How anthropogenic activities affect soil heavy metal concentration on a broad scale: a geochemistry survey in Yangtze River Delta, Eastern China

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• 作者：Jianguo Li (1)
  Lijie Pu (1) (2)
  Qilin Liao (3)
  Ming Zhu (1)
  Xiaoqing Dai (1)
  Yan Xu (1)
  Lifang Zhang (4)
  Ming Hua (3)
  Yang Jin (3)
  
  1. School of Geographic and Oceanographic Sciences ; Nanjing University ; No. 163 Xianlin Road ; Qixia District ; 210023 ; Nanjing ; Jiangsu Province ; People鈥檚 Republic of China
  2. The Key Laboratory of the Coastal Zone Exploitation and Protection ; Ministry of Land and Resources ; Nanjing ; 210023 ; China
  3. Geological Survey of Jiangsu Province ; Nanjing ; 210018 ; China
  4. School of Public Administration ; Nanjing University of Finance and Economics ; Nanjing ; 210046 ; China
  
• 关键词：Soil heavy metal concentration ; Land use ; Enrichment factor ; Yangtze River Delta
• 刊名：Environmental Earth Sciences
• 出版年：2015
• 出版时间：February 2015
• 年：2015
• 卷：73
• 期：4
• 页码：1823-1835
• 全文大小：2,311 KB
• 参考文献：1. Aoyama M, Kuroyanagi S (1996) Effects of heavy metal accumulation associated with pesticide application on the decomposition of cellulose and orchard grass in soils. Soil Sci Plant Nutr 42(1):121鈥?31 CrossRef
  2. Atafar Z, Mesdaghinia A, Nouri J, Homaee M, Yunesian M, Ahmadimoghaddam M, Mahvi AH (2010) Effect of fertilizer application on soil heavy metal concentration. Environ Monit Assess 160:83鈥?9 CrossRef
  3. Atiemo SM, Ofosu FG, Aboh IJK, Oppon OC (2012) Levels and sources of heavy metal contamination in road dust in selected major highways of Accra, Ghana. X Ray Spectrom 41(2):105鈥?10 CrossRef
  4. Bai J, Xiao R, Cui B, Zhang K, Wang Q, Liu X, Gao H, Huang L (2011) Assessment of heavy metal pollution in wetland soils from the young and old reclaimed regions in the Pearl River Estuary, South China. Environ Pollut 159(3):817鈥?24 CrossRef
  5. Basta N, Pantone D, Tabatabai M (1993) Path analysis of heavy metal adsorption by soil. Agron J 85(5):1054鈥?057 CrossRef
  6. Bremner J, Mulvaney C (1982) Nitrogen鈥攖otal. In: Page A (ed) Methods of soil analysis, part 2. Chemical and microbiological properties, American Society of Agronomy, Soil Science Society of America, pp 595鈥?24
  7. Buat-Menard P, Chesselet R (1979) Variable influence of the atmospheric flux on the trace metal chemistry of oceanic suspended matter. Earth Planet Sc Lett 42(3):399鈥?11 CrossRef
  8. Caeiro S, Costa MH, Ramos TB, Fernandes F, Silveira N, Coimbra A, Medeiros G, Painho M (2005) Assessing heavy metal contamination in Sado Estuary sediment: an index analysis approach. Ecol Indic 5(2):151鈥?69 CrossRef
  9. Chen TB, Zheng YM, Lei M, Huang ZC, Wu HT, Chen H, Fan KK, Yu K, Wu X, Tian QZ (2005) Assessment of heavy metal pollution in surface soils of urban parks in Beijing, China. Chemosphere 60(4):542鈥?51 CrossRef
  10. Cheng S (2003) Heavy metal pollution in China: origin, pattern and control. Environ Sci Pollut R 10(3):192鈥?98 CrossRef
  11. Chrastn媒 V, Van臎k A, Teper L, Cabala J, Proch谩zka J, Pechar L, Drahota P, Pen铆啪ek V, Kom谩rek M, Nov谩k M (2012) Geochemical position of Pb, Zn and Cd in soils near the Olkusz mine/smelter, South Poland: effects of land use, type of contamination and distance from pollution source. Environ Monit Assess 184(4):2517鈥?536 CrossRef
