膜法水处理中膜污染的化学控制研究进展
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摘要
膜过滤是一类重要的水处理技术,膜法水处理中膜污染是限制膜过滤技术推广应用的主要因素之一,减少和控制膜污染极为重要。化学法因其良好的处理效果和可操控性成为目前膜污染控制研究的热点。对国内外膜法水处理中关于化学控制膜污染的最新研究进展进行了分类和概括,总结了化学控制膜污染的主要技术手段,并对其主要技术原理及应用领域进行了阐述,最后对化学控制膜污染的研究重点及方向进行了展望。
Membrane filtration is a kind of important water treatment technology,but in membrane water treatment,membrane fouling is one of the main factors that restricts the popularization and application of membrane filtration technology. Reducing and controlling membrane fouling is very important. At present,the chemical method is a research hotspot on membrane fouling control because of its good treatment effects and controllability. The newest research progress in the chemical control over membrane fouling in membrane water treatment in China and abroad are classified and summarized. The main technical measures to control the membrane fouling by chemical method are also summarized. Their main technical theories and application fields are expounded. In addition,the research emphases and directions of chemical control over membrane fouling are predicted.
Membrane filtration is a kind of important water treatment technology,but in membrane water treatment,membrane fouling is one of the main factors that restricts the popularization and application of membrane filtration technology. Reducing and controlling membrane fouling is very important. At present,the chemical method is a research hotspot on membrane fouling control because of its good treatment effects and controllability. The newest research progress in the chemical control over membrane fouling in membrane water treatment in China and abroad are classified and summarized. The main technical measures to control the membrane fouling by chemical method are also summarized. Their main technical theories and application fields are expounded. In addition,the research emphases and directions of chemical control over membrane fouling are predicted.
引文
[1] Pulido J M. A review on the use of membrane technology and fouling control for olive mill wastewater treatment[J]. Science of the Total Environment,2016,563/564:664-675.
[2] Pourbozorg M,Li T,Law A W K. Effect of turbulence on fouling control of submerged hollow fibre membrane filtration[J]. Water Research,2016,99:101-111.
[3] Ruigomez I,Vera L,Gonzalez E,et al. A novel rotating HF membrane to control fouling on anaerobic membrane bioreactors treating wastewater[J]. Journal of Membrane Science,2016,501:45-52.
[4] Li Tian,Law A W K,Jiang Yishuai,et al. Fouling control of submerged hollow fibre membrane bioreactor with transverse vibration[J].Journal of Membrane Science,2016,505:216-224.
[5] Tan Yujun,Sun Lijuan,Li Bingtian,et al. Fouling characteristics and fouling control of reverse osmosis membranes for desalination of dyeing wastewater with high chemical oxygen demand[J]. Desalination,2017,419:1-7.
[6]陈俊平,杨昌柱,葛守飞,等.膜生物反应器在污水处理过程中的膜污染控制[J].净水技术,2005,24(3):38-44.
[7]康永,胡肖勇.膜污染机理与化学清洗方式研究[J].清洗世界,2012,28(2):28-33.
[8] Arhin S G,Banadda N,Komakech A J,et al. Membrane fouling control in low pressure membranes:A review on pretreatment techniques for fouling abatement[J]. Environmental Engineering Research,2016,21(2):109-120.
[9] Stoller M. On the effect of flocculation as pretreatment process and particle size distribution for membrane fouling reduction[J]. Desalination,2009,240(1):209-217.
[10] Ang W S,Tiraferri A. Fouling and cleaning of RO membranes fouled by mixtures of organic foulants simulating wastewater effluent[J].Journal of Membrane Science,2011,376(1):196-206.
[11] He Xiang,Meng Fangang,Lin Anli,et al. Monovalent ion-mediated fouling propensity of model proteins during low-pressure membrane filtration[J]. Separation&Purification Technology,2015,152:200-206.
[12] Abid H S,Johnson D J,Hashaikeh R,et al. A review of efforts to reduce membrane fouling by control of feed spacer characteristics[J].Desalination,2017,420:384-402.
