硅烷偶联剂在橡胶中的应用研究进展
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摘要
介绍硅烷偶联剂在橡胶工业中的应用研究进展,展望橡胶用硅烷偶联剂的发展趋势和应用前景。硅烷偶联剂的使用大大提高了橡胶制品的综合性能,促进了无机填料在橡胶工业中的应用。目前橡胶用硅烷偶联剂主要种类为含硫烃基类、乙烯基类、甲基丙烯酰氧烷基类、氨烃基类和环氧烃基类。随着新型轮胎和橡胶制品的快速发展,市场对橡胶用硅烷偶联剂的性能和使用技术也提出更高的要求,尤其是轮胎绿色化进程的加快,对硅烷偶联剂的需求快速增长,以NXT为代表的新型硅烷偶联剂是未来橡胶用硅烷偶联剂的发展方向之一。
引文
[1]余和平,李思东.环氧化天然橡胶研究进展[J].橡胶工业,1998,45(4):246-252.
[2]吕婧,赵菲.天然橡胶种类对白炭黑填充胶性能的影响[J].世界橡胶工业,2015,42(4):1-4.
[3]张玥珺,徐敏,赵西坡,等.含硫硅烷偶联剂对增强填料的改性及其在橡胶中的应用研究进展[J].合成橡胶工业,2017,40(4):327-331.
[4]Nik Z,Noriman,Hanafi Ismail.Properties of Styrene Butadiene Rubber(SBR)/Recycled Acrylonitrile Butadiene Rubber(NBRr)Blends:The Effects of Carbon Black/Silica(CB/Sil)Hybrid Filler and Silane Coupling Agent Si69[J].Journal of Applied Polymer Science,2012,124(1):19-27.
[5]Xie Yanjun,Callum A S,Xiao Zefong,et a1.Silane Coupling Agents Used for Natural Fiber/Polymer Composites:A review[J].Composites(Part A):Applied Science&Manufacturing,2010,41(7):806-819.
[6]鲁学峰,郝智,盛翔,等.不同改性白炭黑增强天然橡胶复合材料的性能研究[J].化工新型材料,2017,45(8):232-234.
[7]Murakami K,Lio S,Ikeda Y,et al.Effect of Silane-coupling Agent on Natural Rubber Filled with Silica Generated in Situ[J].Journal of Materials Science,2003,38(7):1447-1455.
[8]彭华龙,房建明,谢翛然,等.橡胶助剂Silane-M在SBR/无机填料复合材料中的应用[J].广东化工,2016,43(2):50-52.
[9]Pongdhorn Sae-oui,Chakrit Sirisinha,Uthai Thepsuwan,et al.Roles of Silane Coupling Agents on Properties of Silica-filled Polychloroprene[J].European Polymer Journal,2006,42(3):479-486.
[10]颜和祥,张勇,张隐西,等.硅烷偶联剂及其对白炭黑的改性研究进展[J].橡胶工业,2004,51(6):376-378.
[11]邬继荣,陈利民,许文东.新型硅烷偶联剂研究进展[J].化工生产与技术,2009,16(4):48-50.
[12]张先亮,唐红顶,廖俊.硅烷偶联剂-原理、合成与应用[M].北京:化学工业出版社,2011.
[13]崔凌峰,熊玉竹,戴骏,等.改性白炭黑/天然橡胶复合材料的制备及性能[J].高分子材料科学与工程,2017,33(5):158-163.
[14]张帆,管俊芳,邱鑫强,等.改性白炭黑对NR/BR/SBR并用橡胶力学性能的影响[J].硅酸盐通报,2015,34(2):585-590.
[15]Liu Jiesheng,Wu Shaopeng,Dong E.Effect of Coupling Agent as Integral Blend Additive on Silicone Rubber Sealant[J].Journal of Applied Polymer Science,2013,128(4):2337-2343.
[16]白世义,张震,杜丽萍,等.乙烯基硅烷偶联剂[J].有机硅材料,2000,14(2):23-25.
[17]Cevdet Kaynak,Cengiz Celikbilek,Guneri Akovali,et al.Use of Silane Coupling Agents to Improve Epoxy-rubber Interface[J].European Polymer Journal,2003,39(3):1125-1132.
[18]彭占杰,崔杰,韩丙凯,等.硅烷偶联剂在橡胶复合材料中的研究进展[J].特种橡胶制品,2014,35(6):65-69.
[19]崔小明.硅烷偶联剂在橡胶工业中的应用研究进展[J].精细与专用化学品,2012,21(3):15-18.
