Metal distribution and bioavailability in surface sediments from the Huaihe River, Anhui, China

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• 作者：Jie Wang ; Guijian Liu ; lanlan Lu ; Houqi Liu
• 关键词：Trace metal ; Speciation ; Sediment ; RAC ; Correlation analysis ; Huaihe River
• 刊名：Environmental Monitoring and Assessment
• 出版年：2016
• 出版时间：January 2016
• 年：2016
• 卷：188
• 期：1
• 全文大小：1,352 KB
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• 作者单位：Jie Wang (1) (2)
  Guijian Liu (1) (2)
  lanlan Lu (1)
  Houqi Liu (1)
  
  1. CAS Key Laboratory of Crust-Mantle Materials and the Environments, School of Earth and Space Sciences, University of Science and Technology of China, Hefei, 230026, China
  2. State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, The Chinese Academy of Sciences, Xi鈥檃n, Shaanxi, 710075, China
  
• 刊物类别：Earth and Environmental Science
• 刊物主题：Environment
  Monitoring, Environmental Analysis and Environmental Ecotoxicology
  Ecology
  Atmospheric Protection, Air Quality Control and Air Pollution
  Environmental Management
  
• 出版者：Springer Netherlands
• ISSN：1573-2959

文摘

This study presents the total concentrations and chemical fractionations of metals (Cu, Pb, Zn, Ni, Fe, and Mn) in 54 surface sediment samples collected from the Huaihe River (Anhui Province) in eastern China. Compared with the average shale values, Zn and Pb exhibited the most substantial anthropogenic enrichment, especially in Fengtai and Huainan areas, the main industrial districts along the Huaihe River (Anhui Province). Low levels of Cu and Ni were observed in the sediments. Based on risk assessment code (RAC), the metals associated with weak acid soluble (F1) in the Huaihe River sediments followed the order: Mn鈥?gt;鈥塟n鈥?gt;鈥塁u鈥?gt;鈥塒b鈥?gt;鈥塏i鈥?gt;鈥塅e. Manganese presented the most potential for releasing into the aqueous environment and can easily enter the food chain. Copper, zinc, nickel, and iron were found dominant in the residual fraction, implying that these four metals were strongly bound to the sediments. Lead showed a different partitioning pattern from that of other metals studied, with a large percentage in Fe-Mn oxide fraction, indicating that slight redox potential changes may make significant influence on the removability of Pb. Moreover, Cu in oxidizable (F3) and residual (F4) fractions presented high positive correlation with organic matter, which can explain the high percentage of Cu in these two fractions. Keywords Trace metal Speciation Sediment RAC Correlation analysis Huaihe River