-C_3N_4)is an organic polymer semiconductor material and visible light-responsive.Its practical application is limited by its small BET area and low absorbability.Various modifications of g-C_3N_4 such as doping,composition and loading have always been one of the hotspots in the field of materials chemistry.This review summarizes the research of g-C_3N_4 on porous material loading,isomorphic or heterojunction composition with semiconductor materials reported in recent years at home and abroad to explore the future research direction of the modification for g-C_3N_4.
Graphite-like carbon nitride(g-C_3N_4)is an organic polymer semiconductor material and visible light-responsive.Its practical application is limited by its small BET area and low absorbability.Various modifications of g-C_3N_4 such as doping,composition and loading have always been one of the hotspots in the field of materials chemistry.This review summarizes the research of g-C_3N_4 on porous material loading,isomorphic or heterojunction composition with semiconductor materials reported in recent years at home and abroad to explore the future research direction of the modification for g-C_3N_4.
引文
[1]CHEN J,OLLIS D F,RULKENS W H,et al.Photocatalyzed oxidation of alcohols ans organochlorides in the prensence of native TiO2 and metallized TiO2 suspensions.Part(Ⅰ):Photocatalytic activity and pH influence[J].Water Research,1999,33(3):661-668.
[2]CHEN J,OLLIS D F,RULKENS W H,et al.Photocatalyzed oxidation of alcohols and organochlorides in the prensence of native TiO2and metallized TiO2suspensions.Part(II):Photocatalytic mechanisms[J].Water Research,1999,33(3):669-676.
[3]LIU A Y,COHEN M L.Prediction of new low compressibility solids[J].Science,1989,245(4920):841-842.
[4]LI X Y,WANG Y,KANG L H,et al.A novel,non-metallic graphitic carbon nitride catalyst for acetylene hydrochlorination[J].Journal of Catalysis,2014,311:288-294.
[5]CHEN X Y,KUO D H,LU D F.Nanonization of g-C3N4with the assistance of activated carbon for improved visible light photocatalysis[J].RSC Adv,2016,6:66814-66821.
[6]LEE R,TRAN P D,PRAMANA S S,et al.Assembling graphitic-carbon-nitride with cobalt-oxide-phosphate to construct an efficient hybrid photocatalyst for water splitting application[J].Catalysis Science&Technology,2013,3(7):1694-1698.
[7]DONG G,ZHANG L.Synthesis and enhanced Cr(VI)photoreduction property of formate anion containing graphitic carbon nitride[J].The Journal of Physical Chemistry,2013,117(8):4062-4068.
[8]DIMITRIOS A GIANNAKOUDAKIS,NIKOLINA A TRAV-LOU,JEFF SECOR,et al.Oxidized g-C3N4nanospheres as catalytically photoactive linkers in MOF/g-C3N4composite of hierarchical pore structure[J].Small,2017,13:1601758-1601766.
[9]SUYANA PANNERI,MINJU THOMAS,PRIYANKAGANGULY,et al.C3N4anchored ZIF 8composites:photoregenerable,high capacity sorbents as adsorptive photocatalysts for the effective removal of tetracycline from water[J].Catalysis Science&Technology,2017,7:2118-2128.
[10]姚光远,黄伟欣,李春全,等.g-C3N4/高岭土复合材料的制备及其光催化性能研究[J].无机材料学报,2016,31(9):929-934.
[11]袁炳楠,董悦,郭明辉.木材表面g-C3N4的固定及其光降解性能表征[J].南京林业大学学报(自然科学版),2018,42(1):193-197.
[12]李冬梅,程志华,黄明珠,等.可见光响应GO/g-C3N4改性平板膜的制备条件及其表面性能研究[J].环境科学学报,2018,7:1-18.
[13]ZHAO W L,ZHU M Y,DAI B.The preparation of Cu-gC3N4/AC catalyst for acetylene hydrochlorination[J].Catalysts,2016,193(6):1-10.
[14]陶雪芬,蒋雨涛,魏晶晶,等.g-C3N4/AC的制备及其可见光催化活性研究[J].当代化工,2017,46(7):1287-1289.
[15]吴昊,范明明,张萍波,等.g-C3N4固载磷钨酸催化剂的制备及催化性能[J].中国油脂,2018,43(7):41-45.
[16]于柳,王宇超,徐荣,等.SiW12/g-C3N4纳米复合材料的制备及光催化活性[J].分子科学学报,2018,34(3):177-182.
[17]涂盛辉,戴策,林立,等.双金属纳米Ag/Cu负载g-C3N4催化剂的制备及光催化制氢活性[J].南昌大学学报(理科版),2017,41(6):555-560.
