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浙江省典型农田土壤重金属污染及生态风险评价
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  • 英文篇名:Heavy Metals in Typical Farmland Soils of Zhejiang Province: Levels, Sources and Ecological Risks
  • 作者:张云芸 ; 马瑾 ; 魏海英 ; 石陶然
  • 英文作者:ZHANG Yunyun;MA Jin;WEI Haiying;SHI Taoran;College of Environmental Sciences and Resource, Shanxi University;State Key Laboratory of Environment Criteria and Risk Assessment/Chinese Research Academy of Environmental Sciences;
  • 关键词:土壤 ; 重金属 ; 生态风险 ; 预警 ; 浙江
  • 英文关键词:soil;;heavy metal;;ecological risk;;early warning;;Zhejiang province
  • 中文刊名:生态环境学报
  • 英文刊名:Ecology and Environmental Sciences
  • 机构:山西大学环境与资源学院;中国环境科学研究院/环境基准与风险评估国家重点实验室;
  • 出版日期:2019-06-18
  • 出版单位:生态环境学报
  • 年:2019
  • 期:06
  • 基金:国家重点研发计划项目(2016YFD0800302);; 中央级公益性科研院所基本科研业务专项(2016YSKY032)
  • 语种:中文;
  • 页:167-175
  • 页数:9
  • CN:44-1661/X
  • ISSN:1674-5906
  • 分类号:X53;X826
摘要
浙江是中国经济社会发展最快的省份之一,人类活动对土壤环境扰动强烈。为系统了解浙江省典型农田土壤重金属的污染水平、空间分布特征及生态风险,采集并分析了67个代表性农田土壤表层样品中的8种重金属元素(As、Cd、Cr、Cu、Mn、Ni、Pb和Zn),采用主成分分析法进行来源解析,采用污染负荷指数(PLI)、潜在生态风险指数(RI)和生态风险预警指数(IER)对农田土壤重金属污染与环境风险进行评价。结果表明,浙江省典型农田土壤环境重金属为轻度污染状态,研究区域农田土壤中的Cr、Ni和As处于轻微污染水平;Pb、Hg、Cu和Zn处于轻度污染水平;Cd处于重度污染水平,应作为优先控制元素。研究区域农田土壤Cr、Cu、Zn和Ni的来源主要受自然因素控制,Cd和Hg主要来源于工农业生产等人为活动,Pb主要来源于交通源。浙江省的金华市义乌、绍兴市诸暨、绍兴市嵊州、丽水市缙云县岩沿村应作为浙江省典型农田土壤的优先控制区域。浙江省典型农田土壤重金属环境存在轻微生态风险。
        Zhejiang is one of the provinces with the fastest economic and social development in China, the soil environment is strongly disturbed by human activities. In order to systematically understand the levels, sources and ecological risks of heavy metals in typical farmland soils of Zhejiang Province, 67 representative soil samples were collected and eight heavy metals(As,Cd, Cr, Cu, Mn, Ni, Pb and Zn) were determined. The pollution load index(PLI), potential ecological risk index(RI) and ecological risk warning index(IER) was used to evaluate heavy metal pollution and ecological risks. The results showed that farmland soils were slightly polluted by Cr, Ni, As, Pb, Hg, Cu and Zn, which were seriously polluted by Cd, so Cd was suggested to be the priority control pollutant. Principal Component Analysis(PCA) was used to analyze their sources, the result showed that Cr, Cu, Zn and Ni in farmland soils mainly came from natural sources, Cd and Hg mainly originated from artificial activities such as industrial and agricultural production, while Pb mainly came from traffic sources. According to the results of spatial distribution analysis, Yiwu in Jinhua city, Zhuji in Shaoxing city, Shengzhou in Shaoxing city, and Yanyan village in Jinyun county of Lishui city was suggested to be the priority control regions. There were slight ecological risks resulted by heavy metals pollution in the farmland soils of Zhejiang province.
引文
CAI J,WANG J D,ZHANG Y J,et al.,2017.Source apportionment of Pb-containing particles in Beijing during January 2013[J].Environment Pollution,226:30-40.
    CHANG C Y,YU H Y,CHEN J J,et al.,2014.Accumulation of heavy metals in leaf vegetables from agricultural soils and associated potential health risks in the Pearl River Delta,South China[J].Environmental Monitoring and Assessment,186(3):1547-1560.
