南黄海盆地古近系烃源岩地球化学特征及油源对比
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摘要
南黄海盆地古近系烃源岩生烃潜力及原油来源,目前研究比较薄弱.通过对南部坳陷烃源岩和原油样品的有机地球化学分析,揭示古近系烃源岩和原油地球化学特征,并进行油源对比.结果表明南部坳陷古近系烃源岩主要发育在阜四段和阜二段,有机质丰度中等-好,有机质类型为Ⅱ_2-Ⅲ型,有机质为低成熟-成熟阶段.阜四段烃源岩形成于贫氧、较高盐度环境,阜二段烃源岩形成于厌氧、相对低盐度环境.原油的饱和烃含量较高,UCM鼓峰较小,已进入成熟阶段,对比结果显示戴南组原油可能来源于阜四段烃源岩,而阜三段原油可能与阜二段烃源岩有关.
Researches on the hydrocarbon potential of the source rock in the Paleogene Funing Formation,and origin of the Paleogene crude oil in the southern depression of the South Yellow Sea Basin(SYSB)are relatively weak.Based on the systematically organic geochemical analyses(TOC,Rock-Eval,GC-MS of saturates and aromatics,stable carbon isotope)of the Paleogene core,cuttings,oil sand and crude oil samples,combined with vitrinite reflectance determination,the geochemical characteristics of source rocks and crude oil are revealed,and oil-source correlation is obtained.The results indicate that the Paleogene source rocks in the southern depression mainly deposited in the fourth (E_1f_4) and second memebers (E_1f_2) of Funing Formation,with moderate-good organic matter(OM)abundance,type Ⅱ_2-Ⅲ kerogen and within low mature-mature stage.Mixed OM sources,dominated by terrestrial OM are observed in E_1f_4 and E_1f_2 source rocks,biomarker ratios indicate that E_1f_4source rocks were deposited in dysoxic,relatively high salinity condition.Whereas during E_1f_2 source rocks deposition,anoxic and relatively low salinity condition is prevailed.The Paleogene crude oil contains relatively high saturates content,with small UCM peak,and has entered into the mature stage.Oil-source correlation results indicate that the Dainan crude oil(oil sand extraction)is related to the E_1f_4source rocks,whereas E_1f_3 crude oil may be derived from E_1f_2 source rocks.
Researches on the hydrocarbon potential of the source rock in the Paleogene Funing Formation,and origin of the Paleogene crude oil in the southern depression of the South Yellow Sea Basin(SYSB)are relatively weak.Based on the systematically organic geochemical analyses(TOC,Rock-Eval,GC-MS of saturates and aromatics,stable carbon isotope)of the Paleogene core,cuttings,oil sand and crude oil samples,combined with vitrinite reflectance determination,the geochemical characteristics of source rocks and crude oil are revealed,and oil-source correlation is obtained.The results indicate that the Paleogene source rocks in the southern depression mainly deposited in the fourth (E_1f_4) and second memebers (E_1f_2) of Funing Formation,with moderate-good organic matter(OM)abundance,type Ⅱ_2-Ⅲ kerogen and within low mature-mature stage.Mixed OM sources,dominated by terrestrial OM are observed in E_1f_4 and E_1f_2 source rocks,biomarker ratios indicate that E_1f_4source rocks were deposited in dysoxic,relatively high salinity condition.Whereas during E_1f_2 source rocks deposition,anoxic and relatively low salinity condition is prevailed.The Paleogene crude oil contains relatively high saturates content,with small UCM peak,and has entered into the mature stage.Oil-source correlation results indicate that the Dainan crude oil(oil sand extraction)is related to the E_1f_4source rocks,whereas E_1f_3 crude oil may be derived from E_1f_2 source rocks.
引文
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Cranwell,P.A.,1977.Organic Geochemistry of Cam Loch(Sutherland)Sediments.Chemical Geology,20:205-221.https://doi.org/10.1016/0009-2541(77)90044-4
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Fang,C.H.,Zhang,Z.H.,Wang,Y.F.,et al.,2008.Geochemical Characteristics of the Lower Tertiary Source Rock in Qintong Sag,Subei Basin.Journal of Xi’an Shiyou University(Natural Science Edition),23(6):1-5(in Chinese with English abstract).
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Luo,W.F.,Yu,W.D.,Ma,X.D.,et al.,2018.Exploration Achievement of Lithological Oil Reservoirs in the South of Haian Depression,the Subei Basin and Its Enlightenment.China Petroleum Exploration,23(3):56-63(in Chinese with English abstract).
