微波-活性炭处理有机废水的研究进展
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摘要
微波-活性炭技术具有选择性强、升温快、效率高、时间短、易于自动控制等特点,在有机废水处理领域应用广泛.其机理主要是"热点"理论和"羟基自由基"理论.本文主要综述了近十年来微波-活性炭处理含酚废水、焦化废水,制药废水、染料废水和其他有机废水的研究现状,并对微波-活性炭技术进行了展望.
Microwave-activated carbon hybrid technology has the characteristics such as strong selectivity,heating rapidly,high efficiency,short time,easy automatic control and so on. It is widely used in the field of organic wastewater treatment. The mechanism of microwave-activated carbon treatment of wastewater is mainly "hots pot effect‘theory and ' hydroxyl radical " theory. In this review,we summarize the recent 10 years of microwave and activated carbon treatment of Phenolic Effluent,coking wastewater,pharmaceutical wastewater,dye wastewater and other organic wastewater research status. Moreover,brief insight into the related microwave activated carbon technology is presented.
Microwave-activated carbon hybrid technology has the characteristics such as strong selectivity,heating rapidly,high efficiency,short time,easy automatic control and so on. It is widely used in the field of organic wastewater treatment. The mechanism of microwave-activated carbon treatment of wastewater is mainly "hots pot effect‘theory and ' hydroxyl radical " theory. In this review,we summarize the recent 10 years of microwave and activated carbon treatment of Phenolic Effluent,coking wastewater,pharmaceutical wastewater,dye wastewater and other organic wastewater research status. Moreover,brief insight into the related microwave activated carbon technology is presented.
引文
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[2]敬璇，李正山．高浓度有机废水处理技术研究进展[J]．成都大学学报(自然科学版)，2012,31(1):85-89.JING X,LI Z S. Research progress of high concentration organic wastewater treatment techniques[J]. Journal of Chengdu University(Natural Science),2012,31(1):85-89.
[3]李雨，张世敏，彭金辉，等．微波-活性炭催化降解有机废水的研究现状和发展趋势[J]．环境科学导刊，2008,27(4):59-62.LI Y. ZHANG S M,PENG J H,et al. Research review and development trend of degrading organic wastewater by microwave heating with activated carbon catalysi[J].Environmental Science Survey,2008,27(4):59-62.
[4]彭金辉，张利波，张世敏，等．综合利用烟杆废料制取优质活性炭[J]．林产化学与工业，2002,22(3):85-87.PENG J H. ZHANG L B,ZHANG S M. et al. Preparation of activated carbon from tobacco stems[J]. Chemistry And Industry of Forest Products,2002,22(3):85-87.
[5]张耀斌．微波辅助湿式空气氧化水中难降解有机物的研究[D]．大连:大连理工大学，2005:2-5ZHANG Y B. Study on microwave assisted wet air oxidation of biorefractory organic contaminant in water[D]. Dalian:Dalian University of Technology,2005:2-5
[6] QUAN X,ZHANG Y,CHEN S,et al. Generation of hydroxyl radical in aqueous solution by microwave energy using activated carbon as catalyst and its potential in removal of persistent organic substances[J]. Journal of Molecular Catalysis A Chemical,2007,263(1):216-220.
[7]姜南，孙德栋，潘婕妤，等．微波辅助活性炭催化硫酸根自由基处理苯酚废水[J]．大连工业大学学报，2016(3):199-202.JIANG N,SUN D D,PAN J Y,et al. Degradation of phenol wastewater by microwave-activated carbon in catalyzing sulfate radical[J]. Journal of Dalian Polytechnic University,2016(3):199-202.
[8]丁涛．微波协同活性炭和H2O2处理苯酚废水的研究[J]．广州化工，2014(19):61-63.DING T. Study on synergetic degradation of phenol by microwave active carbon and H2O2[J]. Guangzhou Chemical Industry,2014(19):61-63.
[9]刘龙，赵浩，徐炎华．微波-H2O2-活性炭协同催化氧化处理苯酚废水[J]．南京工业大学学报(自然科学版)，2010,32(1):46-49.LIU L, ZHAO H, XU Y H. Synergetic oxidation of microwave and H2O2-activated carbon on phenol wastewater[J]. Journal of Nanjing University of Technology(Natural science edition),2010,32(1):46-49.
[10]吴慧英，陈积义，施周，等．微波辐射/活性炭工艺处理高浓度苯酚废水研究[J]．湖南大学学报:自然科学版，2008,35(2):89-92.WU H Y, CHEN J Y, SHI Z, et al. Microwave irradiation/activated carbon process to treat highconcentration phenolic wastewater[J]. Journal of Hunan University(Natural Sciences),2008,35(2):89-92.
