电化学高级氧化与生化处理的联合工艺研究进展
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摘要
综述近年来电化学高级氧化技术与生化处理联合工艺的研究进展,主要包括生化处理-电化学氧化联合工艺、电化学氧化-生化处理联合工艺以及一体化工艺在实际废水处理中的研究进展,并提出研发多级组合工艺、研制新型电极材料以及控制体系中有毒卤代衍生副产物的生成是未来本领域发展的重点方向。
The recent research progress in combined process of electrochemical advanced oxidation and biochemical treatment is reviewed,including the biochemical treatment-electrochemical oxidation combined process,the electrochemical oxidation-biochemical treatment combined process and the integrated process in the treatment of real wastewater.It is also suggested that the development of multistage combination technology of electrochemical advanced oxidation technology,the development of new electrode materials and the control of the formation of toxic halogenated by-products will be the important directions for future research.
The recent research progress in combined process of electrochemical advanced oxidation and biochemical treatment is reviewed,including the biochemical treatment-electrochemical oxidation combined process,the electrochemical oxidation-biochemical treatment combined process and the integrated process in the treatment of real wastewater.It is also suggested that the development of multistage combination technology of electrochemical advanced oxidation technology,the development of new electrode materials and the control of the formation of toxic halogenated by-products will be the important directions for future research.
引文
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[22] Samet Y,Agengui L,Abdelhédi R.Anodic oxidation of chlorpyrifos in aqueous solution at lead dioxide electrodes[J].Journal of Electroanalytical Chemistry,2010,650(1):152-158.
[23] García-Morales M A,Roa-Morales G,Barrera-Díaz C,et al.Synergy of electrochemical oxidation using boron-doped diamond (BDD) electrodes and ozone (O3) in industrial wastewater treatment[J].Electrochemistry Communications,2013,27(5):34-37.
[24] Duan F,Li Y,Cao H,et al.Activated carbon electrodes:electrochemical oxidation coupled with desalination for wastewater treatment[J].Chemosphere,2015,125:205-211.
[25] Mascia M,Vacca A,Palmas S.Electrochemical treatment as a pre-oxidative step for algae removal using Chlorella vulgaris,as a model organism and BDD anodes[J].Chemical Engineering Journal,2013,219(3):512-519.
[26] Senthilkumar S,Basha C A,Perumalsamy M,et al.Electrochemical oxidation and aerobic biodegradation with isolated bacterial strains for dye wastewater:Combined and integrated approach[J].Electrochimica Acta,2012,77:171-178.
[2] Sánchez-Carretero A,Sáez C,Caáizares P,et al.Electrochemical production of perchlorates using conductive diamond electrolyses[J].Chemical Engineering Journal,2011,166(2):710-714.
[3] Brillas E,Sirés I,Oturan M A.Electro-Fenton process and related electrochemical technologies based on Fenton’s reaction chemistry[J].Chemical Reviews,2009,109(12):6570.
[4] Flox C,Cabot P L,Centellas F,et al.Solar photoelectro-Fenton degradation of cresols using a flow reactor with a boron-doped diamond anode[J].Applied Catalysis B Environmental,2007,75(1):17-28.
[5] Oturan M A,Aaron J J.Advanced oxidation processes in water/wastewater treatment:principles and applications.A review[J].Critical Reviews in Environmental Science & Technology,2014,44(23):2577-2641.
[6] Moreira F C,Soler J,Fonseca A,et al.Incorporation of electrochemical advanced oxidation processes in a multistage treatment system for sanitary landfill leachate[J].Water Research,2015,81(6):375-387.
[7] Radjenovic J,Sedlak D L.Challenges and opportunities for electrochemical processes as next-generation technologies for the treatment of contaminated water[J].Environmental Science & Technology,2015,49(19):11292.
[8] Ihara I,Umetsu K,Kanamura K,et al.Electrochemical oxidation of the effluent from anaerobic digestion of dairy manure[J].Bioresource Technology,2006,97(12):1360-1364.
[9] Urtiaga A,Rueda A,Anglada A,et al.Integrated treatment of landfill leachates including electrooxidation at pilot plant scale[J].Journal of Hazardous Materials,2009,166(2):1530-1534.
