天津地区霾天气特征研究
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摘要
基于2014～2017年天津地区PM_(2.5)质量浓度,能见度和相对湿度监测数据开展霾天气特征研究.结果表明:天津中度以上霾过程分为五类:高压后部型,北部弱高压型,低压槽型,均压场型和锋前低压型.在现行标准下,中度霾一般对应重度污染天气,重度霾对应重度到严重污染天气;五级重度污染天气一般有中-重度霾发生,六级严重污染天气有重度霾天气发生.2013年"大气污染防治行动计划"开展以后,天津PM_(2.5)质量浓度和霾日均显著减少,2017年相比2013年霾日减少了55%,中度及其以上霾日由2013年的41d下降到2017年的20d,下降幅度超过50%.基于实况监测的PM_(2.5)质量浓度,能见度和相对湿度,可以较好的构建区域能见度计算方程.统计数据显示,其估算的能见度和实况值相关系数为0.94,相对误差为18.6%,非霾日辨识准确率为85%,霾日辨识准确率为95.6%,轻微霾辨识准确率为83%,轻度霾辨识准确率为78%,中度霾辨识准确率为93%,重度及以上霾辨识准确率为94%,对于判断霾等级,有较强的适用性.将该方程与空气质量模式结合开展霾等级预报,2015～2017年24h预报产品检验显示:能见度预报值与实况值相关系数为0.75,预报均值13.9km,实况均值14.1km,相对误差为29.6%,FAC2(预报值在实况值两倍范围内百分比)为98.1%,霾日预报准确率81.4%,霾日漏报率18.6%,霾日空报率20.6%,如果容错1级,轻微霾日预报准确率为96%,轻度霾日预报准确率为85%,中度及以上霾日预报准确率为69%,可有效支撑天津霾等级预报的开展.
A research was carried out on characteristics of the haze weather in Tianjin based on the monitoring data of PM_(2.5) mass concentration, visibility and relative humidity in the area from 2014 to 2017, The findings showed that there are five types of haze processes above moderate degree in Tianjin: that in the rear of high pressure, that caused by weak high pressure from north, that caused by low pressure trough, that caused by uniform pressure field and that caused by low pressure before front. As per the current standards, moderate haze generally corresponds to severely polluted weather; severe haze corresponds to severely to untra-severely polluted weather. Moderate to severe haze usually occurs in Level V severely polluted weather, and severe haze occurs in Level VI ultra-severely polluted weather. After "Air Pollution Prevention Action Plan" was implemented in 2013, PM_(2.5) mass concentration and haze days were significantly reduced, by 2017, the number of haze days had decreased by 55% compared with 2013, moderate and above haze days decreased by 50% from 41 d in 2013 to 20 d in 2017. Based on the monitoring data of PM_(2.5) mass concentration, visibility and relative humidity, the calculation equation of regional visibility can be well constructed. Statistics showed that the correlation coefficient between visibility and real value in the estimation is 0.94, with the relative error 18.6%, identification accuracy rate of the non-haze day is 85%, that of the haze days 95.6%, that of the ultra-slight haze days 83%, that of the slight haze days 78%, that of moderate haze days 93% and that of severe and above haze days 94%, which is greatly applicable for judgement of haze level. This equation was combined with the air quality model to predict the haze level. Inspection of the forecasting product showed: the correlation coefficient between the forecast values and real values of visibility is 0.75, with average forecast value 13.9km and the average real value 14.1km, and the relative error rate 29.6%, the FAC2(the ratio of the forecast value to two times the real value) is 98.1%, the forecast accuracy rate, forecast missing rate and false rate of the haze days are 81.4%, 18.6% and 20.6%, respectively. Let the tolerance be of Level I, the forecast accuracy rates of ultra-slight haze days, the slight haze days and the moderate and above haze days are 96%, 85% and 69%, respectively, which may effectively support the haze level forecast in Tianjin.