[13] Hu Meng,Zheng Sunxiang,Mi Baoxia. Organic fouling of graphene oxide membranes and its implications for membrane fouling control in engineered osmosis[J]. Environmental Science&Technology,2016,50(2):685-693.
[14] Jelemensky M,Sharma A,Paulen R,et al. Time-optimal control of diafiltration processes in the presence of membrane fouling[J]. Computers&Chemical Engineering,2016,91:343-351.
[15]许云杰,吴俊杰.膜的改性及其在环境领域应用研究进展[J].四川环境,2009,28(4):108-112.
[16]岳鹏,丁昀,杨庆,等.超滤技术在城镇给水处理中的研究进展与应用[J].净水技术,2017,36(4):36-42.
[17] Wong L Y,Ng C A,Bashir M J K,et al. Enhancement of membrane fouling control in hybrid aerobic membrane bioreactor system for domestic waste water application:Effect of alum concentration[J].Procedia Engineering,2016,148:726-734.
[18] Cheng Xiaoxiang,Liang Heng,Qu Fangshu,et al. Fabrication of Mn oxide incorporated ceramic membranes for membrane fouling control and enhanced catalytic ozonation of p-chloronitrobenzene[J].Chemical Engineering Journal,2017,308:1010-1020.
[19] Kang Yan,Zheng Sunxiang,Finnerty C,et al. Regenerable polyelectrolyte membrane for ultimate fouling control in forward osmosis[J]. Environmental Science&Technology,2017,51(6):3242-3249.
[20]钟明强,刘俊华.聚丙烯共混改性研究进展[J].中国塑料,1999(9):9-19.
[21] Hester J F,Banerjee P A,Mayes A M. Preparation of protein-resistant surfaces on poly(vinylidene fluoride)membranes via surface segregation[J]. Macromolecules,1999,32(5):1643-1650.
[22]李金桂.材料的表面改性与涂覆技术的新进展[J].腐蚀与防护,1999(2):51-55.
[23] Cheng Zhenping,Zhu Xiulin,And E T K,et al. Modification of poly(ether imide)membranes via surface-initiated atom transfer radical polymerization[J]. Macromolecules,2006,39(4):1660-1663.
[24] Wang P,Tan K L,Kang E T,et al. Plasma-induced immobilization of poly(ethylene glycol)onto poly(vinylidene fluoride)microporous membrane[J]. Journal of Membrane Science,2002,195(1):103-114.
[25] Becker W,Schmidt-Naake G. Proton exchange membranes by irradiation induced grafting of styrene onto FEP and ETFE:Influences of the crosslinker N,N-methylene-bis-acrylamide[J]. Chemical Engineering&Technology,2002,25(4):373-377.
[26] Xu Zhikang,Dai Qingwen,Wu Jian,et al. Covalent attachment of phospholipid analogous polymers to modify a polymeric membrane surface:A novel approach[J]. Langmuir,2004,20(4):1481-1488.
[27] Borea L,Naddeo V,Belgiorno V. Application of electrochemical processes to membrane bioreactors for improving nutrient removal and fouling control[J]. Environmental Science and Pollution Research,2017,24(1):321-333.
[28] Ensano B M B,Borea L,Naddeo V,et al. Combination of electrochemical processes with membrane bioreactors for wastewater treatment and fouling control:A review[J]. Frontiers in Environmental Science,2016,4(57):1-15.
[29]毕芳华,贾辉,王捷,等.基于MFC电场强化的MBR膜污染控制[J].化工学报,2015,66(12):5103-5110.
[30]杨怡婷,王磊,孟晓荣,等.在线清洗对倒置A2/O-MBR复合膜污染控制研究[J].水处理技术,2015,41(7):113-116.
[31] Cheng Xiaoxiang,Liang Heng,Ding An,et al. Ferrous iron/peroxymonosulfate oxidation as a pretreatment for ceramic ultrafiltration membrane:Control of natural organic matter fouling and degradation of atrazine[J]. Water Research,2017,113:32-41.