    HAKANSON L,1980.An ecological risk index for aquatic pollution control:A sedimentological approach[J].Water Research,14(8):975-1001.
    HAN L F,GAO B,HAO H,et al.,2018.Lead contamination in sediments in the past 20 years:a challenge for China[J].Science of the Total Environment,640-641:746-756.
    LIU D X,MA J H,SUN Y L,et al.,2016.Spatial distribution of soil magnetic susceptibility and correlation with heavy metal pollution in Kaifeng City,China[J].Catena,139:53-60.
    LIU X,WU J,XU J,2006.Characterizing the risk assessment of heavy metals and sampling uncertainty analysis in paddy field by geostatistics and GIS[J].Environmental Pollution,141(2):257-264.
    RAPANT S,KORDIK J,2003.An environmental risk assessment map of the Slovak Republic:Application of data from geochemical atlases[J].Environmental Geology,44(4):400-407.
    SHI T R,MA J,WU F Y,et al.,2019.Mass balance-based inventory of heavy metals inputs to and outputs from agricultural soils in Zhejiang Province,China[J].Science of the Total Environment,649:1269-1280.
    TOMLINSON D L,WILSON J G,HARRIS C R,et al.,1980.Problems in the assessment of heavy metals levels in estuaries and the formation of pollution index[J].Helgol?nder Meeresun-tersuchungen,33(1-4):566-575.
    XIAO R,WANG S,LI R,et al.,2017.Soil heavy metal contamination and health risks associated with artisanal gold mining in Tongguan,Shaanxi,China[J].Ecotoxicology and Environmental Safely,141:17-24.
    ZHAO F J,MA Y,ZHU Y G,et al.,2015.Soil contamination in China:Current status and mitigation strategies[J].Environmental Science&Technology,49(2):750-759.
    ZHOU J,LIANG J N,HU Y M,et al.,2018.Exposure risk of local residents to copper near the largest flash copper smelter in China[J].Science of the Total Environment,630(15):453-461.
    曹伟,周生路,王国梁,等,2010.长江三角洲典型区工业发展影响下土壤重金属空间变异特征[J].地理科学,30(2):283-289.CAO W,ZHOU S L,WANG G L,et al.,2010.Spatial variability of soil heavy metals under the influence of industrial development in typical areas of the Yangtze River Delta[J].Scientia Geographica Sinica,30(2):283-289.
    陈江,张海燕,何小峰,等,2010.湖州市土壤重金属元素分布及潜在生态风险评价[J].土壤,42(4):595-599.CHEN J,ZHANG H Y,HE X F,et al.,2010.Distribution and evaluation on potential ecological risk of heavy metals in soils of Huzhou[J].Soil,42(4):595-599.
    丁能飞,林义成,杨丽,等,2007.苍南县土壤重金属含量的调查及评价[J].浙江农业科学(4):424-427.DING N F,LIN Y C,YANG L,et al.,2007.Investigation and evaluation of heavy metal content in soil of Cangnan county[J].Journal of Zhejiang Agricultural Science(4):424-427.
    杜艳,常江,徐笠,2010.土壤环境质量评价方法研究进展[J].土壤通报,41(3):749-756.DU Y,CHANG J,XU L,2010.Research progress of soil environmental quality assessment methods[J].Chinese Journal of Soil Science,41(3):749-756.
    高智群,张美剑,赵科理,等,2016.土壤-水稻系统重金属空间异质性研究:以浙江省嵊州市为例[J].中国环境科学,36(1):215-224.GAO Z Q,ZHANG M J,ZHAO K L,et al.,2016.Heavy metal contamination in soil-rice system and its spatial variation in Shengzhou city[J].China Environmental Science,36(1):215-224.
    蒋玉根,戴学龙,张秀英,等,2008.县域尺度土壤重金属含量的空间变异:以富阳市为例[J].浙江农业学报,20(5):339-343.JIANG Y G,DAI X L,ZHANG X Y,et al.,2008.Spatial distribution of heavy metals in arable topsoil at a regional scale of county:A case of Fuyang county,Zhejiang province of China[J].Acta Agriculturae Zhejiangensis,20(5):339-343.