A research was carried out on characteristics of the haze weather in Tianjin based on the monitoring data of PM_(2.5) mass concentration, visibility and relative humidity in the area from 2014 to 2017, The findings showed that there are five types of haze processes above moderate degree in Tianjin: that in the rear of high pressure, that caused by weak high pressure from north, that caused by low pressure trough, that caused by uniform pressure field and that caused by low pressure before front. As per the current standards, moderate haze generally corresponds to severely polluted weather; severe haze corresponds to severely to untra-severely polluted weather. Moderate to severe haze usually occurs in Level V severely polluted weather, and severe haze occurs in Level VI ultra-severely polluted weather. After "Air Pollution Prevention Action Plan" was implemented in 2013, PM_(2.5) mass concentration and haze days were significantly reduced, by 2017, the number of haze days had decreased by 55% compared with 2013, moderate and above haze days decreased by 50% from 41 d in 2013 to 20 d in 2017. Based on the monitoring data of PM_(2.5) mass concentration, visibility and relative humidity, the calculation equation of regional visibility can be well constructed. Statistics showed that the correlation coefficient between visibility and real value in the estimation is 0.94, with the relative error 18.6%, identification accuracy rate of the non-haze day is 85%, that of the haze days 95.6%, that of the ultra-slight haze days 83%, that of the slight haze days 78%, that of moderate haze days 93% and that of severe and above haze days 94%, which is greatly applicable for judgement of haze level. This equation was combined with the air quality model to predict the haze level. Inspection of the forecasting product showed: the correlation coefficient between the forecast values and real values of visibility is 0.75, with average forecast value 13.9km and the average real value 14.1km, and the relative error rate 29.6%, the FAC2(the ratio of the forecast value to two times the real value) is 98.1%, the forecast accuracy rate, forecast missing rate and false rate of the haze days are 81.4%, 18.6% and 20.6%, respectively. Let the tolerance be of Level I, the forecast accuracy rates of ultra-slight haze days, the slight haze days and the moderate and above haze days are 96%, 85% and 69%, respectively, which may effectively support the haze level forecast in Tianjin.
引文
[1]吴兑.关于霾与雾的区别和灰霾天气预警的讨论[J].气象,2005,31(4):3-7.Wu D.A Discussion on Difference between Haze and Fog and Warning of Ash Haze Weather[J].Meteorological monthly.2005,31(4):3-7.
[2]吴兑,毕雪岩,邓雪娇,等.珠江三角洲大气灰霾导致能见度下降问题研究[J].气象学报,2006,64(4):510-517.Wu D,Bi X,Deng X J,et al.Effect of atmospheric haze on the deterioration of visibility over the pear river detla[J].Acta Meteorological sinica,2006,64(4):510-517.
[3]陈欢欢,吴兑,谭浩波,等.珠江三角洲2001~2008年灰霾天气过程特征分析[J].热带气象学报,2010,26(2):147-155.Chen H H,Wu D,Tan H B,et al.Study on the character of haze weather process from the year 2001 to 2008 over the pearl river delta[J].Journal of tropical meteorology,2010,26(2):147-155.
[4]吴蒙,范绍佳,吴兑,等.广州地区灰霾与清洁天气变化特征及影响因素分析[J].中国环境科学,2012,32(8):1409-1415.Wu M,Fan S J,Wu D,et al.Characteristics and influence factors study of haze and cleaning weather over Guangzhou Area[J].China Environmental Science.2012,32(8):1409-1415.
[5]刘琼,耿福海,陈勇航,等.上海不同强度干霾期间气溶胶垂直分布特征[J].中国环境科学,2012,32(2):207-213.Liu Q,Geng F H,Chen Y H,et al.Vertical distribution of aerosols during different intense dry haze periods around Shanghai[J].China Environmental Science,2012,32(2):207-213.
[6]王苑,耿福海,陈勇航,等.基于微脉冲激光雷达的上海浦东地区不同强度霾研究[J].中国环境科学,2013,33(1):21-29.Wang Y,Geng F H,Chen Y H,et al.Study of haze with different intensity categories at Pudong District in Shanghai based on micropulse lidar[J].China Environmental Science,2013,33(1):21-29.
[7]王静,牛生杰,许丹,等.南京一次典型雾霾天气气溶胶光学特性[J].中国环境科学,2013,33(2):201-208.Wang J,Niu S J,Xu D,et al.Aerosol optical properties during the typical haze/fog event in Nanjing[J].China Environmental Science.2013,33(2):201-208.
[8]朱佳雷,王体健,邢莉,等.江苏省一次重霾污染天气的特征和机理分析[J].中国环境科学,2011,31(12):1943-1950.Zhu J L,Wang T J,Xing L,et al.Analysis on the characteristics and mechanism of a heavy haze episode in Jiangsu Province[J].China Environmental Science.2011,31(12):1943-1950.
