Recent advances in active sites identification and regulation of M-N/C electro-catalysts towards ORR
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摘要
Transition metal and nitrogen co-doped carbon(M–N/C) catalysts are recognized as the most prospective alternatives for platinum-based electro-catalysts towards oxygen reduction reaction(ORR) in polymer electrolyte fuel cells. Recently, significant progress has been achieved in the identification and regulation of active sites of this kind of catalysts. In this mini review,we summarize the techniques and strategies to identify active sites in M–N/C catalysts, the main debates on active sites types, the measurement method for active site density, the reactivity descriptors for M–N/C catalysts, and directions to the design of ORR M–N/C catalysts.
Transition metal and nitrogen co-doped carbon(M–N/C) catalysts are recognized as the most prospective alternatives for platinum-based electro-catalysts towards oxygen reduction reaction(ORR) in polymer electrolyte fuel cells. Recently, significant progress has been achieved in the identification and regulation of active sites of this kind of catalysts. In this mini review,we summarize the techniques and strategies to identify active sites in M–N/C catalysts, the main debates on active sites types, the measurement method for active site density, the reactivity descriptors for M–N/C catalysts, and directions to the design of ORR M–N/C catalysts.
Transition metal and nitrogen co-doped carbon(M–N/C) catalysts are recognized as the most prospective alternatives for platinum-based electro-catalysts towards oxygen reduction reaction(ORR) in polymer electrolyte fuel cells. Recently, significant progress has been achieved in the identification and regulation of active sites of this kind of catalysts. In this mini review,we summarize the techniques and strategies to identify active sites in M–N/C catalysts, the main debates on active sites types, the measurement method for active site density, the reactivity descriptors for M–N/C catalysts, and directions to the design of ORR M–N/C catalysts.
引文
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54 Chen X,Yu L,Wang S,Deng D,Bao X.Nano Energy,2017,32:353-358
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59 Lim KH,Kim H.Appl Catal B-Environ,2014,158-159:355-360
60 Deng J,Ren P,Deng D,Yu L,Yang F,Bao X.Energy Environ Sci,2014,7:1919-1923
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67 Liang W,Chen J,Liu Y,Chen S.ACS Catal,2014,4:4170-4177
68 Meng H,Jaouen F,Proietti E,Lefèvre M,Dodelet JP.Electrochem Commun,2009,11:1986-1989
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2 Sa YJ,Kim JH,Joo SH.J Electrochem Sci Te,2017,8:169-182
3 Wang Y,Li J,Wei Z.ChemElectroChem,2018,5:1764-1774
4 Huo P,Zhao P,Wang Y,Liu B,Yin G,Dong M.Energies,2018,11:167
5 Kang SY,Kim HJ,Chung YH.Nano Converg,2018,5:13
6 Kiani M,Zhang J,Luo Y,Jiang C,Fan J,Wang G,Chen J,Wang R.JEnergy Chem,2018,27:1124-1139
7 Li JC,Hou PX,Liu C.Small,2017,13:1702002
8 Li R,Zhang D,Zhou Y,Wang X,Guo G.Sci China Chem,2016,59:746-751
9 Lu S,Jin Y,Gu H,Zhang W.Sci China Chem,2017,60:999-1006