Nott,C.J.,Xie,S.C.,Avsejs,L.A.,et al.,2000.n-Alkane Distributions in Ombrotrophic Mires as Indicators of Vegetation Change Related to Climatic Variation.Organic Geochemistry,31(2-3):231-235.https://doi.org/10.1016/s0146-6380(99)00153-9
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Peters,K.E.,Moldowan,J.M.,1993.The Biomarker Guide:Interpreting Molecular Fossils in Petroleum and Ancient Sediments.Prentice Hall,New Jersey.
Sachsenhofer,R.F.,Popov,S.V.,Akhmetiev,M.A.,et al.,2017.The Type Section of the Maikop Group(Oligocene-Lower Miocene)at the Belaya River(North Caucasus):Depositional Environment and Hydrocarbon Potential.AAPG Bulletin,101(3):289-319.https://doi.org/10.1306/08051616027
Song,Y.,Bechtel,A.,Sachsenhofer,R.F.,et al.,2017.Depositional Environment of the Lower Cretaceous Muling Formation of the Laoheishan Basin(NE China):Implications from Geochemical and Petrological Analyses.Organic Geochemistry,104:19-34.https://doi.org/10.1016/j.orggeochem.2016.11.008
Song,Y.,Liu,Z.J.,Meng,Q.T.,et al.,2016.Multiple Controlling Factors of the Enrichment of Organic Matter in the Upper Cretaceous Oil Shale Sequences of the Songliao Basin,NE China:Implications from Geochemical Analyses.Oil Shale,33(2):142-166.https://doi.org/10.3176/oil.2016.2.04
Tissot,B.T.,Welte,D.H.,1984.Petroleum Formation and Occurrences.Springer-Verlag,Berlin.
van Kaam-Peters,H.M.E.,Schouten,S.,de Leeuw,J.W.,et al.,1997.A Molecular and Carbon Isotope Biogeochemical Study of Biomarkers and Kerogen Pyrolysates of the Kimmeridge Clay Facies:Palaeoenvironmental Implications.Organic Geochemistry,27(7-8):399-422.https://doi.org/10.1016/s0146-6380(97)00084-3
Wu,X.Q.,Chen,Y.B.,Liu,Q.Y.,et al.,2019.Molecular Geochemical Characteristics of Source Rocks in the 5th Member of the Upper Triassic Xujiahe Formation in the Xinchang Gas Field,the Western Sichuan Depression.Earth Science,44(3):859-871(in Chinese with English abstract).https://doi.org/10.3799/dqkx.2018.236
Wu,Z.Q.,Lu,K.,Yan,G.J.,et al.,2008.Geophysical Exploration Methods of Early Cenozoic Oil Gas in South Yellow Sea.Marine Geology Letters,24(8):1-7(in Chinese with English abstract).
Xiao,G.L.,2002.Reassessment of Petroleum Geologic Features and Potential Reserves in the South Yellow Sea Basin.Marine Geology&Quaternary Geology,22(2):81-87(in Chinese with English abstract).
Xu,X.H.,Zhou,X.J.,Peng,J.N.,2014.Exploration Targets in Southern Yellow Sea through Analysis of TectonoDepositional Evolution and Hydrocarbon Accumulation of Marine Basin in Yangtze Area.Petroleum Geology&Experiment,36(5):523-531,545(in Chinese with English abstract).
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Zhang,M.M.,Li,Z.,2018.Thermal Maturity of the Permian Lucaogou Formation Organic-Rich Shale at the Northern Foot of Bogda Mountains,Junggar Basin(NW China):Effective Assessments from Organic Geochemistry.Fuel,211:278-290.https://doi.org/10.1016/j.fuel.2017.09.069
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Cai,J.,Cui,M.,Liu,Z.F.,et al.,2014a.Sedimentary Facies and Analyze on Reservoir-Seal Assemblage of the Dainan Formation of Paleogene in Nan 5 Sag,Nanhuanghai Basin.Journal of East China Institute of Technology(Natural Science Edition),37(4):395-402(in Chinese with English abstract).
Cai,J.,Zhao,Z.G.,Zhang,X.L.,et al.,2014b.On Sedimentary Facies in Funing Formation of Northern Sag in North Depression in South Yellow Sea Basin.Journal of Geology,38(4):530-535(in Chinese with English abstract).
Cai,J.,Wu,K.Q.,Wang,P.,et al.,2016.Sedimentary Facies of the Paleogene Funing Formation in the South Depression of the South Yellow Sea Basin.Journal of Geology,40(1):125-134(in Chinese with English abstract).