[9]吴兑,廖碧婷,吴蒙,等.环首都圈霾和雾的长期变化特征与典型个例的近地层输送条件[J].环境科学学报,2014,34(1):1-11.Wu D,Liao B,Wu M,et al.The long-term trend of haze and fog days and the surface layer transport conditions under haze weather in North China[J].Acta Scientiae Circumstantiae,2014,34(1):1-11.
[10]薛亦峰,周震,聂滕,等.2015年12月北京市空气重污染过程分析及污染源排放变化[J].环境科学,2016,37(5):1593-1601.Xue Y F,Zhou Z,Nie T,et al.Exploring the Severe Haze in Beijing During December,2015:Pollution Process and Emissions Variation[J].Environmental Science.2016,37(5):1593-1601.
[11]穆穆,张人禾.应对灰霾天气:气象科学与技术大有可为[J].中国科学:地球科学,2014,44(1):1-2.Mu M,Zhang R H.Dealing with Haze Weather:Great Prospects for Meteorological Science and Technology[J].Chinese Science:Geosciences,2014,44(1):1-2.
[12]董春卿,郑有飞,武永利,等.边界层方案对山西冬季一次静稳天气PM_(2.5)浓度模拟的影响[J].中国环境科学,2016,36(6):1669-1680.Dong C Q,Zheng Y F,Wu Y L,et al.The effects of different planetary boundary layer schemes on PM_(2.5) concentration simulations in winter stable weather of Shanxi[J].China Environmental Science.2016,36(6):1669-1680.
[13]李令军,王占山,张大伟,等.2013~2014年北京大气重污染特征研究[J].中国环境科学,2016,36(1):27-35.Ling J,Wang Z S,Zhang D W,et al.Analysis of heavy air pollution episodes in Beijing during 2013~2014[J].China Environmental Science,2016,36(1):27-35.
[14]刘兴瑞,马嫣,崔芬萍,等.南京北郊一次重污染事件期间PM_(2.5)理化特性及其对大气消光的影响[J].环境化学,2016,35(6):1164-1171.LiuX R,Ma Y,Cui F P,et al.Physicochemical characteristics of PM_(2.5)and impacts on light extinction during the heavy pollution period at North Suburban Nanjing[J].Environmental Chemistry,2016,35(6):1164-1171.
[15]蔡子颖,韩素芹,张敏,等.天津地区污染天气分析中垂直扩散指标构建及运用[J].环境科学,2018,39(6):2548-2556.Cai Z Y,Han S Q,Zhang M,et al.Construction and Application of Vertical Diffusion Index for Analyzing Weather During Pollution Events in Tianjin[J].Environmental Science,2018,39(6):2548-2556.
[16]Tang G,Zhu X,Hu B,et al.Impact of emission controls on air quality in Beijing during APEC 2014:lidar ceilometer observations[J].Atmospheric Chemistry&Physics,2015,15(21):12667-12680.
[17]Han S,Hao T,Zhang Y,et al.Vertical observation and analysis on rapid formation and evolutionary mechanisms of a prolonged haze episode over central-eastern China.Science of total environment[J].Science of the total environment,2018,2018(616):135-146.
[18]李梦,唐贵谦,黄俊,等.京津冀冬季大气混合层高度与大气污染的关系[J].环境科学,2015,36(6):1935-1943.Li M,Tang G Q,Huang J,et al.Characteristics of Winter Atmospheric Mixing Layer Height in Beijing-Tianjin-Hebei Region and Their Relationship with the Atmospheric Pollution[J].Environmental Science,2015,36(6):1935-1943.
[19]蔡子颖,韩素芹,汪靖,等.基于天气背景天津地区重污染天气特征分析[J].环境科学学报,2017,37(10):3906-3917.Cai Z Y,Han S Q,Wang J,et al.Analysis of synoptic characteristics of heavy pollution in Tianjin based on weather background[J].Acta Scientiae Circumstantiae,2017,37(10):3906-3917.
[20]周鑫,丁菊丽,田伟,等.能见度参数化方案概述[J].气象研究与应用,2009,30(3):22-25.Zhou X,Ding J,Tian W,et al.Introduction of Visibility Parameterization Scheme[J].Journal of meteorological research and application.2009,30(3):22-25.
[21]边海,张裕芬,韩素芹,等.天津市大气能见度与颗粒物污染的关系[J].中国环境科学,2012,32(3):406-410.Bian H,Han S Q,Zhang Y F,et al.Relationship between atmospheric visibility and particulate matter pollution in Tianjin[J].China Environmental Science.2012,32(3):406-410.