[32] Wei Xinyu,Wang Zhi,Fan Fanghui,et al. Advanced treatment of a complex pharmaceutical wastewater by nanofiltration:Membrane foulant identification and cleaning[J]. Desalination,2010,251(1):167-175.
[33]梁钟璇. MEUF中超滤膜污染特征及膜的清洗[D].湖南:湖南大学,2010.
[34] Lee H,Amy G,Cho J,et al. Cleaning strategies for flux recovery of an ultrafiltration membrane fouled by natural organic matter[J].Water Research,2001,35(14):3301-3308.
[35]葛旭东,高瑞昶.古龙酸纳滤浓缩过程的膜污染及膜清洗[J].化学工业与工程,2008,25(1):28-31.
[36] Lu Jun,Liu Ning,Li Liangxiong,et al. Organic fouling and regeneration of zeolite membrane in wastewater treatment[J]. Separation&Purification Technology,2010,72(2):203-207.
[37] Madaeni S S,Mansourpanah Y. Chemical cleaning of reverse osmosis membranes fouled by whey[J]. Desalination,2001,161(1):13-24.
[38] Kuzmenko D,Arkhangelsky E,Belfer S,et al. Chemical cleaning of UF membranes fouled by BSA[J]. Desalination,2005,179(1):323-333.
[39] Kazemimoghadam M,Mohammadi T. Chemical cleaning of ultrafiltration membranes in the milk industry[J]. Desalination,2007,204(1):213-218.
[40]陈禹志.预氧化强化混凝-膜除藻工艺膜污染控制研究[J].膜科学与技术,2016,36(1):104-108.
[41] Yan Zhongsen,Liu Bin,Qu Fangshu,et al. Control of ultrafiltration membrane fouling caused by algal extracellular organic matter(EOM)using enhanced Al coagulation with permanganate[J]. Separation and Purification Technology,2017,172:51-58.
[42] Prado M,Borea L,Cesaro A,et al. Removal of emerging contaminant and fouling control in membrane bioreactors by combined ozonation and sonolysis[J]. International Biodeterioration&Biodegradation,2017,119:577-586.
[43] Yu W,Campos L C,Graham N. Application of pulsed UV-irradiation and pre-coagulation to control ultrafiltration membrane fouling in the treatment of micro-polluted surface water[J]. Water Research,2016,107:83-92.
[44] Aslam M,Charfi A,Kim J. Membrane scouring to control fouling under fluidization of non-adsorbing media for wastewater treatment[J/OL]. Environmental Science&Pollution Research,2017:1-11[2017-02-11]. http:∥doi.org/10.1007/s11356-017-8527-2.
[45] Mei Xiaojie,Pei J Q,Wang Zhiwei,et al. Alkali-assisted membrane cleaning for fouling control of anaerobic ceramic membrane bioreactor[J]. Bioresource Technology,2017,240:25-32.
[46] Huang Weiwei,Hu Mengliu,Zhou Wenzong,et al. Effects of combined ozone and PAC pretreatment on ultrafiltration membrane fouling control and mechanisms[J]. Journal of Membrane Science,2017,533:379-389.
[2] Pourbozorg M,Li T,Law A W K. Effect of turbulence on fouling control of submerged hollow fibre membrane filtration[J]. Water Research,2016,99:101-111.
[3] Ruigomez I,Vera L,Gonzalez E,et al. A novel rotating HF membrane to control fouling on anaerobic membrane bioreactors treating wastewater[J]. Journal of Membrane Science,2016,501:45-52.
[4] Li Tian,Law A W K,Jiang Yishuai,et al. Fouling control of submerged hollow fibre membrane bioreactor with transverse vibration[J].Journal of Membrane Science,2016,505:216-224.
[5] Tan Yujun,Sun Lijuan,Li Bingtian,et al. Fouling characteristics and fouling control of reverse osmosis membranes for desalination of dyeing wastewater with high chemical oxygen demand[J]. Desalination,2017,419:1-7.
[6]陈俊平,杨昌柱,葛守飞,等.膜生物反应器在污水处理过程中的膜污染控制[J].净水技术,2005,24(3):38-44.
[7]康永,胡肖勇.膜污染机理与化学清洗方式研究[J].清洗世界,2012,28(2):28-33.