Coplen,T.B.,2011.Guidelines and Recommended Terms for Expression of Stable-Isotope-Ratio and Gas-Ratio Measurement Results.Rapid Communications in Mass Spectrometry,25(17):2538-2560.https://doi.org/10.1002/rcm.5129
Cranwell,P.A.,1977.Organic Geochemistry of Cam Loch(Sutherland)Sediments.Chemical Geology,20:205-221.https://doi.org/10.1016/0009-2541(77)90044-4
Didyk,B.M.,Simoneit,B.R.T.,Brassell,S.C.,et al.,1978.Organic Geochemical Indicators of Palaeoenvironmental Conditions of Sedimentation.Nature,272(5650):216-222.https://doi.org/10.1038/272216a0
Eglinton,G.,Hamilton,R.J.,1967.Leaf Epicuticular Waxes.Science,156(3780):1322-1335.https://doi.org/10.1126/science.156.3780.1322
Fang,C.H.,Wang,Y.F.,Zheng,D.W.,et al.,2007.Maceral and Petrology of Lower Tertiary Source Rock in Qintong Sag,Subei Basin.Lithologic Reservoirs,19(4):87-90,130(in Chinese with English abstract).
Fang,C.H.,Zhang,Z.H.,Wang,Y.F.,et al.,2008.Geochemical Characteristics of the Lower Tertiary Source Rock in Qintong Sag,Subei Basin.Journal of Xi’an Shiyou University(Natural Science Edition),23(6):1-5(in Chinese with English abstract).
Ficken,K.J.,Li,B.,Swain,D.L.,et al.,2000.An n-Alkane Proxy for the Sedimentary Input of Submerged/Floating Freshwater Aquatic Macrophytes.Organic Geochemistry,31(7-8):745-749.https://doi.org/10.1016/s0146-6380(00)00081-4
Gross,D.,Sachsenhofer,R.F.,Bechtel,A.,et al.,2015.Organic Geochemistry of Mississippian Shales(Bowland Shale Formation)in Central Britain:Implications for Depositional Environment,Source Rock and Gas Shale Potential.Marine and Petroleum Geology,59:1-21.https://doi.org/10.1016/j.marpetgeo.2014.07.022
Hou,Q.J.,Jin,Q.,Niu,C.M.,et al.,2018.Distribution Characteristics and Main Controlling Factors of Main Hydrocarbon Source Rocks in Liaodong Bay Area.Earth Science,43(6):2160-2171(in Chinese with English abstract).https://doi.org/10.3799/dqkx.2018.586
Lai,W.Z.,2002.Sedimentary Basins and Petroleum of the Yellow Sea.Marine Geology Letters,18(11):13-16(in Chinese with English abstract).
Langford,F.F.,Blanc-Valleron,M.M.,1990.Interpreting Rock-Eval Pyrolysis Data Using Graphs of Pyrolizable Hydrocarbonsvs.Total Organic Carbon.AAPG Bulletin,74(6):799-804.https://doi.org/10.1306/0c9b238f-1710-11d7-8645000102c1865d
Li,S.F.,Hu,S.Z.,He,S.,et al.,2010.Oil-Source Correlation for Biodegraded Oils in the North Slope of the Biyang Depression.Acta Petrolei Sinica,31(6):946-951(in Chinese with English abstract).
Liang,D.G.,Chen,J.P.,2005.Oil-Source Correlations for High and over Matured Marine Source Rocks in South China.Petroleum Exploration and Development,32(2):8-14(in Chinese with English abstract).
Liao,Y.S.,1992.The New Development in Petroleum Stable Isotope Geochemistry.Journal of Chinese Mass Spectrometry Society,13(4):22-33(in Chinese with English abstract).
Liu,B.,Bechtel,A.,Sachsenhofer,R.F.,et al.,2017.Depositional Environment of Oil Shale within the Second Member of Permian Lucaogou Formation in the Santanghu Basin,Northwest China.International Journal of Coal Geology,175:10-25.https://doi.org/10.1016/j.coal.2017.03.011
Luo,W.F.,Yu,W.D.,Ma,X.D.,et al.,2018.Exploration Achievement of Lithological Oil Reservoirs in the South of Haian Depression,the Subei Basin and Its Enlightenment.China Petroleum Exploration,23(3):56-63(in Chinese with English abstract).
