Distribution, source identification, and historical trends of organic micropollutants in coastal sediment in Jakarta Bay, Indonesia

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• 作者：Rinawati^a ; ^b ; Tatsuya Koike^a ; Hiroaki Koike^a ; Rina Kurumisawa^a ; Maki Ito^a ; Shigeaki Sakurai^a ; Ayako Togo^a ; Mahua Saha^a ; Zainal Arifin^c ; Hideshige Takada^a ; ^{shige@cc.tuat.ac.jp}
• 关键词：Polycyclic aromatic hydrocarbon (PAH) ; Polychlorinated biphenyl (PCB) ; Linear alkylbenzene (LABs) ; Hopane ; Molecular marker
• 刊名：Journal of Hazardous Materials
• 出版年：2012
• 期刊代码：50_03043894
• 类别：ce
• 出版时间：30 May, 2012
• 卷：217-218
• 期：Complete
• 页码：208-216
• 文件大小：601 K

摘要

We determined concentrations of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), linear alkylbenzenes (LABs), and hopanes in coastal sediments collected from Jakarta Bay and Tokyo Bay. PAH concentrations in sediments from Jakarta Bay (257-1511 ng/g-dry) were lower than or comparable to those from Tokyo Bay (1372-1615 ng/g-dry). Ratios of alkyl-PAHs to parent PAHs showed a greater contribution of petrogenic inputs in Jakarta Bay than in Tokyo Bay. This difference is consistent with the higher ratio of hopanes to PAHs in Jakarta Bay. LAB concentrations in Jakarta Bay (geometric mean, 1400 ng/g-dry) were higher than those in Tokyo Bay (661 ng/g-dry). The internal to external (I/E) ratios of LABs in Jakarta Bay (0.92-2.88) were lower than those in Tokyo Bay (2.8-4.8), indicating that Jakarta Bay receives untreated or poorly treated sewage. Significant amounts of tetrapropylene-based alkylbenzenes were detected in several locations in Jakarta Bay, suggesting current usage of the non-degradable surfactants alkylbenzene sulfonates that are banned in many countries. The PCB concentration in Jakarta Bay was 1 order of magnitude lower than in Tokyo Bay, suggesting minimal usage of PCBs in industrial or commercial products in Jakarta. Analyses of a sediment core indicate increasing inputs of PAHs, hopanes, and LABs into Jakarta Bay during recent decades.