[22]陈义珍,赵丹,柴发合,等.广州市与北京市大气能见度与颗粒物质量浓度的关系[J].中国环境科学,2010,30(7):967-971.Chen Y Z,Zhao D,Chai F H,et al.Correlation between the atmospheric visibility and aerosol fine particle concentrations in Guangzhou and Beijing[J].China Environmental Science.2010,30(7):967-971.
[23]姚青,蔡子颖,韩素芹,等.2009年秋冬季天津低能见度天气下气溶胶污染特征[J].气象,2012,38(9):1096-1102.Yao Q,Cai Z Y,Han S Q,et al.Study on Pollution Characteristics of aerosols during low visibility weather at Tianjin City in Autumn and Winter 2009[J].Meteorological monthly.2012,38(9):1096-1102.
[24]姚青,韩素芹,蔡子颖,等.天津城区春季大气气溶胶消光特性研究[J].中国环境科学,2012,32(5):795-802.Yao Q,Han S Q,Cai Z Y,et al.Study on characteristic of aerosol extinction at Tianjin City in the spring[J].China Environmental Science,2012,32(5):795-802.
[25]刘西川,高太长,刘磊,等.降水现象对大气消光系数和能见度的影响[J].应用气象学报,2010,21(4):433-441.Liu X C,Gao T C,Liu L,et al.Influences of Precipitation on atmospheric Extinction coefficient and Visibility[J].Journal of applied metrological science,2010,21(4):433-441.
[26]刘宁微,马雁军,王扬锋.辽宁中部城市群夏季大气能见度的观测研究[J].气象学报,2012,70(4):814-820.Liu N W,Ma Y J,Wang Y F,et al.Observational study of atmospheric visibility in summer in the area of multicities in central Liaoning Province[J].Acta Meteorological Sinica,2012,70(4):814-820.
[27]饶晓琴,马学款,黄威.2014年12月大气环流和天气分析[J].气象,2015,41(3):380-387.Wang J K,Gui H L,Ma X K,et al.Analysis of the December 2017Atmospheric circulation and weather[J].Meteorological Monthly.2015,41(3):380-387.
[28]熊亚军,廖晓农,李梓铭,等.KNN数据挖掘算法在北京地区霾等级预报中的应用[J].气象,2015,41(1):98-104.Xiong Y J,Liao X N,Li Z M,et al.Application of KNN data mining algorithm to haze grade forecasting in Beijing[J].Meteorological Monthly.2015,41(1):98-104.
[29]赵秀娟,徐敬,张自银,等.北京区域环境气象数值预报系统及PM_(2.5)预报检验[J].应用气象学报,2016,27(2):160-172.Zhao X J,Xu J,Zhang Z Y,et al.Beijing Regional Environmental Metrology prediction system and its performance test of PM_(2.5)concentration[J].Journal of applied metrological science.2016,27(2):160-172.
[30]邓涛,邓雪娇,吴兑,等.珠三角灰霾数值预报模式与业务运行评估[J].气象科技进展,2012,2(6):38-44.Deng T,Deng X J,Wu D,et al.Study on Numerical Forecast Model of Haze over Pearl River Delta Region and Routine Business Assessment[J].Advances in Meteorological Science and Technology.2012,2(6):38-44.
[31]李锋,朱彬,安俊岭,等.2013年12月初长江三角洲及周边地区重霾污染的数值模拟[J].中国环境科学,2015,35(7):1965-1974.Li F,Zhu B,An J L,et al.Modeling study of a severe haze episode occurred over the Yangtze River Delta and its surrounding regions during early December,2013[J].China Environmental Science,2015,35(7):1965-1974.
[32]蔡子颖,刘爱霞,韩素芹,等.天津低能见度特征初探[J].气象,2014,40(1):114-118.Cai Z Y,Liu A X,Han S Q,et al.Research of Characteristics on low visibility in Tianjin[J].Meteorological monthly.2014,40(1):114-118.
[33]马楠,赵春生,陈静,等.基于实测PM_(2.5)、能见度和相对湿度分辨雾霾的新方法[J].中国科学:地球科学,2015,45(2):227-235.Ma N,Zhao C S,Chen J,et al.A novel method for distinguishing fog and haze based on PM_(2.5),visibility,and relative humidity[J].Science China:Earth Sciences,2014(57):2156-2164.