Nott,C.J.,Xie,S.C.,Avsejs,L.A.,et al.,2000.n-Alkane Distributions in Ombrotrophic Mires as Indicators of Vegetation Change Related to Climatic Variation.Organic Geochemistry,31(2-3):231-235.https://doi.org/10.1016/s0146-6380(99)00153-9
Peters,K.E.,1986.Guidelines for Evaluating Petroleum Source Rock Using Programmed Pyrolysis.AAPG Bulletin,70:318-329.https://doi.org/10.1306/94885688-1704-11d7-8645000102c1865d
Peters,K.E.,Moldowan,J.M.,1993.The Biomarker Guide:Interpreting Molecular Fossils in Petroleum and Ancient Sediments.Prentice Hall,New Jersey.
Sachsenhofer,R.F.,Popov,S.V.,Akhmetiev,M.A.,et al.,2017.The Type Section of the Maikop Group(Oligocene-Lower Miocene)at the Belaya River(North Caucasus):Depositional Environment and Hydrocarbon Potential.AAPG Bulletin,101(3):289-319.https://doi.org/10.1306/08051616027
Song,Y.,Bechtel,A.,Sachsenhofer,R.F.,et al.,2017.Depositional Environment of the Lower Cretaceous Muling Formation of the Laoheishan Basin(NE China):Implications from Geochemical and Petrological Analyses.Organic Geochemistry,104:19-34.https://doi.org/10.1016/j.orggeochem.2016.11.008
Song,Y.,Liu,Z.J.,Meng,Q.T.,et al.,2016.Multiple Controlling Factors of the Enrichment of Organic Matter in the Upper Cretaceous Oil Shale Sequences of the Songliao Basin,NE China:Implications from Geochemical Analyses.Oil Shale,33(2):142-166.https://doi.org/10.3176/oil.2016.2.04
Tissot,B.T.,Welte,D.H.,1984.Petroleum Formation and Occurrences.Springer-Verlag,Berlin.
van Kaam-Peters,H.M.E.,Schouten,S.,de Leeuw,J.W.,et al.,1997.A Molecular and Carbon Isotope Biogeochemical Study of Biomarkers and Kerogen Pyrolysates of the Kimmeridge Clay Facies:Palaeoenvironmental Implications.Organic Geochemistry,27(7-8):399-422.https://doi.org/10.1016/s0146-6380(97)00084-3
Wu,X.Q.,Chen,Y.B.,Liu,Q.Y.,et al.,2019.Molecular Geochemical Characteristics of Source Rocks in the 5th Member of the Upper Triassic Xujiahe Formation in the Xinchang Gas Field,the Western Sichuan Depression.Earth Science,44(3):859-871(in Chinese with English abstract).https://doi.org/10.3799/dqkx.2018.236
Wu,Z.Q.,Lu,K.,Yan,G.J.,et al.,2008.Geophysical Exploration Methods of Early Cenozoic Oil Gas in South Yellow Sea.Marine Geology Letters,24(8):1-7(in Chinese with English abstract).
Xiao,G.L.,2002.Reassessment of Petroleum Geologic Features and Potential Reserves in the South Yellow Sea Basin.Marine Geology&Quaternary Geology,22(2):81-87(in Chinese with English abstract).
Xu,X.H.,Zhou,X.J.,Peng,J.N.,2014.Exploration Targets in Southern Yellow Sea through Analysis of TectonoDepositional Evolution and Hydrocarbon Accumulation of Marine Basin in Yangtze Area.Petroleum Geology&Experiment,36(5):523-531,545(in Chinese with English abstract).
Yao,Y.J.,Feng,Z.Q.,Hao,T.Y.,et al.,2008.A New Understanding of the Structural Layers in the South Yellow Sea Basin and Their Hydrocarbon-Bearing Characteristics.Earth Science Frontiers,15(6):232-240(in Chinese with English abstract).
Yao,Y.J.,Xia,B.,Feng,Z.Q.,et al.,2005.Tectonic Evolution of the South Yellow Sea since the Paleozoic.Petroleum Geology&Experiment,27(2):124-128(in Chinese with English abstract).
Zhang,M.M.,Li,Z.,2018.Thermal Maturity of the Permian Lucaogou Formation Organic-Rich Shale at the Northern Foot of Bogda Mountains,Junggar Basin(NW China):Effective Assessments from Organic Geochemistry.Fuel,211:278-290.https://doi.org/10.1016/j.fuel.2017.09.069
Zheng,Q.G.,Cai,L.G.,Ding,W.L.,et al.,2005.Development and Evolution of Basins in Yellow Sea.Oil&Gas Geology,26(5):647-654(in Chinese with English abstract).
蔡佳,崔敏,刘志峰,等,2014a.南黄海盆地南五凹古近系戴南组沉积相及储盖组合分析.东华理工大学学报(自然科学版),37(4):395-402.
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