[20]Cichomski E M,Tolpekina T V,Schultz S M,et al.Structural Influences of Silane Coupling Agents on the Dynamic Properties of a SBR/Silica Compound[J].Polymer Processing Society,2013,7(18):8-10.
[21]杨雪梅,陈福林,刘晓暄,等.有机过氧化物硫化体系在橡胶应用中的研究进展[J].特种橡胶制品,2009,30(3):79-84.
[22]He Shaojia,Xue Yang,Lin Jun,et a1.Effect of Silane Coupling Agent on the Structure and Mechanical Properties of Nanodispersed Clay Filled Styrene Butadiene Rubber[J].Polymer Composites,2014,37(3):890-896.
[23]江学良,徐雄,张娇,等.端巯基硅烷改性白炭黑填充丁基橡胶[J].武汉工程大学学报,2014,36(9):33-37.
[24]Ren Hui,Qu Yixin,Zhao Suhe.Reinforcement of StyreneButadiene Rubber with Silica Modified by Silane Coupling Agents:Experimental and Theoretical Chemistry Study[J].Chinese Journal of Chemical Engineering,2006,14(1):93-98.
[25]王灿,阮少阳,尹超.我国含硫硅烷偶联剂的生产与应用[J].橡胶科技市场,2011,10(10):8-12.
[26]Zheng Junchi,Ye Xin,Han Dongli,et al.Silica Modified by Alcohol Polyoxy-ethylene Ether and Silane Coupling Agent Together to Achieve High Performance Rubber Composites Using the Latex Compounding Method[J].Polymers,2018,10(1):1-17.
[27]Sung-Seen Choi.Influence of Storage Time and Temperature and Silane Coupling Agent on Bound Rubber Formation in Filled Styrene-Butadiene Rubber Compounds[J].Polymer Testing,2002,21(2):201-208.
[28]王妮妮,王启飞,廖明义,等.Si69/白炭黑/炭黑补强体系对SIBR胎面胶性能的影响[J].弹性体,2006,16(4):17-20.
[29]崔凌峰,熊玉竹,戴骏,等.含硫偶联剂对白炭黑-天然橡胶的硫化特性及力学性能的影响[J].中国粉体技术,2017,23(1):48-52.
[30]Tomoyoshi Fukuda,Syuji Fujii,Yoshinobu Nakamura,et al.Mechanical Properties of Silica Particle-filled Styrene-Butadiene Rubber Composites Containing Polysulfide-type Silane Coupling Agents:Influence of Loading Method of Silane[J].Applied Polymer,2013,130(1):322-329.
[31]孙燕,朱臣昌,潘成松.Si69和Si-264在有效硫化体系中补强效果之比较[J].世界橡胶工业,2009,36(3):8-13.
[32]Qu Liangliang,Yu Guozhu,Xie Ximing,et al.Effect of Silane Coupling Agent on Filler and Rubber Interaction of Silica Reinforced Solution Styrene Butadiene Rubber[J].Polymer Composites,2013,34(10):1575-1582.
[33]Joshi P G,Cruse R J,Pickwell R J,et al.白炭黑胎面胶的新一代硅烷偶联剂[J].涂学忠,译.轮胎工业,2005,25(2):96-102.
[34]车伟,林世军.硅烷偶联剂NXT在全钢载重子午线轮胎钢丝带束层粘合胶中的应用[J].轮胎工业,2008,28(9):543-547.
[35]Wirunya Keawwattana,Thiranan Thuechart,Jumras Limtrakul.The Effect of Coupling Agents on Natural Zeolite-Filled Natural Rubber[J].Journal of Chemistry and Chemical Engineering,2011(5):413-422.
[36]孙晋,宋义虎,周明,等.3-己酰基硫代-1-丙基三乙氧基硅烷的合成及其在SSBR/SiO2复合体系中偶联效果研究[J].高分子学报,2007(5):446-450.
[37]葛国杰.硅烷偶联剂在SSBR/SiO2体系中的作用研究[D].青岛:青岛科技大学,2013.
[38]花曙太,刘连波,罗洪罡,等.硅烷偶联剂对白炭黑胶料性能的影响[J].橡胶科技,2013,11(8):28-30.
[39]Yan Hexiang,Sun Kang,Zhang Yong,et al.Effects of Mixing Conditions on the Reaction of 3-Octanoylthio-1-Propyltriethoxysilane during Mixing with Silica Filler and Natural Rubber[J].Journal of Applied Polymer Science,2004,94(6):2295-2301.