[34]白永清,祁海霞,刘琳,等.武汉大气能见度与PM_(2.5)浓度及相对湿度关系的非线性分析及能见度预报[J].气象学报,2016,74(2):189-199.Bai Y Q,Qi H X,Liu L,et al.Study on the nonlinear relationship among the visibility,PM_(2.5) concentration and relative humidity in Wuhan and visibility prediction[J].Acta Meteorological sinica.2016,74(2):189-199.
[35]胡俊,赵天良,张泽锋,等.霾污染环境大气能见度参数化方案的改进[J].环境科学研究,2017,30(11):1680-1688.Hu J,Zhao T L,Zhang Z F,et al.Upgradeding atmospheric visibility parameterization scheme for haze pollution environment[J].Research of Environmental Sciences,2017,30(11):1680-1688.
[36]沈铁迪,王体健,陈璞珑,等.南京城区夏秋季能见度与PM_(2.5)化学成分的关系[J].中国环境科学,2015,35(3):652-658.Shen T D,Wang T J,Chen P L,et al.Relationship between atmospheric visibility and chemical composition of PM 2.5 in the summer and autumn of Nanjing[J].China Environmental Science.2015,35(3):652-658.
[37]古金霞,董海燕,白志鹏,等.天津市颗粒物散射消光特征及化学组分贡献研究[J].中国环境科学,2012,32(1):17-22.Gu J X,Dong H Y,Bai Z P,et al.Light scattering extinction characterization of particulates and chemical composition contribution in Tianjin[J].China Environmental Science.2012,32(1):17-22.
[38]尚倩,李子华,杨军,等.南京冬季大气气溶胶粒子谱分布及其对能见度的影响[J].环境科学,2011,32(9):2750-2760.Shan Q,Li Z H,Yang J,et al.Size Distributions of Aerosol Particles and the Impact on Visibility in Winter of Nanjing[J].Environmental Science.2011,32(9):2750-2760.
[39]韩素芹,张裕芬,李英华,等.天津市春季气溶胶消光特征和辐射效应的数值模拟[J].中国环境科学,2011,31(1):8-12.Han S Q,Zhang Y F,Li Y H,et al.Simulation of extinction and radiant effect of aerosol in spring of Tianjin City[J].China Environmental Science,2011,31(1):8-12.
[40]Mu Q,Lammel G,Gencarelli C N,et al.Regional modelling of polycyclic aromatic hydrocarbons:WRF/Chem-PAH model development and East Asia case studies[J].Atmospheric Chemistry&Physics,2017,2017(17):12253-12267.
[41]Ryu Y H,Hodzic A,Barre J,et al.Quantifying errors in surface ozone predictions associated with clouds over CONUS:A WRF-Chem modeling study using satellite cloud retrievals[J].Atmospheric Chemistry&Physics,2018,(18):7509-7525.
[42]Zhang L,Li Q,Wang T,et al.Combined impacts of nitrous acid and nitryl chloride on lower-tropospheric ozone:new module development in WRF-Chem and application to China[J].Atmospheric Chemistry&Physics,2017,(17):9733-9750.
[43]中国气象局.QX/T 113中华人民共和国气象行业标准:霾的观测和预报等级[S].2010.China Meteorological Administration.QX/T 113.Meteorological industry standard of the People's Republic of China:Haze observation and forecast level
[2]吴兑,毕雪岩,邓雪娇,等.珠江三角洲大气灰霾导致能见度下降问题研究[J].气象学报,2006,64(4):510-517.Wu D,Bi X,Deng X J,et al.Effect of atmospheric haze on the deterioration of visibility over the pear river detla[J].Acta Meteorological sinica,2006,64(4):510-517.
[3]陈欢欢,吴兑,谭浩波,等.珠江三角洲2001~2008年灰霾天气过程特征分析[J].热带气象学报,2010,26(2):147-155.Chen H H,Wu D,Tan H B,et al.Study on the character of haze weather process from the year 2001 to 2008 over the pearl river delta[J].Journal of tropical meteorology,2010,26(2):147-155.
[4]吴蒙,范绍佳,吴兑,等.广州地区灰霾与清洁天气变化特征及影响因素分析[J].中国环境科学,2012,32(8):1409-1415.Wu M,Fan S J,Wu D,et al.Characteristics and influence factors study of haze and cleaning weather over Guangzhou Area[J].China Environmental Science.2012,32(8):1409-1415.
[5]刘琼,耿福海,陈勇航,等.上海不同强度干霾期间气溶胶垂直分布特征[J].中国环境科学,2012,32(2):207-213.Liu Q,Geng F H,Chen Y H,et al.Vertical distribution of aerosols during different intense dry haze periods around Shanghai[J].China Environmental Science,2012,32(2):207-213.
