工业源挥发性有机物治理功能材料研究进展
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摘要
挥发性有机物(volatile organic compounds,VOCs)是大气中一类重要的污染物质,即使在低浓度下也会对人类的健康造成威胁。对VOCs的治理刻不容缓,而VOCs治理关键功能材料性能的优劣是整个VOCs治理技术的核心。文章总结了近年来用于吸附法、光催化法以及催化燃烧法治理VOCs的功能材料的最新科研成果,希望以此能够为将来VOCs治理材料的设计与研发提供一定的参考。
Volatile organic compounds(VOCs) is one class of important atmospheric pollutants, which threat to human health even at a low concentration. The control of VOCs emission is a task which brooks no delay. The quality of functional materials is a key part of the whole VOCs emission control process. In this paper, we summarize the latest academic research progress in functional materials applied in adsorption, photocatalysis and catalytic combustion, and provide some guidance for the design and research of VOCs control materials for the future.
Volatile organic compounds(VOCs) is one class of important atmospheric pollutants, which threat to human health even at a low concentration. The control of VOCs emission is a task which brooks no delay. The quality of functional materials is a key part of the whole VOCs emission control process. In this paper, we summarize the latest academic research progress in functional materials applied in adsorption, photocatalysis and catalytic combustion, and provide some guidance for the design and research of VOCs control materials for the future.
引文
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[5]ZHAO S,HU F,LI J.Hierarchical core-shell Al2O3@Pd-CoAlOmicrospheres for low-temperature toluene combustion[J].ACSCatalysis,2016,6(6):3433-3441.
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[9]?ULIGOJ A,?TANGAR U L,RISTI?A,et al.TiO2-SiO2 films from organic-free colloidal TiO2 anatase nanoparticles as photocatalyst for removal of volatile organic compounds from indoor air[J].Applied Catalysis B:Environmental,2016,184:119-131.
[10]STUCCHI M,BIANCHI C L,PIROLA C,et al.Copper NPs decorated titania:A novel synthesis by high energy US with a study of the photocatalytic activity under visible light[J].Ultrasonics Sonochemistry,2016,31:295-301.
[11]LI M,WU S,SHIH Y.Characterization of volatile organic compound adsorption on multiwall carbon nanotubes under different levels of relative humidity using linear solvation energy relationship[J].Journal of Hazardous Materials,2016,315:35-41.
[12]QIAN X,YUE D,TIAN Z,et al.Carbon quantum dots decorated Bi2WO6 nanocomposite with enhanced photocatalytic oxidation activity for VOCs[J].Applied Catalysis B:Environmental,2016,193:16-21.
[13]SOLSONA B,GARC A T,SANCHIS R,et al.Total oxidation of VOCs on mesoporous iron oxide catalysts:Soft chemistry route versus hard template method[J].Chemical Engineering Journal,2016,290:273-281.
[14]LIU P,HE H,WEI G,et al.Effect of Mn substitution on the promoted formaldehyde oxidation over spinel ferrite:catalyst characterization,performance and reaction mechanism[J].Applied Catalysis B:Environmental,2016,182:476-484.
[15]HUANG H,ZHANG C,WANG L,et al.Promotional effect of HZSM-5 on the catalytic oxidation of toluene over MnOx/HZSM-5catalysts[J].Catal Sci Technol,2016,6(12):4260-4270.
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[19]LILLO-RóDENAS M,CAZORLA-AMORóS D,LINARES-SOLANO A.Behaviour of activated carbons with different pore size distributions and surface oxygen groups for benzene and toluene adsorption at low concentrations[J].Carbon,2005,43(8):1758-1767.
[20]宋剑飞.活性炭吸附VOCs及其构效关系研究[D].长沙:中南大学,2014.
[21]SILVESTRE-ALBERO A,SILVESTRE-ALBERO J,SEP LVEDA-ESCRIBANO A,et al.Ethanol removal using activated carbon:effect of porous structure and surface chemistry[J].Microporous and Mesoporous Materials,2009,120(1):62-68.
[22]GAUR V,ASTHANA R,VERMA N.Removal of SO2 by activated carbon fibers in the presence of O2 and H2O[J].Carbon,2006,44(1):46-60.
[23]MOHAMMED J,NASRI N S,AHMAD ZAINI M A,et al.Adsorption of benzene and toluene onto KOH activated coconut shell based carbon treated with NH3[J].International Biodeterioration&Biodegradation,2015,102:245-255.
[24]ZHU M,TONG Z,ZHAO Z,et al.A microporous graphitized biocarbon with high adsorption capacity toward benzene volatile organic compounds(VOCs)from humid air at ultralow pressures[J].Industrial&Engineering Chemistry Research,2016,55(13):3765-3774.