[40]彭华龙,刘岚,罗远芳,等.含硫硅烷偶联剂对白炭黑填充天然橡胶填料网络结构及流变行为的影响[J].合成橡胶工业,2009,32(3):227-231.
[41]彭华龙,刘岚,罗远芳,等.橡胶助剂Silane-M对丁苯橡胶/白炭黑复合材料硫化性能的影响[J].合成橡胶工业,2009,32(4):306-308.
[2]吕婧,赵菲.天然橡胶种类对白炭黑填充胶性能的影响[J].世界橡胶工业,2015,42(4):1-4.
[3]张玥珺,徐敏,赵西坡,等.含硫硅烷偶联剂对增强填料的改性及其在橡胶中的应用研究进展[J].合成橡胶工业,2017,40(4):327-331.
[4]Nik Z,Noriman,Hanafi Ismail.Properties of Styrene Butadiene Rubber(SBR)/Recycled Acrylonitrile Butadiene Rubber(NBRr)Blends:The Effects of Carbon Black/Silica(CB/Sil)Hybrid Filler and Silane Coupling Agent Si69[J].Journal of Applied Polymer Science,2012,124(1):19-27.
[5]Xie Yanjun,Callum A S,Xiao Zefong,et a1.Silane Coupling Agents Used for Natural Fiber/Polymer Composites:A review[J].Composites(Part A):Applied Science&Manufacturing,2010,41(7):806-819.
[6]鲁学峰,郝智,盛翔,等.不同改性白炭黑增强天然橡胶复合材料的性能研究[J].化工新型材料,2017,45(8):232-234.
[7]Murakami K,Lio S,Ikeda Y,et al.Effect of Silane-coupling Agent on Natural Rubber Filled with Silica Generated in Situ[J].Journal of Materials Science,2003,38(7):1447-1455.
[8]彭华龙,房建明,谢翛然,等.橡胶助剂Silane-M在SBR/无机填料复合材料中的应用[J].广东化工,2016,43(2):50-52.
[9]Pongdhorn Sae-oui,Chakrit Sirisinha,Uthai Thepsuwan,et al.Roles of Silane Coupling Agents on Properties of Silica-filled Polychloroprene[J].European Polymer Journal,2006,42(3):479-486.
[10]颜和祥,张勇,张隐西,等.硅烷偶联剂及其对白炭黑的改性研究进展[J].橡胶工业,2004,51(6):376-378.
[11]邬继荣,陈利民,许文东.新型硅烷偶联剂研究进展[J].化工生产与技术,2009,16(4):48-50.
[12]张先亮,唐红顶,廖俊.硅烷偶联剂-原理、合成与应用[M].北京:化学工业出版社,2011.
[13]崔凌峰,熊玉竹,戴骏,等.改性白炭黑/天然橡胶复合材料的制备及性能[J].高分子材料科学与工程,2017,33(5):158-163.
[14]张帆,管俊芳,邱鑫强,等.改性白炭黑对NR/BR/SBR并用橡胶力学性能的影响[J].硅酸盐通报,2015,34(2):585-590.
[15]Liu Jiesheng,Wu Shaopeng,Dong E.Effect of Coupling Agent as Integral Blend Additive on Silicone Rubber Sealant[J].Journal of Applied Polymer Science,2013,128(4):2337-2343.
[16]白世义,张震,杜丽萍,等.乙烯基硅烷偶联剂[J].有机硅材料,2000,14(2):23-25.
[17]Cevdet Kaynak,Cengiz Celikbilek,Guneri Akovali,et al.Use of Silane Coupling Agents to Improve Epoxy-rubber Interface[J].European Polymer Journal,2003,39(3):1125-1132.
[18]彭占杰,崔杰,韩丙凯,等.硅烷偶联剂在橡胶复合材料中的研究进展[J].特种橡胶制品,2014,35(6):65-69.
[19]崔小明.硅烷偶联剂在橡胶工业中的应用研究进展[J].精细与专用化学品,2012,21(3):15-18.
[20]Cichomski E M,Tolpekina T V,Schultz S M,et al.Structural Influences of Silane Coupling Agents on the Dynamic Properties of a SBR/Silica Compound[J].Polymer Processing Society,2013,7(18):8-10.
[21]杨雪梅,陈福林,刘晓暄,等.有机过氧化物硫化体系在橡胶应用中的研究进展[J].特种橡胶制品,2009,30(3):79-84.