[11]高鹏，徐璐，辛宁，等．焦化废水污染控制技术研究进展[J]．环境工程技术学报，2016,6(4):357-362.GAO P,XU L,XIN N,et al. Advances in research on coking wastewater control technologies[J]. Journal of Environmental Engineering Technology,2016,6(4):357-362.
[12]高玉，孙宝铁，高秀丽，等．微波-活性炭联合处理焦化废水的应用前景[J]．环境与可持续发展，2017,42(4):120-124.GAO Y, SUN B L, GAO X L, et al. Treatment of hydroquinone wastewater by manganese modified microelectrolysis proces[J]. Environment and Sustainable Development,2017,42(4):120-124.
[13]李雨，彭金辉，雷鹰，等．微波-活性炭法处理焦化废水生化后出水实验研究[C]．全国冶金物理化学学术会议专辑，贵阳，2010.LI Y,PENG J H,LEI Y,et al. Experimental research on coking wastewater biochemical treatment with microwaveactivated carbon process[C]. Album of National Symposium on Metallurgical Physical Chemistry(Volume2),Guiyang,2010.
[14]林莉，陆晓华，李青云，等．微波-活性炭联用对焦化废水中氨氮和COD的同时去除研究[J]．长江科学院院报，2011,28(11):19-21.LIN L,LU X H,LI Q Y,et al. Combined effect of microwave and activated carbon on the removal of ammonia nitrogen and cod in coking wastewater[J].Journal of Yangtze River Scientific Research Institute,2011,28(11):19-21.
[15]李向东，冯启言，于洪锋．气浮-水解-好氧工艺处理制药废水[J]．环境工程，2005,23(3):17-18.LI X D, FENG Q Y, YU H F. Treatment of pharmaceutical wastewater by air flotation-hydrolysisaerobic process[J]. Environmental Engineering,2005,23(3):17-18.
[16]赵庆良，蔡萌萌，刘志刚，等．气浮-活性污泥工艺处理制药废水[J]．中国给水排水，2006,22(1):77-79.ZHAO Q L,CAI M M,LIU Z G,et al. Pharmaceutical wastewater treatment with daf-activated sludge processes[J]. China Water&Wastewater,2006,22(1):77-79.
[17]高畅宇，姚日生，王淮，等．活性炭吸附微波辐射噁草酮生产废水的研究[J]．化工进展，2012(s1):470-473.GAO C Y,YAO R S,WNAG W,et al. Treatment of oxadiazon wastewater by activated carbon adsorptionmicrowave radiation xiidation process[J]. Chemical Industry and Engineering Progress,2012(s1):470-473.
[18]李亚峰，高颖，王景新．微波强化Fenton/活性炭工艺处理制药废水的影响因素[J]．环境工程学报，2014,8(6):17-21.LI Y F,GAO Y,WANG J X. Influencing factors of microwave enhanced Fenton/active carbon process for pharmaceutical wastewater[J]. Chinese Journal of Environmental Engineering,2014,8(6):17-21.
[19]刘畅．微波协同活性炭处理盐酸黄连素废水最佳降解条件的研究[J]．绿色科技，2016,25(2):73-75.LIU C. Study on the optimum degradation conditions of berberine hydrochloride wastewater treated by microwave and activated carbon[J]. Journal of Green Science and Technology,2016,25(2):73-75.
[20]杨占红．不同方法深度处理印染废水的比较研究[J]．工业水处理，2010,30(7):42-45.YANG Z H. Research on the comparison of different methods for the advanced treatment of printing and dyeing wastewater[J]. Industrial Water Treatment, 2010,30(7):42-45.
[21]龚兵丽，邱宇平，赵雅萍，等．黑碳吸附亚甲基蓝染料废水的行为研究[J]．环境科学与技术，2009,32(11):18-23.GONG L B,QUE Y P,ZHAO Y P,et al. Laboratory study on adsorption of methylene blue on black carbon in aqueous solution[J]. Environmental Science&Technology,2009,32(11):18-23.
[22]李江，张翠红，陈志敏．微波辐照活性炭法处理罗丹明B废水的研究[J]．安徽化工，2018,44(4):91-95.LI J,ZHANG C H,CHEN Z M. Study on treatment of Rhodamine B wastewater by microwave radiation-activated carbon[J]. Anhui Chemical Industry,2018,44(4):91-95.
[23]彭丽．微波活性炭法处理酸性红88废水及其机理[J]．环境工程学报，2016(12):75-80.PEN G L. Treatment of acid red 88 wastewater by microwave irradiation method with activated carbon technology[J]. Chinese Journal of Environmental Engineering,2016(12):75-80.
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