Improving the Accuracy of Daily PM2.5 Distributions Derived from the Fusion of Ground-Level Measurements with Aerosol Optical Depth Observations, a Case Study in North China

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• 作者：Baolei Lv ; Yongtao Hu ; Howard H. Chang ; Armistead G. Russell ; Yuqi Bai
• 刊名：Environmental Science & Technology
• 出版年：2016
• 出版时间：May 3, 2016
• 年：2016
• 卷：50
• 期：9
• 页码：4752-4759
• 全文大小：492K
• 年卷期：0
• ISSN：1520-5851

文摘

The accuracy in estimated fine particulate matter concentrations (PM_2.5), obtained by fusing of station-based measurements and satellite-based aerosol optical depth (AOD), is often reduced without accounting for the spatial and temporal variations in PM_2.5 and missing AOD observations. In this study, a city-specific linear regression model was first developed to fill in missing AOD data. A novel interpolation-based variable, PM_2.5 spatial interpolator (PMSI_2.5), was also introduced to account for the spatial dependence in PM_2.5 across grid cells. A Bayesian hierarchical model was then developed to estimate spatiotemporal relationships between AOD and PM_2.5. These methods were evaluated through a city-specific 10-fold cross-validation procedure in a case study in North China in 2014. The cross validation R² was 0.61 when PMSI_2.5 was included and 0.48 when PMSI_2.5 was excluded. The gap-filled AOD values also effectively improved predicted PM_2.5 concentrations with an R² = 0.78. Daily ground-level PM_2.5 concentration fields at a 12 km resolution were predicted with complete spatial and temporal coverage. This study also indicates that model prediction performance should be assessed by accounting for monitor clustering due to the potential misinterpretation of model accuracy in spatial prediction when validation monitors are randomly selected.