  12. Covelli S, Langone L, Acquavita A, Piani R, Emili A (2012) Historical flux of mercury associated with mining and industrial sources in the Marano and Grado Lagoon (northern Adriatic Sea). Estuar Coast Shelf Sci 113:7鈥?9 CrossRef
  13. Delgado A, Torrent J (2000) Phosphorus forms and desorption patterns in heavily fertilized calcareous and limed acid soils. Soil Sci Soc Am J 64(6):2031鈥?037 CrossRef
  14. Du Laing G, Rinklebe J, Vandecasteele B, Meers E, Tack FMG (2009) Trace metal behaviour in estuarine and riverine floodplain soils and sediments: a review. Sci Total Environ 407(13):3972鈥?985 CrossRef
  15. Finney BP, Huh CA (1989) History of metal pollution in the Southern California Bight: an update. Environ Sci Technol 23(3):294鈥?03 CrossRef
  16. Garnaud S, Mouchel JM, Chebbo G, Thevenot DR (1999) Heavy metal concentrations in dry and wet atmospheric deposits in Paris district: comparison with urban runoff. Sci Total Environ 235(1鈥?):235鈥?45 CrossRef
  17. Guan DS, Chen YI, Ruan GB (2001) Study on heavy metal concentrations and the impact of human activity on them in urban and suburb soils of Guangzhou. Acta Scientiarum Naturalium Universitatis Sunyatseni 40(4):93鈥?01 (in Chinese)
  18. Hang X, Wang H, Zhou J, Ma C, Du C, Chen X (2009) Risk assessment of potentially toxic element pollution in soils and rice ( / Oryza sativa) in a typical area of the Yangtze River Delta. Environ Pollut 157(8):2542鈥?549 CrossRef
  19. Hettiarachchi GM, Pierzynski GM, Ransom MD (2001) In situ stabilization of soil lead using phosphorus. J Environ Qual 30(4):1214鈥?221 CrossRef
  20. Huang B, Kuo S, Bembenek R (2004) Availability of cadmium in some phosphorus fertilizers to field-grown lettuce. Water Air Soil Poll 158(1):37鈥?1 CrossRef
  21. Huang SS, Liao QL, Hua M, Wu XM, Bi KS, Yan CY, Chen B, Zhang XY (2007) Survey of heavy metal pollution and assessment of agricultural soil in Yangzhong district, Jiangsu Province, China. Chemosphere 67(11):2148鈥?155 CrossRef
  22. Jackson ML (1958) Soil chemical analysis. Englewood Cliffs Press, New Jersey
  23. Kelly J, Thornton I, Simpson P (1996) Urban geochemistry: a study of the influence of anthropogenic activity on the heavy metal content of soils in traditionally industrial and non-industrial areas of Britain. Appl Geochem 11(1):363鈥?70 CrossRef
  24. Kumar Sharma R, Agrawal M, Marshall F (2007) Heavy metal contamination of soil and vegetables in suburban areas of Varanasi, India. Ecotox Environ Safe 66(2):258鈥?66 CrossRef
  25. Kumpiene J, Lagerkvist A, Maurice C (2008) Stabilization of As, Cr, Cu, Pb and Zn in soil using amendments鈥揳 review. Waste Manag 28(1):215鈥?25 CrossRef
  26. Li XD, Poon CS, Liu PS (2001) Heavy metal contamination of urban soils and street dusts in Hong Kong. Appl Geochem 16(11鈥?2):1361鈥?368 CrossRef
  27. Li QS, Wu ZF, Chu B, Zhang N, Cai SS, Fang JH (2007) Heavy metals in coastal wetland sediments of the Pearl River Estuary, China. Environ Pollut 149(2):158鈥?64 CrossRef
  28. Li XY, Chen TB, Lei M, Xie YF (2010) Concentrations and risk of heavy metals in surface soil and dust in urban squares and school campus in Beijing. Geogr Res 29(6):989鈥?96 (in Chinese)
  29. Li XZ, Sun YG, Mander U, He YL (2013) Effects of land use intensity on soil nutrient distribution after reclamation in an estuary landscape. Landsc Ecol 28(4):699鈥?07 CrossRef
  30. Li JG, Pu LJ, Zhu M, Liao QL, Wang HY, Cai FF (2014a) Spatial pattern of heavy metal concentration in the soil of rapid urbanization area: a case of Ehu Town, Wuxi City, Eastern China. Environ Earth Sci 71:3355鈥?362 CrossRef