[10] Panizza M,Martinez-Huitle C A.Role of electrode materials for the anodic oxidation of a real landfill leachate-comparison between Ti-Ru-Sn ternary oxide,PbO2 and boron-doped diamond anode[J].Chemosphere,2013,90(4):1455-1460.
[11] Feki F,Aloui F,Feki M,et al.Electrochemical oxidation post-treatment of landfill leachates treated with membrane bioreactor[J].Chemosphere,2009,75(2):256-260.
[12] Grafias P,Xekoukoulotakis N P,Mantzavinos D,et al.Pilot treatment of olive pomace leachate by vertical-flow constructed wetland and electrochemical oxidation:An efficient hybrid process[J].Water Research,2010,44(9):2773-2780.
[13] Katsoni A,Mantzavinos D,Diamadopoulos E.Sequential treatment of diluted olive pomace leachate by digestion in a pilot scale UASB reactor and BDD electrochemical oxidation[J].Water Research,2014,57(12):76-86.
[14] Garcia-Segura S,Keller J,Brillas E,et al.Removal of organic contaminants from secondary effluent by anodic oxidation with a boron-doped diamond anode as tertiary treatment[J].Journal of Hazardous Materials,2015,283:551-557.
[15] Urtiaga A M,Pérez G,Ibáňez R,et al.Removal of pharmaceuticals from a WWTP secondary effluent by ultrafiltration/reverse osmosis followed by electrochemical oxidation of the RO concentrate[J].Desalination,2013,331(24):26-34.
[16] Moreira F C,Rui A R B,Brillas E,et al.Electrochemical advanced oxidation processes:A review on their application to synthetic and real wastewaters[J].Applied Catalysis B Environmental,2017,202:217-261.
[17] Zhou M,Liu L,Jiao Y,et al.Treatment of high-salinity reverse osmosis concentrate by electrochemical oxidation on BDD and DSA electrodes[J].Desalination,2011,277(1):201-206.
[18] Bagastyo A Y,Batstone D J,Kristiana I,et al.Electrochemical treatment of reverse osmosis concentrate on boron-doped electrodes in undivided and divided cell configurations[J].Journal of Hazardous Materials,2014,279:111-116.
[19] Radjenovic J,Bagastyo A,Rozendal R A,et al.Electrochemical oxidation of trace organic contaminants in reverse osmosis concentrate using RuO/IrO-coated titanium anodes[J].Water Research,2011,45(4):1579-1586.
[20] Eversloh C L,Henning N,Schulz M,et al.Electrochemical treatment of iopromide under conditions of reverse osmosis concentrates—elucidation of the degradation pathway[J].Water Res,2014,48:237-246.
[21] Song L J,Zhu N W,Yuan H P,et al.Enhancement of waste activated sludge aerobic digestion by electrochemical pre-treatment[J].Water Research,2010,44(15):4371-4378.
[22] Samet Y,Agengui L,Abdelhédi R.Anodic oxidation of chlorpyrifos in aqueous solution at lead dioxide electrodes[J].Journal of Electroanalytical Chemistry,2010,650(1):152-158.
[23] García-Morales M A,Roa-Morales G,Barrera-Díaz C,et al.Synergy of electrochemical oxidation using boron-doped diamond (BDD) electrodes and ozone (O3) in industrial wastewater treatment[J].Electrochemistry Communications,2013,27(5):34-37.
[24] Duan F,Li Y,Cao H,et al.Activated carbon electrodes:electrochemical oxidation coupled with desalination for wastewater treatment[J].Chemosphere,2015,125:205-211.
[25] Mascia M,Vacca A,Palmas S.Electrochemical treatment as a pre-oxidative step for algae removal using Chlorella vulgaris,as a model organism and BDD anodes[J].Chemical Engineering Journal,2013,219(3):512-519.
[26] Senthilkumar S,Basha C A,Perumalsamy M,et al.Electrochemical oxidation and aerobic biodegradation with isolated bacterial strains for dye wastewater:Combined and integrated approach[J].Electrochimica Acta,2012,77:171-178.
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