[22]He Shaojia,Xue Yang,Lin Jun,et a1.Effect of Silane Coupling Agent on the Structure and Mechanical Properties of Nanodispersed Clay Filled Styrene Butadiene Rubber[J].Polymer Composites,2014,37(3):890-896.
[23]江学良,徐雄,张娇,等.端巯基硅烷改性白炭黑填充丁基橡胶[J].武汉工程大学学报,2014,36(9):33-37.
[24]Ren Hui,Qu Yixin,Zhao Suhe.Reinforcement of StyreneButadiene Rubber with Silica Modified by Silane Coupling Agents:Experimental and Theoretical Chemistry Study[J].Chinese Journal of Chemical Engineering,2006,14(1):93-98.
[25]王灿,阮少阳,尹超.我国含硫硅烷偶联剂的生产与应用[J].橡胶科技市场,2011,10(10):8-12.
[26]Zheng Junchi,Ye Xin,Han Dongli,et al.Silica Modified by Alcohol Polyoxy-ethylene Ether and Silane Coupling Agent Together to Achieve High Performance Rubber Composites Using the Latex Compounding Method[J].Polymers,2018,10(1):1-17.
[27]Sung-Seen Choi.Influence of Storage Time and Temperature and Silane Coupling Agent on Bound Rubber Formation in Filled Styrene-Butadiene Rubber Compounds[J].Polymer Testing,2002,21(2):201-208.
[28]王妮妮,王启飞,廖明义,等.Si69/白炭黑/炭黑补强体系对SIBR胎面胶性能的影响[J].弹性体,2006,16(4):17-20.
[29]崔凌峰,熊玉竹,戴骏,等.含硫偶联剂对白炭黑-天然橡胶的硫化特性及力学性能的影响[J].中国粉体技术,2017,23(1):48-52.
[30]Tomoyoshi Fukuda,Syuji Fujii,Yoshinobu Nakamura,et al.Mechanical Properties of Silica Particle-filled Styrene-Butadiene Rubber Composites Containing Polysulfide-type Silane Coupling Agents:Influence of Loading Method of Silane[J].Applied Polymer,2013,130(1):322-329.
[31]孙燕,朱臣昌,潘成松.Si69和Si-264在有效硫化体系中补强效果之比较[J].世界橡胶工业,2009,36(3):8-13.
[32]Qu Liangliang,Yu Guozhu,Xie Ximing,et al.Effect of Silane Coupling Agent on Filler and Rubber Interaction of Silica Reinforced Solution Styrene Butadiene Rubber[J].Polymer Composites,2013,34(10):1575-1582.
[33]Joshi P G,Cruse R J,Pickwell R J,et al.白炭黑胎面胶的新一代硅烷偶联剂[J].涂学忠,译.轮胎工业,2005,25(2):96-102.
[34]车伟,林世军.硅烷偶联剂NXT在全钢载重子午线轮胎钢丝带束层粘合胶中的应用[J].轮胎工业,2008,28(9):543-547.
[35]Wirunya Keawwattana,Thiranan Thuechart,Jumras Limtrakul.The Effect of Coupling Agents on Natural Zeolite-Filled Natural Rubber[J].Journal of Chemistry and Chemical Engineering,2011(5):413-422.
[36]孙晋,宋义虎,周明,等.3-己酰基硫代-1-丙基三乙氧基硅烷的合成及其在SSBR/SiO2复合体系中偶联效果研究[J].高分子学报,2007(5):446-450.
[37]葛国杰.硅烷偶联剂在SSBR/SiO2体系中的作用研究[D].青岛:青岛科技大学,2013.
[38]花曙太,刘连波,罗洪罡,等.硅烷偶联剂对白炭黑胶料性能的影响[J].橡胶科技,2013,11(8):28-30.
[39]Yan Hexiang,Sun Kang,Zhang Yong,et al.Effects of Mixing Conditions on the Reaction of 3-Octanoylthio-1-Propyltriethoxysilane during Mixing with Silica Filler and Natural Rubber[J].Journal of Applied Polymer Science,2004,94(6):2295-2301.
[40]彭华龙,刘岚,罗远芳,等.含硫硅烷偶联剂对白炭黑填充天然橡胶填料网络结构及流变行为的影响[J].合成橡胶工业,2009,32(3):227-231.
[41]彭华龙,刘岚,罗远芳,等.橡胶助剂Silane-M对丁苯橡胶/白炭黑复合材料硫化性能的影响[J].合成橡胶工业,2009,32(4):306-308.
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