  31. Li JG, Pu LJ, Liao QL, Zhu M, Liu LL, Zhang LF, Wang QQ, Dai XQ (2014b) The sources and gradient effect of soil heavy metal concentrations in Wuxi City. Scientia Geographica Sinica 34(4):496鈥?04 (in Chinese)
  32. Liaghati T, Preda M, Cox M (2004) Heavy metal distribution and controlling factors within coastal plain sediments, Bells Creek catchment, southeast Queensland, Australia. Environ Int 29(7):935鈥?48 CrossRef
  33. Liu JY, Zhuang DF, Zhang ZX, Gao ZQ, Deng XZ (2002) The establishment of land-use spatial鈥搕emporal database and its relative studies in China. Geo-inf Sci 4(3):3鈥? (in Chinese)
  34. Liu JY, Chang XY, Tu XL, Chen YH, Chen N, Fu SM (2008) Application of enrichment index method to evaluation of thallium contamination of soils around a slag dump of a sulphuric acid plant. Soils 40(6):939鈥?44 (in Chinese)
  35. Liu E, Birch GF, Shen J, Yuan H, Zhang E, Cao Y (2012) Comprehensive evaluation of heavy metal contamination in surface and core sediments of Taihu Lake, the third largest freshwater lake in China. Environ Earth Sci 67(1):39鈥?1 CrossRef
  36. MAC (Ministry of Agriculture of China) (2006) Chinese agricultural testing standard, (NY/T 1121.5-2006; NY/T 1121.6-2006)
  37. Nan ZR, Zhao CY, Li JJ, Chen FH, Sun W (2002) Relations between soil properties and selected heavy metal concentrations in spring wheat ( / Triticum aestivum L.) grown in contaminated soils. Water Air Soil Poll 133(1鈥?):205鈥?13 CrossRef
  38. Nicholson FA, Chambers BJ, Williams JR, Unwin RJ (1999) Heavy metal contents of livestock feeds and animal manures in England and Wales. Bioresour Technol 70(1):23鈥?1 CrossRef
  39. Pekey H, Karaka艧 D, Ayberk S, Tolun L, Bako臒lu M (2004) Ecological risk assessment using trace elements from surface sediments of Izmit Bay (Northeastern Marmara Sea) Turkey. Mar Pollut Bull 48(9):946鈥?53 CrossRef
  40. SEPAC (State Environmental Protection Administration of China). (1995). Chinese environmental qualitye standard for soils(GB15618-1995)
  41. Sinex SA, Wright DA (1988) Distribution of trace metals in the sediments and biota of Chesapeake Bay. Mar Pollut Bull 19(9):425鈥?31 CrossRef
  42. Sowana A, Shrestha RP, Parkpian P, Pongquan S (2011) Influence of coastal land use on soil heavy-metal contamination in Pattani Bay, Thailand. J Coastal Res 27(2):252鈥?62 CrossRef
  43. Sun Y, Zhou Q, Xie X, Liu R (2010) Spatial, sources and risk assessment of heavy metal contamination of urban soils in typical regions of Shenyang, China. J Hazard Mater 174(1):455鈥?62 CrossRef
  44. Sutherland R (2000) Bed sediment-associated trace metals in an urban stream, Oahu, Hawaii. Environ Geol 39(6):611鈥?27 CrossRef
  45. Tan J, Kang Y (2009) Changes in soil properties under the influences of cropping and drip irrigation during the reclamation of severe salt-affected soils. Agric Sci Chin 8(10):1228鈥?237 CrossRef
  46. Taylor SR, McLennan SM (1995) The geochemical evolution of the continental crust. Rev Geophys 33(2):241鈥?65 CrossRef
  47. Tomlinson D, Wilson J, Harris C, Jeffrey D (1980) Problems in the assessment of heavy-metal levels in estuaries and the formation of a pollution index. Helgol盲nder Meeresuntersuchungen 33(1鈥?):566鈥?75 CrossRef
  48. Wang F, Chen Z, Sun Y, Gao Y, Yu J (2006) Investigation on the pollution of organoarsenical additives to animal feed in the surroundings and farmland near hog farms. Acta Ecol Sinica 26(1):154鈥?62 (in Chinese)
