Novel Insights into Fukushima Nuclear Accident from Isotopic Evidence of Plutonium Spread along Coastal Rivers

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• 作者：Olivier Evrard ; Fabien Pointurier ; Yuichi Onda ; Caroline Chartin ; Am茅lie Hubert ; Hugo Lepage ; Anne-Claire Pottin ; Ir猫ne Lef猫vre ; Philippe Bont茅 ; J. Patrick Laceby ; Sophie Ayrault
• 刊名：Environmental Science & Technology
• 出版年：2014
• 出版时间：August 19, 2014
• 年：2014
• 卷：48
• 期：16
• 页码：9334-9340
• 全文大小：333K
• ISSN：1520-5851

文摘

The Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident led to important releases of radionuclides into the environment, and trace levels of plutonium (Pu) were detected in northeastern Japan. However, measurements of Pu isotopic atom and activity ratios are required to differentiate between the contributions of global nuclear test fallout and FDNPP emissions. In this study, we used a double-focusing sector field ICP鈥揗S to measure Pu atom and activity ratios in recently deposited sediment along rivers draining the most contaminated part of the inland radioactive plume. Results showed that plutonium isotopes (i.e., ²³⁹Pu, ²⁴⁰Pu, ²⁴¹Pu, and ²⁴²Pu) were detected in all samples, although in extremely low concentrations. The ²⁴¹Pu/²³⁹Pu atom ratios measured in sediment deposits (0.0017鈥?.0884) were significantly higher than the corresponding values attributed to the global fallout (0.00113 卤 0.00008 on average for the Northern Hemisphere between 31掳鈥?1掳 N: Kelley, J. M.; Bond, L. A.; Beasley, T. M. Global distribution of Pu isotopes and ²³⁷Np. Sci. Total. Env. 1999, 237/238, 483鈥?00). The results indicated the presence of Pu from FDNPP, in slight excess compared to the Pu background from global fallout that represented up to ca. 60% of Pu in the analyzed samples. These results demonstrate that this radionuclide has been transported relatively long distances (45 km) from FDNPP and been deposited in rivers representing a potential source of Pu to the ocean. In future, the high ²⁴¹Pu/²³⁹Pu atom ratio of the Fukushima accident sourced-Pu should be measured to quantify the supply of continental-originating material from Fukushima Prefecture to the Pacific Ocean.