[6]王苑,耿福海,陈勇航,等.基于微脉冲激光雷达的上海浦东地区不同强度霾研究[J].中国环境科学,2013,33(1):21-29.Wang Y,Geng F H,Chen Y H,et al.Study of haze with different intensity categories at Pudong District in Shanghai based on micropulse lidar[J].China Environmental Science,2013,33(1):21-29.
[7]王静,牛生杰,许丹,等.南京一次典型雾霾天气气溶胶光学特性[J].中国环境科学,2013,33(2):201-208.Wang J,Niu S J,Xu D,et al.Aerosol optical properties during the typical haze/fog event in Nanjing[J].China Environmental Science.2013,33(2):201-208.
[8]朱佳雷,王体健,邢莉,等.江苏省一次重霾污染天气的特征和机理分析[J].中国环境科学,2011,31(12):1943-1950.Zhu J L,Wang T J,Xing L,et al.Analysis on the characteristics and mechanism of a heavy haze episode in Jiangsu Province[J].China Environmental Science.2011,31(12):1943-1950.
[9]吴兑,廖碧婷,吴蒙,等.环首都圈霾和雾的长期变化特征与典型个例的近地层输送条件[J].环境科学学报,2014,34(1):1-11.Wu D,Liao B,Wu M,et al.The long-term trend of haze and fog days and the surface layer transport conditions under haze weather in North China[J].Acta Scientiae Circumstantiae,2014,34(1):1-11.
[10]薛亦峰,周震,聂滕,等.2015年12月北京市空气重污染过程分析及污染源排放变化[J].环境科学,2016,37(5):1593-1601.Xue Y F,Zhou Z,Nie T,et al.Exploring the Severe Haze in Beijing During December,2015:Pollution Process and Emissions Variation[J].Environmental Science.2016,37(5):1593-1601.
[11]穆穆,张人禾.应对灰霾天气:气象科学与技术大有可为[J].中国科学:地球科学,2014,44(1):1-2.Mu M,Zhang R H.Dealing with Haze Weather:Great Prospects for Meteorological Science and Technology[J].Chinese Science:Geosciences,2014,44(1):1-2.
[12]董春卿,郑有飞,武永利,等.边界层方案对山西冬季一次静稳天气PM_(2.5)浓度模拟的影响[J].中国环境科学,2016,36(6):1669-1680.Dong C Q,Zheng Y F,Wu Y L,et al.The effects of different planetary boundary layer schemes on PM_(2.5) concentration simulations in winter stable weather of Shanxi[J].China Environmental Science.2016,36(6):1669-1680.
[13]李令军,王占山,张大伟,等.2013~2014年北京大气重污染特征研究[J].中国环境科学,2016,36(1):27-35.Ling J,Wang Z S,Zhang D W,et al.Analysis of heavy air pollution episodes in Beijing during 2013~2014[J].China Environmental Science,2016,36(1):27-35.
[14]刘兴瑞,马嫣,崔芬萍,等.南京北郊一次重污染事件期间PM_(2.5)理化特性及其对大气消光的影响[J].环境化学,2016,35(6):1164-1171.LiuX R,Ma Y,Cui F P,et al.Physicochemical characteristics of PM_(2.5)and impacts on light extinction during the heavy pollution period at North Suburban Nanjing[J].Environmental Chemistry,2016,35(6):1164-1171.
[15]蔡子颖,韩素芹,张敏,等.天津地区污染天气分析中垂直扩散指标构建及运用[J].环境科学,2018,39(6):2548-2556.Cai Z Y,Han S Q,Zhang M,et al.Construction and Application of Vertical Diffusion Index for Analyzing Weather During Pollution Events in Tianjin[J].Environmental Science,2018,39(6):2548-2556.
[16]Tang G,Zhu X,Hu B,et al.Impact of emission controls on air quality in Beijing during APEC 2014:lidar ceilometer observations[J].Atmospheric Chemistry&Physics,2015,15(21):12667-12680.
[17]Han S,Hao T,Zhang Y,et al.Vertical observation and analysis on rapid formation and evolutionary mechanisms of a prolonged haze episode over central-eastern China.Science of total environment[J].Science of the total environment,2018,2018(616):135-146.