    孔丝纺,刘阳生,曾辉,等,2010.焚烧源挥发性重金属的排放对周边土壤和植被污染的研究进展[J].生态环境学报,19(4):985-990.KONG S F,LIU Y S,ZENG H,et al.,2010.Current progress in research on the pollution of volatile heavy metals from incineration plant to its ambient soil and vegetation[J].Ecology and Environmental Science,19(4):985-990.
    梁巧玲,杨晖,2014.丽水市城郊农田土壤及其蔬菜中Pb与Cd的污染评价[J].贵州农业科学,42(1):140-144.LIANG Q L,YANG H,2014.Pollution evaluation of Pb and Cd in vegetables suburban farmland of Lishui city[J].Guizhou Agricultural Sciences,42(1):140-144.
    李春芳,王菲,曹文涛,等,2017.龙口市污水灌溉区农田重金属来源、空间分布及污染评价[J].环境科学,38(3):1018-1027.LI C F,WANG F,CAO W T,et al.,2017.Source analysis,spatial distribution and pollution assessment of heavy metals in sewage irrigation area farmland soils of Longkou city[J].Environmental Science,38(3):1018-1027.
    林庆让,1986.浙江矿产资源概况[J].中国地质(8):25-27.LIN Q R,1986.General situation of mineral resources in Zhejiang province[J].Chinese Geology(8):25-27.
    刘庆,王静,史衍玺,等,2007.浙江省慈溪市农田土壤重金属污染初步研究[J].农业环境科学学报,26(2):639-644.LIU Q,WANG J,SHI Y X,et al.,2007.Heavy metal pollution in cropland soil in Cixi of Zhejiang province[J].Journal of Agro-Environment Science,26(2):639-644.
    李一蒙,马建华,刘德新,等,2015.开封城市土壤重金属污染及潜在生态风险评价[J].环境科学,36(3):1037-1044.LI Y M,MA J H,LIU D X,et al.,2015.Heavy metal pollution and potential ecological risk assessment of soil in Kaifeng city[J].Environmental Science,36(3):1037-1044.
    罗小玲,郭庆荣,谢志宜,等,2014.珠江三角洲地区典型农村土壤重金属污染现状分析[J].生态环境学报,23(3):485-489.LUO X L,GUO Q R,XIE Z Y,et al.,2014.Study on heavy metal pollution in typical rural soils in Pearl River Delta area[J].Ecology and Environmental Sciences,23(3):485-489.
    吕惠进,2001.浙江省非重金属矿产资源的开发利用政策[J].矿业研究与开发,21(1):9-11.LV H J,2001.Proposals for exploitation of nonmetalic miner resources in Zhejiang province[J].Mining Research and Development,21(1):9-11.
    孙华,毛小军,2008.诸暨浬浦铜矿区土壤重金属空间变异分析[J].农业环境科学学报,27(6):2178-2182.SUN H,MAO X J,2008.Spatial variability analysis of heavy metals in soil of Lipu copper mine,Zhuji[J].Journal of Agro-Environment Science,27(6):2178-2182.
    孙晋伟,黄益宗,石孟春,等,2008.土壤重金属生物毒性研究进展[J].生态学报,28(6):2861-2869.SUN J W,HUANG Y Z,SHI M C,et al.,2008.Advances in studies on biological toxicity of heavy metals in soil[J].Acta Ecological Sinica,28(6):2861-2869.
    王国武,何英才,2000.浙江省矿产资源形势与开发策略[J].科技通报,16(S1):66-71.WANG G W,HE Y C,2000.The situation of mineral resources and tactics of their development in Zhejiang[J].Bulletin of science and technology,16(S1):66-71.
    吴军林,贾文仲,1999.浙江省萤石矿产资源开发利用的对策建议[J].浙江地质,15(2):75-88.WU J L,JIA W Z,1999.Countermeasures and suggestions on the development and utilization of the fluorite resource in Zhejiang province[J].Zhejiang Land and Resource,15(2):75-88.
    吴洋,杨军,周小勇,等,2015.广西都安县耕地土壤重金属污染风险评价[J].环境科学,36(8):2964-2971.WU Y,YANG J,ZHOU X Y,et al.,2015.Risk assessment of heavy metal pollution in cultivated soils in Du'an County of Guangxi province[J].Environmental Science,36(8):2964-2971.