[8] Arhin S G,Banadda N,Komakech A J,et al. Membrane fouling control in low pressure membranes:A review on pretreatment techniques for fouling abatement[J]. Environmental Engineering Research,2016,21(2):109-120.
[9] Stoller M. On the effect of flocculation as pretreatment process and particle size distribution for membrane fouling reduction[J]. Desalination,2009,240(1):209-217.
[10] Ang W S,Tiraferri A. Fouling and cleaning of RO membranes fouled by mixtures of organic foulants simulating wastewater effluent[J].Journal of Membrane Science,2011,376(1):196-206.
[11] He Xiang,Meng Fangang,Lin Anli,et al. Monovalent ion-mediated fouling propensity of model proteins during low-pressure membrane filtration[J]. Separation&Purification Technology,2015,152:200-206.
[12] Abid H S,Johnson D J,Hashaikeh R,et al. A review of efforts to reduce membrane fouling by control of feed spacer characteristics[J].Desalination,2017,420:384-402.
[13] Hu Meng,Zheng Sunxiang,Mi Baoxia. Organic fouling of graphene oxide membranes and its implications for membrane fouling control in engineered osmosis[J]. Environmental Science&Technology,2016,50(2):685-693.
[14] Jelemensky M,Sharma A,Paulen R,et al. Time-optimal control of diafiltration processes in the presence of membrane fouling[J]. Computers&Chemical Engineering,2016,91:343-351.
[15]许云杰,吴俊杰.膜的改性及其在环境领域应用研究进展[J].四川环境,2009,28(4):108-112.
[16]岳鹏,丁昀,杨庆,等.超滤技术在城镇给水处理中的研究进展与应用[J].净水技术,2017,36(4):36-42.
[17] Wong L Y,Ng C A,Bashir M J K,et al. Enhancement of membrane fouling control in hybrid aerobic membrane bioreactor system for domestic waste water application:Effect of alum concentration[J].Procedia Engineering,2016,148:726-734.
[18] Cheng Xiaoxiang,Liang Heng,Qu Fangshu,et al. Fabrication of Mn oxide incorporated ceramic membranes for membrane fouling control and enhanced catalytic ozonation of p-chloronitrobenzene[J].Chemical Engineering Journal,2017,308:1010-1020.
[19] Kang Yan,Zheng Sunxiang,Finnerty C,et al. Regenerable polyelectrolyte membrane for ultimate fouling control in forward osmosis[J]. Environmental Science&Technology,2017,51(6):3242-3249.
[20]钟明强,刘俊华.聚丙烯共混改性研究进展[J].中国塑料,1999(9):9-19.
[21] Hester J F,Banerjee P A,Mayes A M. Preparation of protein-resistant surfaces on poly(vinylidene fluoride)membranes via surface segregation[J]. Macromolecules,1999,32(5):1643-1650.
[22]李金桂.材料的表面改性与涂覆技术的新进展[J].腐蚀与防护,1999(2):51-55.
[23] Cheng Zhenping,Zhu Xiulin,And E T K,et al. Modification of poly(ether imide)membranes via surface-initiated atom transfer radical polymerization[J]. Macromolecules,2006,39(4):1660-1663.
[24] Wang P,Tan K L,Kang E T,et al. Plasma-induced immobilization of poly(ethylene glycol)onto poly(vinylidene fluoride)microporous membrane[J]. Journal of Membrane Science,2002,195(1):103-114.
[25] Becker W,Schmidt-Naake G. Proton exchange membranes by irradiation induced grafting of styrene onto FEP and ETFE:Influences of the crosslinker N,N-methylene-bis-acrylamide[J]. Chemical Engineering&Technology,2002,25(4):373-377.
[26] Xu Zhikang,Dai Qingwen,Wu Jian,et al. Covalent attachment of phospholipid analogous polymers to modify a polymeric membrane surface:A novel approach[J]. Langmuir,2004,20(4):1481-1488.