[18]李梦,唐贵谦,黄俊,等.京津冀冬季大气混合层高度与大气污染的关系[J].环境科学,2015,36(6):1935-1943.Li M,Tang G Q,Huang J,et al.Characteristics of Winter Atmospheric Mixing Layer Height in Beijing-Tianjin-Hebei Region and Their Relationship with the Atmospheric Pollution[J].Environmental Science,2015,36(6):1935-1943.
[19]蔡子颖,韩素芹,汪靖,等.基于天气背景天津地区重污染天气特征分析[J].环境科学学报,2017,37(10):3906-3917.Cai Z Y,Han S Q,Wang J,et al.Analysis of synoptic characteristics of heavy pollution in Tianjin based on weather background[J].Acta Scientiae Circumstantiae,2017,37(10):3906-3917.
[20]周鑫,丁菊丽,田伟,等.能见度参数化方案概述[J].气象研究与应用,2009,30(3):22-25.Zhou X,Ding J,Tian W,et al.Introduction of Visibility Parameterization Scheme[J].Journal of meteorological research and application.2009,30(3):22-25.
[21]边海,张裕芬,韩素芹,等.天津市大气能见度与颗粒物污染的关系[J].中国环境科学,2012,32(3):406-410.Bian H,Han S Q,Zhang Y F,et al.Relationship between atmospheric visibility and particulate matter pollution in Tianjin[J].China Environmental Science.2012,32(3):406-410.
[22]陈义珍,赵丹,柴发合,等.广州市与北京市大气能见度与颗粒物质量浓度的关系[J].中国环境科学,2010,30(7):967-971.Chen Y Z,Zhao D,Chai F H,et al.Correlation between the atmospheric visibility and aerosol fine particle concentrations in Guangzhou and Beijing[J].China Environmental Science.2010,30(7):967-971.
[23]姚青,蔡子颖,韩素芹,等.2009年秋冬季天津低能见度天气下气溶胶污染特征[J].气象,2012,38(9):1096-1102.Yao Q,Cai Z Y,Han S Q,et al.Study on Pollution Characteristics of aerosols during low visibility weather at Tianjin City in Autumn and Winter 2009[J].Meteorological monthly.2012,38(9):1096-1102.
[24]姚青,韩素芹,蔡子颖,等.天津城区春季大气气溶胶消光特性研究[J].中国环境科学,2012,32(5):795-802.Yao Q,Han S Q,Cai Z Y,et al.Study on characteristic of aerosol extinction at Tianjin City in the spring[J].China Environmental Science,2012,32(5):795-802.
[25]刘西川,高太长,刘磊,等.降水现象对大气消光系数和能见度的影响[J].应用气象学报,2010,21(4):433-441.Liu X C,Gao T C,Liu L,et al.Influences of Precipitation on atmospheric Extinction coefficient and Visibility[J].Journal of applied metrological science,2010,21(4):433-441.
[26]刘宁微,马雁军,王扬锋.辽宁中部城市群夏季大气能见度的观测研究[J].气象学报,2012,70(4):814-820.Liu N W,Ma Y J,Wang Y F,et al.Observational study of atmospheric visibility in summer in the area of multicities in central Liaoning Province[J].Acta Meteorological Sinica,2012,70(4):814-820.
[27]饶晓琴,马学款,黄威.2014年12月大气环流和天气分析[J].气象,2015,41(3):380-387.Wang J K,Gui H L,Ma X K,et al.Analysis of the December 2017Atmospheric circulation and weather[J].Meteorological Monthly.2015,41(3):380-387.
[28]熊亚军,廖晓农,李梓铭,等.KNN数据挖掘算法在北京地区霾等级预报中的应用[J].气象,2015,41(1):98-104.Xiong Y J,Liao X N,Li Z M,et al.Application of KNN data mining algorithm to haze grade forecasting in Beijing[J].Meteorological Monthly.2015,41(1):98-104.
[29]赵秀娟,徐敬,张自银,等.北京区域环境气象数值预报系统及PM_(2.5)预报检验[J].应用气象学报,2016,27(2):160-172.Zhao X J,Xu J,Zhang Z Y,et al.Beijing Regional Environmental Metrology prediction system and its performance test of PM_(2.5)concentration[J].Journal of applied metrological science.2016,27(2):160-172.
[30]邓涛,邓雪娇,吴兑,等.珠三角灰霾数值预报模式与业务运行评估[J].气象科技进展,2012,2(6):38-44.Deng T,Deng X J,Wu D,et al.Study on Numerical Forecast Model of Haze over Pearl River Delta Region and Routine Business Assessment[J].Advances in Meteorological Science and Technology.2012,2(6):38-44.