[18]张倩,胡绍争,李法云,等.高效可见光响应Zn0.11Sn0.12Cd0.84S1.12/g-C3N4异质结光催化剂的制备及性能[J].高等学校化学学报,2016,37(3):521-528.
[19]杨芷,刘修平,项文睿,等.光纤负载g-C3N4/TiO2薄膜催化剂的制备及其降解间二甲苯性能研究[J].分子科学学报,2018,34(3):199-206.
[20]张黎明,吴磊,邵云,等.Cu-g-C3N4/WO3可见光下降解四环素的性能研究[J].人工晶体学报,2018,47(6):1128-1135.
[21]SHAFAQ SAHAR,AKIF ZEB,刘亚男,et al.Fe3O4/g-C3N4复合催化剂增强芬顿/光-芬顿和类过氧化酶反应的活性及稳定性(英文)[J].催化学报,2017,38(12):2110-2119.
[22]周银,张平,邹赛,等.可磁分离Fe3O4/g-C3N4复合材料的制备及其性能[J/OL].复合材料学报,2018,7:1-8.
[23]崔诗琦,张秀芳,王聪.薄层g-C3N4/β-SnWO4异质结光催化剂的制备及性能[J].大连工业大学学报,2018,37(3):179-182.
[24]ANISE AKHUNDI,AZIZ HABIBI-YANGJEH.Graphitic carbon nitride nanosheets decorated with CuCr2O4nanoparticles:Novel photocatalysts with high performances in visible light degradation of water pollutants[J].Journal of Colloid and Interface Science,2017,504:697-710.
[25]CHEN J F,ZHONG J B,LI J Z,et al.Synthesis and characterization of novel Ag2CO3/g-C3N4 composite photocatalysts with excellent solar photocatalytic activity and mechanism insight[J].Molecular Catalysis,2017,435:91-98.
[26]韩红桔,傅敏,李亚林,等.原位聚合PPy/g-C3N4复合物增强可见光催化性能(英文)[J].催化学报,2018,39(4):831-840.
[27]赵云霏,毋瑞仙,蒋平平,等.g-C3N4和Ni2P的复合及其光催化产氢性能研究[J].分子催化,2018,32(2):142-151.
[28]阎鑫,卢锦花,惠小艳,等.g-C3N4/MoS2纳米片/氧化石墨烯三元复合催化剂的制备及可见光催化性能[J].无机材料学报,2018,33(5):515-520.
[29]YANG X L,QIAN F F,ZOU G J,et al.Facile fabrication of acidified g-C3N4/g-C3N4hybrids with enhanced photocatalysis performance under visible light irradiation[J].Catalysis B:Environmental,2016,193:22-35.
[30]李军奇,郝红娟,周健,等.g-C3N4/g-C3N4异质结结构的制备及其光催化性能[J].陕西科技大学学报,2016,34(2):59-63.
[2]CHEN J,OLLIS D F,RULKENS W H,et al.Photocatalyzed oxidation of alcohols and organochlorides in the prensence of native TiO2and metallized TiO2suspensions.Part(II):Photocatalytic mechanisms[J].Water Research,1999,33(3):669-676.
[3]LIU A Y,COHEN M L.Prediction of new low compressibility solids[J].Science,1989,245(4920):841-842.
[4]LI X Y,WANG Y,KANG L H,et al.A novel,non-metallic graphitic carbon nitride catalyst for acetylene hydrochlorination[J].Journal of Catalysis,2014,311:288-294.
[5]CHEN X Y,KUO D H,LU D F.Nanonization of g-C3N4with the assistance of activated carbon for improved visible light photocatalysis[J].RSC Adv,2016,6:66814-66821.
[6]LEE R,TRAN P D,PRAMANA S S,et al.Assembling graphitic-carbon-nitride with cobalt-oxide-phosphate to construct an efficient hybrid photocatalyst for water splitting application[J].Catalysis Science&Technology,2013,3(7):1694-1698.
[7]DONG G,ZHANG L.Synthesis and enhanced Cr(VI)photoreduction property of formate anion containing graphitic carbon nitride[J].The Journal of Physical Chemistry,2013,117(8):4062-4068.
[8]DIMITRIOS A GIANNAKOUDAKIS,NIKOLINA A TRAV-LOU,JEFF SECOR,et al.Oxidized g-C3N4nanospheres as catalytically photoactive linkers in MOF/g-C3N4composite of hierarchical pore structure[J].Small,2017,13:1601758-1601766.