10 Ma J,Xiang Z,Zhang J.Sci China Chem,2018,61:592-597
11 Tong X,Wei Q,Zhan X,Zhang G,Sun S.Catalysts,2016,7:1
12 Chong L,Wen J,Kubal J,Sen FG,Zou J,Greeley J,Chan M,Barkholtz H,Ding W,Liu DJ.Science,2018,362:1276-1281
13 Jasinski R.Nature,1964,201:1212-1213
14 Jahnke HMS,Zimmermann G.Top Curr Chem,1976,61:131-181
15 Gupta S,Tryk D,Bae I,Aldred W,Yeager E.J Appl Electrochem,1989,19:19-27
16 Shao M,Chang Q,Dodelet JP,Chenitz R.Chem Rev,2016,116:3594-3657
17 Goellner V,Armel V,Zitolo A,Fonda E,Jaouen F.J Electrochem Soc,2015,162:H403-H414
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19 Masa J,Xia W,Muhler M,Schuhmann W.Angew Chem Int Ed,2015,54:10102-10120
20 Ren Q,Wang H,Lu XF,Tong YX,Li GR.Adv Sci,2018,5:1700515
21 Song Z,Cheng N,Lushington A,Sun X.Catalysts,2016,6:116
22 Huang X,Wang Y,Li W,Hou Y.Sci China Chem,2017,60:1494-1507
23 Yeager E.Electrochim Acta,1984,29:1527-1537
24 Xiong D,Li X,Fan L,Bai Z.Catalysts,2018,8:301
25 Borghei M,Lehtonen J,Liu L,Rojas OJ.Adv Mater,2018,30:1703691
26 Fukuzumi S,Lee YM,Nam W.ChemCatChem,2018,10:9-28
27 Ji Y,Dong H,Liu C,Li Y.J Mater Chem A,2018,6:13489-13508
28 Choi CH,Lim HK,Chung MW,Chon G,Ranjbar Sahraie N,Altin A,Sougrati MT,Stievano L,Oh HS,Park ES,Luo F,Strasser P,Dra?i?G,Mayrhofer KJJ,Kim H,Jaouen F.Energy Environ Sci,2018,11:3176-3182
29 Barbusinski K.Ecol Chem Eng S,2009,16:347-358
30 Nandan R,Gautam A,Nanda KK.J Mater Chem A,2017,5:20252-20262
31 Singh D,Mamtani K,Bruening CR,Miller JT,Ozkan US.ACSCatal,2014,4:3454-3462
32 Hu Y,Jensen JO,Zhang W,Martin S,Chenitz R,Pan C,Xing W,Bjerrum NJ,Li Q.J Mater Chem A,2015,3:1752-1760
33 Hu Y,Jensen JO,Zhang W,Cleemann LN,Xing W,Bjerrum NJ,Li Q.Angew Chem Int Ed,2014,53:3675-3679
34 Guo D,Shibuya R,Akiba C,Saji S,Kondo T,Nakamura J.Science,2016,351:361-365
35 Cui X,Yang S,Yan X,Leng J,Shuang S,Ajayan PM,Zhang Z.Adv Funct Mater,2016,26:5708-5717
36 Choi CH,Baldizzone C,Polymeros G,Pizzutilo E,Kasian O,Schuppert AK,Ranjbar Sahraie N,Sougrati MT,Mayrhofer KJJ,Jaouen F.ACS Catal,2016,6:3136-3146
37 Jia Q,Ramaswamy N,Tylus U,Strickland K,Li J,Serov A,Artyushkova K,Atanassov P,Anibal J,Gumeci C,Barton SC,Sougrati MT,Jaouen F,Halevi B,Mukerjee S.Nano Energy,2016,29:65-82
38 Wang N,Lu B,Li L,Niu W,Tang Z,Kang X,Chen S.ACS Catal,2018,8:6827-6836
39 Kramm UI,Herranz J,Larouche N,Arruda TM,Lefèvre M,Jaouen F,Bogdanoff P,Fiechter S,Abs-Wurmbach I,Mukerjee S,Dodelet JP.Phys Chem Chem Phys,2012,14:11673-11688
40 Xiao M,Zhu J,Ma L,Jin Z,Ge J,Deng X,Hou Y,He Q,Li J,Jia Q,Mukerjee S,Yang R,Jiang Z,Su D,Liu C,Xing W.ACS Catal,2018,8:2824-2832
41 Zhong L,Frandsen C,M?rup S,Hu Y,Pan C,Cleemann LN,Jensen JO,Li Q.Appl Catal B-Environ,2018,221:406-412
42 Lefèvre M,Dodelet JP,Bertrand P.J Phys Chem B,2002,106:8705-8713
43 Palaniselvam T,Kashyap V,Bhange SN,Baek JB,Kurungot S.Adv Funct Mater,2016,26:2150-2162
44 Kim D,Li OL,Saito N.Phys Chem Chem Phys,2014,16:14905-14911
45 Artyushkova K,Serov A,Rojas-Carbonell S,Atanassov P.J Phys Chem C,2015,119:25917-25928
46 Jia Q,Liu E,Jiao L,Pann S,Mukerjee S.Adv Mater,2018:e1805157
47 Tylus U,Jia Q,Strickland K,Ramaswamy N,Serov A,Atanassov P,Mukerjee S.J Phys Chem C,2014,118:8999-9008