  49. Wang M, Markert B, Chen W, Peng C, Ouyang Z (2012) Identification of heavy metal pollutants using multivariate analysis and effects of land uses on their accumulation in urban soils in Beijing, China. Environ Monit Assess 184(10):5889鈥?897 CrossRef
  50. Wei B, Yang L (2010) A review of heavy metal contaminations in urban soils, urban road dusts and agricultural soils from China. Microchem J 94(2):99鈥?07 CrossRef
  51. Windom HL, Schropp SJ, Calder FD, Ryan JD, Smith RG Jr, Burney LC, Lewis FG, Rawlinson CH (1989) Natural trace metal concentrations in estuarine and coastal marine sediments of the southeastern United States. Environ Sci Technol 23(3):314鈥?20 CrossRef
  52. Yuan H, Shen J, Liu E, Wang J, Meng X (2011) Assessment of nutrients and heavy metals enrichment in surface sediments from Taihu Lake, a eutrophic shallow lake in China. Environ Geochem Hlth 33(1):67鈥?1 CrossRef
  53. Zhang H, Wang Z, Zhang Y, Hu Z (2012) The effects of the Qinghai鈥揟ibet railway on heavy metals enrichment in soils. Sci Total Environ 439:240鈥?48 CrossRef
  54. Zhao Y, Shi X, Huang B, Yu D, Wang H, Sun W, 脰boern I, Blomb盲ck K (2007) Spatial distribution of heavy metals in agricultural soils of an industry-based peri-urban area in Wuxi, China. Pedosphere 17(1):44鈥?1 CrossRef
  55. Zhou J, Ma D, Pan J, Nie W, Wu K (2008) Application of multivariate statistical approach to identify heavy metal sources in sediment and waters: a case study in Yangzhong. China Environ Geol 54(2):373鈥?80 CrossRef
  56. Zhu Y, Johnson TA, Su J, Qiao M, Guo G-X, Stedtfeld RD, Hashsham SA, Tiedje JM (2013) Diverse and abundant antibiotic resistance genes in Chinese swine farms. Proc Natl Acad Sci 110(9):3435鈥?440 CrossRef
  
• 刊物类别：Earth and Environmental Science
• 刊物主题：None Assigned
• 出版者：Springer Berlin Heidelberg
• ISSN：1866-6299

文摘

Heavy metal pollution in soil is a growing concern, and little is known about how it is distributed in the soils of different districts with different land uses on a broad scale. A total of 873 surface soil samples (0- to 20-cm depth) were collected in the Huishan and Xin districts of Wuxi City. The pollution levels and sources of heavy metals in the two districts were identified using multivariate statistics and spatial analysis methods, and the results are discussed in this paper. The concentration of heavy metals in soils, particularly Hg, was higher in Xin, where there are many industrial parks. The concentrations of As, Cu, Hg, Pb, and Zn were higher than the corresponding background values in the two districts, and the soil Hg in Xin exceeded the grade II threshold value of the Chinese Environmental Quality Standard for Soils. Natural resources (e.g., geogenic and pedogenic factors) were predominately responsible for the heavy metal concentration in Huishan soils, but anthropogenic activities (industrial production and discharge) were the primary factors for soil heavy metal pollution in Xin. The soil heavy metal concentration in forestlands was high in Huishan, and among these metals Hg and As reached a moderate level of pollution [enrichment factor (EF) >2]. No pollution or minimal pollution happened in response to other land uses. In Xin, the Hg in cultivated land, rural-residential land, and underwater sediments reached a moderate level of pollution (EF >2), and the other heavy metal levels were low (EF