[9]SUYANA PANNERI,MINJU THOMAS,PRIYANKAGANGULY,et al.C3N4anchored ZIF 8composites:photoregenerable,high capacity sorbents as adsorptive photocatalysts for the effective removal of tetracycline from water[J].Catalysis Science&Technology,2017,7:2118-2128.
[10]姚光远,黄伟欣,李春全,等.g-C3N4/高岭土复合材料的制备及其光催化性能研究[J].无机材料学报,2016,31(9):929-934.
[11]袁炳楠,董悦,郭明辉.木材表面g-C3N4的固定及其光降解性能表征[J].南京林业大学学报(自然科学版),2018,42(1):193-197.
[12]李冬梅,程志华,黄明珠,等.可见光响应GO/g-C3N4改性平板膜的制备条件及其表面性能研究[J].环境科学学报,2018,7:1-18.
[13]ZHAO W L,ZHU M Y,DAI B.The preparation of Cu-gC3N4/AC catalyst for acetylene hydrochlorination[J].Catalysts,2016,193(6):1-10.
[14]陶雪芬,蒋雨涛,魏晶晶,等.g-C3N4/AC的制备及其可见光催化活性研究[J].当代化工,2017,46(7):1287-1289.
[15]吴昊,范明明,张萍波,等.g-C3N4固载磷钨酸催化剂的制备及催化性能[J].中国油脂,2018,43(7):41-45.
[16]于柳,王宇超,徐荣,等.SiW12/g-C3N4纳米复合材料的制备及光催化活性[J].分子科学学报,2018,34(3):177-182.
[17]涂盛辉,戴策,林立,等.双金属纳米Ag/Cu负载g-C3N4催化剂的制备及光催化制氢活性[J].南昌大学学报(理科版),2017,41(6):555-560.
[18]张倩,胡绍争,李法云,等.高效可见光响应Zn0.11Sn0.12Cd0.84S1.12/g-C3N4异质结光催化剂的制备及性能[J].高等学校化学学报,2016,37(3):521-528.
[19]杨芷,刘修平,项文睿,等.光纤负载g-C3N4/TiO2薄膜催化剂的制备及其降解间二甲苯性能研究[J].分子科学学报,2018,34(3):199-206.
[20]张黎明,吴磊,邵云,等.Cu-g-C3N4/WO3可见光下降解四环素的性能研究[J].人工晶体学报,2018,47(6):1128-1135.
[21]SHAFAQ SAHAR,AKIF ZEB,刘亚男,et al.Fe3O4/g-C3N4复合催化剂增强芬顿/光-芬顿和类过氧化酶反应的活性及稳定性(英文)[J].催化学报,2017,38(12):2110-2119.
[22]周银,张平,邹赛,等.可磁分离Fe3O4/g-C3N4复合材料的制备及其性能[J/OL].复合材料学报,2018,7:1-8.
[23]崔诗琦,张秀芳,王聪.薄层g-C3N4/β-SnWO4异质结光催化剂的制备及性能[J].大连工业大学学报,2018,37(3):179-182.
[24]ANISE AKHUNDI,AZIZ HABIBI-YANGJEH.Graphitic carbon nitride nanosheets decorated with CuCr2O4nanoparticles:Novel photocatalysts with high performances in visible light degradation of water pollutants[J].Journal of Colloid and Interface Science,2017,504:697-710.
[25]CHEN J F,ZHONG J B,LI J Z,et al.Synthesis and characterization of novel Ag2CO3/g-C3N4 composite photocatalysts with excellent solar photocatalytic activity and mechanism insight[J].Molecular Catalysis,2017,435:91-98.
[26]韩红桔,傅敏,李亚林,等.原位聚合PPy/g-C3N4复合物增强可见光催化性能(英文)[J].催化学报,2018,39(4):831-840.
[27]赵云霏,毋瑞仙,蒋平平,等.g-C3N4和Ni2P的复合及其光催化产氢性能研究[J].分子催化,2018,32(2):142-151.
[28]阎鑫,卢锦花,惠小艳,等.g-C3N4/MoS2纳米片/氧化石墨烯三元复合催化剂的制备及可见光催化性能[J].无机材料学报,2018,33(5):515-520.
[29]YANG X L,QIAN F F,ZOU G J,et al.Facile fabrication of acidified g-C3N4/g-C3N4hybrids with enhanced photocatalysis performance under visible light irradiation[J].Catalysis B:Environmental,2016,193:22-35.
[30]李军奇,郝红娟,周健,等.g-C3N4/g-C3N4异质结结构的制备及其光催化性能[J].陕西科技大学学报,2016,34(2):59-63.