48 Ren H,Wang Y,Yang Y,Tang X,Peng Y,Peng H,Xiao L,Lu J,Abru?a HD,Zhuang L.ACS Catal,2017,7:6485-6492
49 Chung HT,Cullen DA,Higgins D,Sneed BT,Holby EF,More KL,Zelenay P.Science,2017,357:479-484
50 Pfisterer JHK,Liang Y,Schneider O,Bandarenka AS.Nature,2017,549:74-77
51 Fazio G,Ferrighi L,Perilli D,Di Valentin C.Int J Quantum Chem,2016,116:1623-1640
52 Holby EF,Zelenay P.Nano Energy,2016,29:54-64
53 Zheng Y,Yang DS,Kweun JM,Li C,Tan K,Kong F,Liang C,Chabal YJ,Kim YY,Cho M,Yu JS,Cho K.Nano Energy,2016,30:443-449
54 Chen X,Yu L,Wang S,Deng D,Bao X.Nano Energy,2017,32:353-358
55 Sebastián D,Serov A,Matanovic I,Artyushkova K,Atanassov P,AricòAS,Baglio V.Nano Energy,2017,34:195-204
56 Yang L,Cheng D,Xu H,Zeng X,Wan X,Shui J,Xiang Z,Cao D.Proc Natl Acad Sci USA,2018,115:6626-6631
57 Gu W,Hu L,Li J,Wang E.Electroanalysis,2018,30:1217-1228
58 Wang Y,Luo E,Xiao M,Ge J,Liu C,Xing W.Sci Sin Chem,2017,47:554-564
59 Lim KH,Kim H.Appl Catal B-Environ,2014,158-159:355-360
60 Deng J,Ren P,Deng D,Yu L,Yang F,Bao X.Energy Environ Sci,2014,7:1919-1923
61 Sahraie NR,Kramm UI,Steinberg J,Zhang Y,Thomas A,Reier T,Paraknowitsch JP,Strasser P.Nat Commun,2015,6:8618
62 Malko D,Kucernak A,Lopes T.Nat Commun,2016,7:13285
63 Ohtsuka M,Kitamura F.Electrochemistry,2015,83:376-380
64 Kattel S,Wang G.J Mater Chem A,2013,1:10790
65 Ramaswamy N,Tylus U,Jia Q,Mukerjee S.J Am Chem Soc,2013,135:15443-15449
66 Kramm UI,Herrmann-Geppert I,Behrends J,Lips K,Fiechter S,Bogdanoff P.J Am Chem Soc,2016,138:635-640
67 Liang W,Chen J,Liu Y,Chen S.ACS Catal,2014,4:4170-4177
68 Meng H,Jaouen F,Proietti E,Lefèvre M,Dodelet JP.Electrochem Commun,2009,11:1986-1989
69 Han Y,Wang Y,Xu R,Chen W,Zheng L,Han A,Zhu Y,Zhang J,Zhang H,Luo J,Chen C,Peng Q,Wang D,Li Y.Energy Environ Sci,2018,11:2348-2352
70 Wu YJ,Wang YC,Wang RX,Zhang PF,Yang XD,Yang HJ,Li JT,Zhou Y,Zhou ZY,Sun SG.ACS Appl Mater Interfaces,2018,10:14602-14613
71 Xiao M,Zhang H,Chen Y,Zhu J,Gao L,Jin Z,Ge J,Jiang Z,Chen S,Liu C,Xing W.Nano Energy,2018,46:396-403
72 Xiao J,Xu Y,Xia Y,Xi J,Wang S.Nano Energy,2016,24:121-129
73 Hu Z,Guo Z,Zhang Z,Dou M,Wang F.ACS Appl Mater Interfaces,2018,10:12651-12658
74 Osmieri L,Escudero-Cid R,Armandi M,Monteverde Videla AHA,García Fierro JL,Ocón P,Specchia S.Appl Catal B-Environ,2017,205:637-653
75 Ratso S,Kruusenberg I,K??rik M,Kook M,Saar R,Kanninen P,Kallio T,Leis J,Tammeveski K.Appl Catal B-Environ,2017,219:276-286
76 Domínguez C,Pérez-Alonso FJ,Salam MA,Al-Thabaiti SA,Pe?a MA,García-García FJ,Barrio L,Rojas S.Appl Catal B-Environ,2016,183:185-196
77 Lee S,Kwak DH,Han SB,Lee YW,Lee JY,Choi IA,Park HS,Park JY,Park KW.ACS Catal,2016,6:5095-5102
78 Pascone PA,de Campos J,Meunier JL,Berk D.Appl Catal B-Environ,2016,193:9-15
79 Yasuda S,Furuya A,Uchibori Y,Kim J,Murakoshi K.Adv Funct Mater,2016,26:738-744
80 Wang B,Wang X,Zou J,Yan Y,Xie S,Hu G,Li Y,Dong A.Nano Lett,2017,17:2003-2009
81 Lai Q,Zheng L,Liang Y,He J,Zhao J,Chen J.ACS Catal,2017,7:1655-1663
82 Wei W,Shi X,Gao P,Wang S,Hu W,Zhao X,Ni Y,Xu X,Xu Y,Yan W,Ji H,Cao M.Nano Energy,2018,52:29-37
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