[31]李锋,朱彬,安俊岭,等.2013年12月初长江三角洲及周边地区重霾污染的数值模拟[J].中国环境科学,2015,35(7):1965-1974.Li F,Zhu B,An J L,et al.Modeling study of a severe haze episode occurred over the Yangtze River Delta and its surrounding regions during early December,2013[J].China Environmental Science,2015,35(7):1965-1974.
[32]蔡子颖,刘爱霞,韩素芹,等.天津低能见度特征初探[J].气象,2014,40(1):114-118.Cai Z Y,Liu A X,Han S Q,et al.Research of Characteristics on low visibility in Tianjin[J].Meteorological monthly.2014,40(1):114-118.
[33]马楠,赵春生,陈静,等.基于实测PM_(2.5)、能见度和相对湿度分辨雾霾的新方法[J].中国科学:地球科学,2015,45(2):227-235.Ma N,Zhao C S,Chen J,et al.A novel method for distinguishing fog and haze based on PM_(2.5),visibility,and relative humidity[J].Science China:Earth Sciences,2014(57):2156-2164.
[34]白永清,祁海霞,刘琳,等.武汉大气能见度与PM_(2.5)浓度及相对湿度关系的非线性分析及能见度预报[J].气象学报,2016,74(2):189-199.Bai Y Q,Qi H X,Liu L,et al.Study on the nonlinear relationship among the visibility,PM_(2.5) concentration and relative humidity in Wuhan and visibility prediction[J].Acta Meteorological sinica.2016,74(2):189-199.
[35]胡俊,赵天良,张泽锋,等.霾污染环境大气能见度参数化方案的改进[J].环境科学研究,2017,30(11):1680-1688.Hu J,Zhao T L,Zhang Z F,et al.Upgradeding atmospheric visibility parameterization scheme for haze pollution environment[J].Research of Environmental Sciences,2017,30(11):1680-1688.
[36]沈铁迪,王体健,陈璞珑,等.南京城区夏秋季能见度与PM_(2.5)化学成分的关系[J].中国环境科学,2015,35(3):652-658.Shen T D,Wang T J,Chen P L,et al.Relationship between atmospheric visibility and chemical composition of PM 2.5 in the summer and autumn of Nanjing[J].China Environmental Science.2015,35(3):652-658.
[37]古金霞,董海燕,白志鹏,等.天津市颗粒物散射消光特征及化学组分贡献研究[J].中国环境科学,2012,32(1):17-22.Gu J X,Dong H Y,Bai Z P,et al.Light scattering extinction characterization of particulates and chemical composition contribution in Tianjin[J].China Environmental Science.2012,32(1):17-22.
[38]尚倩,李子华,杨军,等.南京冬季大气气溶胶粒子谱分布及其对能见度的影响[J].环境科学,2011,32(9):2750-2760.Shan Q,Li Z H,Yang J,et al.Size Distributions of Aerosol Particles and the Impact on Visibility in Winter of Nanjing[J].Environmental Science.2011,32(9):2750-2760.
[39]韩素芹,张裕芬,李英华,等.天津市春季气溶胶消光特征和辐射效应的数值模拟[J].中国环境科学,2011,31(1):8-12.Han S Q,Zhang Y F,Li Y H,et al.Simulation of extinction and radiant effect of aerosol in spring of Tianjin City[J].China Environmental Science,2011,31(1):8-12.
[40]Mu Q,Lammel G,Gencarelli C N,et al.Regional modelling of polycyclic aromatic hydrocarbons:WRF/Chem-PAH model development and East Asia case studies[J].Atmospheric Chemistry&Physics,2017,2017(17):12253-12267.
[41]Ryu Y H,Hodzic A,Barre J,et al.Quantifying errors in surface ozone predictions associated with clouds over CONUS:A WRF-Chem modeling study using satellite cloud retrievals[J].Atmospheric Chemistry&Physics,2018,(18):7509-7525.
[42]Zhang L,Li Q,Wang T,et al.Combined impacts of nitrous acid and nitryl chloride on lower-tropospheric ozone:new module development in WRF-Chem and application to China[J].Atmospheric Chemistry&Physics,2017,(17):9733-9750.
[43]中国气象局.QX/T 113中华人民共和国气象行业标准:霾的观测和预报等级[S].2010.China Meteorological Administration.QX/T 113.Meteorological industry standard of the People's Republic of China:Haze observation and forecast level