离子液体的生物毒性及降解性研究
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摘要
由于离子液体独特的理化性质,其被广泛应用于萃取、催化、电化学等领域,并且离子液体被称为是继水和超临界二氧化碳之后的又一"绿色溶剂"。随着研究的加深,离子液体自身的毒性和降解性也渐渐成为关注的重点。归纳离子液体对微生物、水生生物、植物、动物的毒性研究进展之后对离子液体的降解方法进行总结。降解方法主要包括化学降解法和生物降解法;对吡啶类离子液体的植物、动物毒性以及生物降解性进行较为深入地研究,以期为离子液体毒性及降解性研究提供参考;展望离子液体毒性和降解性改进的研究方向和研究方法,为其在化工等领域应用的绿色化给出了研究方向。
引文
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[2]Berton P,Bica K,Rogers R D,et al.Ionic liquids for consumer products:dissolution,characterization,and controlled release of fragrance compositions[J]. Fluid Phase Equilibria,2017,450(10):51-56.
[3]Cull S,Holbrey J,Vargasmora V,et al. Room temperature ionic liquids as replacements for organic solvents in multiphase bioprocess operations[J]. Biotechnology and Bioengineering,2000,69(2):227-33.
[4]Mccrary P D,Beasley P A,Gurar G,et al. Drug specific,tuning of an ionic liquid's hydrophilic-lipophilic balance to improve water solubility of poorly soluble active pharmaceutical ingredients[J]. New Journal of Chemistry,2013,37(7):2196-2202.
[5]Trush M M,Semenyuta I V,Vdovenko S I,et al. Synthesis,spectroscopic and molecular docking studies of imidazolium and pyridinium based ionic liquids with HSA as potential antimicrobial agents[J]. Journal of Molecular Structure,2017,1137(6):692-699.
[6]Carson L,Chau P K W,Earle M J,et al. Antibiofilm activities of 1-alkyl-3-methylimidazolium chloride ionic liquids[J]. Green Chemistry,2009,11(4):492-497.
[7]林燕,王芳,张志庆,等. 离子液体绿色脱硫机理及应用进展[J]. 化工进展,2013,32(3):549-557.
[8]Pan J,Muppaneni T,Sun Y,et al. Microwave-assisted extraction of lipids from microalgae using an ionic liquid solvent[Bmim][HSO4][J]. Fuel,2016,178:49-55.
[9]柏杨,曹晓燕,代军,等. 离子液体分类、合成、表征及应用研究[J]. 当代化工,2010,39(4):445-448.
[10]郑燕升,莫倩,刘昭明. 离子液体的QSPR/QSAR研究[J]. 化学进展,2009,21(9):1772-1781.
[11]张瑾,刘树深,窦容妮,等. 30种离子液体对青海弧菌Q67的毒性效应[J]. 环境科学,2011,32(4):1108-1113.
[12]Hafez N F M,Mutalib M I A,Bustam M A B,et al. Ecotoxicity of pyridinium based ILs towards guppy fish and four bacterial strains[J]. Procedia Engineering,2016,148:830-838.
[13]Bernot R J,Kennedy E E,Lamberti G A. et al. Effects of ionic liquids on the survival,movement,and feeding behavior of the freshwater snail,Physa acuta[J]. Environmental Toxicology & Chemistry,2005,24(7):1759-1765.
[14]Pretti C,Chiappe C,Pieraccini D,et al.Acute toxicity of ionic liquids to the zebrafish (Danio rerio)[J]. Green Chemistry,2006,8(3):238-240.
[15]陈忠林,王洋,关伟,等. 离子液体[C2mim][Val]对小麦幼苗生长及生理特性的影响[J]. 农业环境科学学报,2011,30(8):1508-1513.
[16]董莹,张淑娴,刘惠君. 两种咪唑氯盐类离子液体对水稻幼苗根部的毒性效应[J]. 环境科学学报,2015,35(10):3384-3389.
[17]Balczewski P,Bachowska B,Bialas T,et al.Synthesis and phytotoxicity of new ionic liquids incorporating chiral cations and/or chiral anions[J]. Journal of Agricultural & Food Chemistry,2007,55(5):1881-1892.
[18]井长勤,陈红丽,李效宇. 离子液体氯化1-辛基-3-甲基咪唑对EMT6细胞的毒性及其机理研究[J]. 环境科学学报,2013,33(6):1809-1814.
[19]Kolwankar K M,Ren Q,Samal A,et al. Learning and structure of neuronal networks[J]. Pramana,2011,77(5):817-826.
[20]Swatloski R P,Holbrey J D,Memon S B,et al.Using caenorhabditis elegans to probe toxicity of 1-alkyl-3-methylimidazolium chloride based ionic liquids[J]. Chemical Communications,2004,35(6):668-669.
[21]Siedlecka E M,Mrozik W,Kaczynski Z,et al. Degradation of 1-butyl-3-methylimidazolium chloride ionic liquid in a Fenton-like system[J]. Journal of Hazardous Materials,2008,154(1/2/3):893-900.
[22]Stepnowski P,Zaleska A. Comparison of different advanced oxidation processes for the degradation of room temperature ionic liquids[J]. Journal of Photochemistry & Photobiology a Chemistry,2005,170(1):45-50.
[23]Stolte S,Abdulkarim S,Arning J,et al.Primary biodegradation of ionic liquid cations,identification of degradation products of 1-methyl-3-octylimidazolium chloride and electrochemical wastewater treatment of poorly biodegradable compounds[J]. Green Chemistry,2008,10(2):214-224.
[24]Docherty K M,Dixon J K,Kulpa C F. Biodegradability of imidazolium and pyridinium ionic liquids by an activated sludge microbial community[J]. Biodegradation,2007,18(4):481-493.
[25]Gathergood N,Garcia M T,Scammells P J. Biodegradable ionic liquids:part Ⅰ. Concept,preliminary targets and evaluation[J]. Green Chemistry,2004,6(3):166-175.