    许金朵,2008.基于GIS的金华市区土壤重金属含量空间分布与污染评价研究[D].南京:南京师范大学:36-39.XU J D,2008.Spatial distribution and pollution assessment of heavy metals in soil of Jinhua city based on GIS[D].Nanjing:Nanjing Normal University:36-39.
    许萌萌,刘爱风,师荣光,等,2018.天津农田重金属污染特征分析及降雨沥浸影响[J].环境科学,39(3):1095-1101.XU M M,LIU A F,SHI R G,et al.,2018.Analysis of heavy metal pollution characteristics and impact of rainfall leaching in Tianjin farmland[J].Environmental Science,39(3):1095-1101.
    尹佳吉,郑喜坤,2015.浙江省土壤重金属污染评价研究[J].世界有色金属(综合),12(11):116-117.YIN J J,ZHENG X K,2015.Research on the evaluation of heavy metal pollution in the soil of Zhejiang province with variable tooth thickness worm[J].World Nonferrous Metal(Comprehensive),12(11):116-117.
    张超兰,李忠义,邓超冰,2009.铅锌矿区农田土壤重金属的统计分析及空间分布研究[J].上海环境科学,28(6):253-257.ZAHNG C L,LI Z Y,DENG C B,2009.Statistical analysis and spatial distribution of heavy metals in farmland soil in lead-zinc mining area[J].Shanghai Environmental Sciences,28(6):253-257.
    张晗,靳青文,黄仁龙,等,2017.大宝山矿区农田土壤重金属污染及其植物累积特征[J].土壤,49(1):141-149.ZHANG H,JIN Q W,HUANG R L,et al.,2017.Heavy metal pollution and plant accumulation characteristics of farmland soil in Dabaoshan mining area[J].Soil,49(1):141-149.
    张君媚,王梦萍,周晓飞,等,2017.庆元县农田土壤环境质量监测与评价[J].农业与技术,37(21):53-54.ZHANG J M,WANG M P,ZHOU X F,et al.,2017.Monitoring and evaluation of farmland soil environmental quality in Qingyuan county[J].Agriculture and Technology,37(21):53-54.
    章明奎,王浩,张慧敏,2008.浙东海积平原农田土壤重金属来源辨识[J].环境科学学报,28(10):1946-1954.ZHANG M K,WANG H,ZHANG H M,2008.Distinguishing different source of heavy metals in soils on the coastal plain of Eastern Zhejiang province[J].Acta Scientiae Circumstantiae,28(10):1946-1954.
    赵科理,傅伟军,叶正钱,等,2016.电子垃圾拆解区土壤重金属空间异质性及分布特征[J].环境科学,37(8):3151-3159.ZHAO K L,FU W J,YE Z Q,et al.,2016.Spatial heterogeneity and distribution characteristics of soil heavy metals in e-waste dismantling area[J].Environmental Science,37(8):3151-3159.
    赵曦,黄艺,李娟,等,2015.大型垃圾焚烧厂周边土壤重金属含量水平、空间分布、来源及潜在生态风险评价[J].生态环境学报,24(6):1013-1021.ZHAO X,HUANG Y,LI J,et al.,2015.Environmental levels,spatial distribution,sources and potential ecological risk of heavy metals in soils surrounding a large soil waste incinerator[J].Ecology and Environmental Sciences,24(6):1013-1021.
    中国环境监测总站,1990.中国土壤元素背景值[M].北京:中国环境科学出版社.CNEMC,1990.The soil background value in China[M].Beijing:China Environmental Science Press.
    周金波,汪峰,楼一鼎,等,2016.宁波市农田土壤重金属污染状况调查[J].浙江农业科学,57(8):1301-1303.ZHOU J B,WANG F,LOU Y D,et al.,2016.Investigation on heavy metal pollution in farmland soil of Ningbo city[J].Zhejiang Agricultural Sciences,57(8):1301-1303.
    周艳,陈樯,邓绍坡,等,2018.西南某铅锌矿区农田土壤重金属空间主成分分析及生态风险评价[J].环境科学,39(6):2884-2892.ZHOU Y,CHEN Q,DENG S P,et al.,2018.Spatial principal component analysis and ecological risk assessment of heavy metals in farmland soil of a lead-zinc mining area in Southwest China[J].Environmental Science,39(6):2884-2892.

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