[27] Borea L,Naddeo V,Belgiorno V. Application of electrochemical processes to membrane bioreactors for improving nutrient removal and fouling control[J]. Environmental Science and Pollution Research,2017,24(1):321-333.
[28] Ensano B M B,Borea L,Naddeo V,et al. Combination of electrochemical processes with membrane bioreactors for wastewater treatment and fouling control:A review[J]. Frontiers in Environmental Science,2016,4(57):1-15.
[29]毕芳华,贾辉,王捷,等.基于MFC电场强化的MBR膜污染控制[J].化工学报,2015,66(12):5103-5110.
[30]杨怡婷,王磊,孟晓荣,等.在线清洗对倒置A2/O-MBR复合膜污染控制研究[J].水处理技术,2015,41(7):113-116.
[31] Cheng Xiaoxiang,Liang Heng,Ding An,et al. Ferrous iron/peroxymonosulfate oxidation as a pretreatment for ceramic ultrafiltration membrane:Control of natural organic matter fouling and degradation of atrazine[J]. Water Research,2017,113:32-41.
[32] Wei Xinyu,Wang Zhi,Fan Fanghui,et al. Advanced treatment of a complex pharmaceutical wastewater by nanofiltration:Membrane foulant identification and cleaning[J]. Desalination,2010,251(1):167-175.
[33]梁钟璇. MEUF中超滤膜污染特征及膜的清洗[D].湖南:湖南大学,2010.
[34] Lee H,Amy G,Cho J,et al. Cleaning strategies for flux recovery of an ultrafiltration membrane fouled by natural organic matter[J].Water Research,2001,35(14):3301-3308.
[35]葛旭东,高瑞昶.古龙酸纳滤浓缩过程的膜污染及膜清洗[J].化学工业与工程,2008,25(1):28-31.
[36] Lu Jun,Liu Ning,Li Liangxiong,et al. Organic fouling and regeneration of zeolite membrane in wastewater treatment[J]. Separation&Purification Technology,2010,72(2):203-207.
[37] Madaeni S S,Mansourpanah Y. Chemical cleaning of reverse osmosis membranes fouled by whey[J]. Desalination,2001,161(1):13-24.
[38] Kuzmenko D,Arkhangelsky E,Belfer S,et al. Chemical cleaning of UF membranes fouled by BSA[J]. Desalination,2005,179(1):323-333.
[39] Kazemimoghadam M,Mohammadi T. Chemical cleaning of ultrafiltration membranes in the milk industry[J]. Desalination,2007,204(1):213-218.
[40]陈禹志.预氧化强化混凝-膜除藻工艺膜污染控制研究[J].膜科学与技术,2016,36(1):104-108.
[41] Yan Zhongsen,Liu Bin,Qu Fangshu,et al. Control of ultrafiltration membrane fouling caused by algal extracellular organic matter(EOM)using enhanced Al coagulation with permanganate[J]. Separation and Purification Technology,2017,172:51-58.
[42] Prado M,Borea L,Cesaro A,et al. Removal of emerging contaminant and fouling control in membrane bioreactors by combined ozonation and sonolysis[J]. International Biodeterioration&Biodegradation,2017,119:577-586.
[43] Yu W,Campos L C,Graham N. Application of pulsed UV-irradiation and pre-coagulation to control ultrafiltration membrane fouling in the treatment of micro-polluted surface water[J]. Water Research,2016,107:83-92.
[44] Aslam M,Charfi A,Kim J. Membrane scouring to control fouling under fluidization of non-adsorbing media for wastewater treatment[J/OL]. Environmental Science&Pollution Research,2017:1-11[2017-02-11]. http:∥doi.org/10.1007/s11356-017-8527-2.
[45] Mei Xiaojie,Pei J Q,Wang Zhiwei,et al. Alkali-assisted membrane cleaning for fouling control of anaerobic ceramic membrane bioreactor[J]. Bioresource Technology,2017,240:25-32.
[46] Huang Weiwei,Hu Mengliu,Zhou Wenzong,et al. Effects of combined ozone and PAC pretreatment on ultrafiltration membrane fouling control and mechanisms[J]. Journal of Membrane Science,2017,533:379-389.