[25]QIAN Q,GONG C,ZHANG Z,et al.Removal of VOCs by activated carbon microspheres derived from polymer:a comparative study[J].Adsorption,2015,21(4):333-341.
[26]WANG G,DOU B,ZHANG Z,et al.Adsorption of benzene,cyclohexane and hexane on ordered mesoporous carbon[J].Journal of Environmental Sciences,2015,30:65-73.
[27]LáSZLóK,BóTA A,NAGY L G,et al.Porous carbon from polymer waste materials[J].Colloids and Surfaces A:Physicochemical and Engineering Aspects,1999,151(1/2):311-320.
[28]KARTEL M T,SYCH N V,TSYBA M M,et al.Preparation of porous carbons by chemical activation of polyethyleneterephthalate[J].Carbon,2006,44(5):1019-1022.
[29]BRATEK W,?WI?TKOWSKI A,PAKU?A M,et al.Characteristics of activated carbon prepared from waste PET by carbon dioxide activation[J].Journal of Analytical and Applied Pyrolysis,2013,100:192-198.
[30]CHOMA J,MARSZEWSKI M,OSUCHOWSKI L,et al.Adsorption properties of activated carbons prepared from waste CDs and DVDs[J].ACS Sustainable Chemistry&Engineering,2015,3(4):733-742.
[31]CHENG W D,CAI C Z.Prediction of Henry constants and adsorption mechanism of volatile organic compounds on multi-walled carbon nanotubes by using support vector regression[J].Chinese Physics Letters,2016,33(4):048201.
[32]PRESSER V,HEON M,GOGOTSI Y.Carbide-derived carbonsfrom porous networks to nanotubes and graphene[J].Advanced Functional Materials,2011,21(5):810-833.
[33]贾进,杨晓阳,闫艳,等.碳化物衍生碳的制备及其在气体存储与超级电容器领域的应用研究进展[J].化工进展,2014,10:2681-2686.
[34]GOGOTSI Y,DASH R K,YUSHIN G,et al.Tailoring of nanoscale porosity in carbide-derived carbons for hydrogen storage[J].Journal of the American Chemical Society,2005,127(46):16006-16007.
[35]ZHU H L,BAI Y J,QI Y X,et al.Large-scale synthesis of hollow highly-graphitic carbon nanospheres by the reaction of AlCl3·6H2Owith CaC2[J].Carbon,2012,50(5):1871-1878.
[36]CHMIOLA J,YUSHIN G,GOGOTSI Y,et al.Anomalous increase in carbon capacitance at pore sizes less than 1 nanometer[J].Science,2006,313(5794):1760-1763.
[37]MANGARELLA M C,EWBANK J L,DUTZER M R,et al.Synthesis of embedded iron nanoparticles in Fe3C-derived carbons[J].Carbon,2014,79:74-84.
[38]YUSHIN G,DASH R,JAGIELLO J,et al.Carbide‐derived carbons:effect of pore size on hydrogen uptake and heat of adsorption[J].Advanced Functional Materials,2006,16(17):2288-2293.
[39]SEVILLA M,FOULSTON R,MOKAYA R.Superactivated carbidederived carbons with high hydrogen storage capacity[J].Energy&Environmental Science,2010,3(2):223-227.
[40]YEON S-H,OSSWALD S,GOGOTSI Y,et al.Enhanced methane storage of chemically and physically activated carbide-derived carbon[J].Journal of Power Sources,2009,191(2):560-567.
[41]ZHANG Y,GUO S,QI Y,et al.Hydrogen storage behaviour of nanocrystalline and amorphous Mg20Ni10-xCox(x=0~4)alloys by meltspinning[J].Rare Metal Materials and Engineering,2012,41(11):1881-1886.
[42]BHATIA S K,NGUYEN T X.Potential of silicon carbide-derived carbon for carbon capture[J].Industrial&Engineering Chemistry Research,2011,50(17):10380-10383.
[43]HUANG H,SONG Z,WEI N,et al.Untrafast viscous water flow through nanostrand-channelled graphene oxide membranes[J].Nature Communication,2013,4:2979.doi:10.1038/ncomms3979.
[44]HUNG W-S,TSOU C-H,DE GUZMAN M,et al.Cross-linking with diamine monomers to prepare composite graphene oxide-framework membranes with varying d-spacing[J].Chemistry of Materials,2014,26(9):2983-2990.
[45]CHEN L,SHI G,SHEN J,et al.Ion sieving in graphene oxide membranes via cationic control of interlayer spacing[J].Nature,2017,550(7676):415-418.
[46]SHI G,LIU J,WANG C,et al.Ion enrichment on the hydrophobic carbon-based surface in aqueous salt solutions due to cation-pi interactions[J].Scientific Reports,2013,3:3436.doi:10.1038/srep03436.
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