纳米零价铁改性技术及其在污染修复中的应用研究进展
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摘要
综述了改性纳米零价铁对卤代有机物、硝酸盐、重金属及染料等环境中广泛存在的污染物的去除机理,并对未来的应用方向进行了展望。
This review summarizes the mechanism for modified nano-zero-valent iron to remove pollutants widely existed in the environment,such as halogenated organic compounds,nitrates,heavy metals,dyes. What's more,its future application directions are forecasted.
This review summarizes the mechanism for modified nano-zero-valent iron to remove pollutants widely existed in the environment,such as halogenated organic compounds,nitrates,heavy metals,dyes. What's more,its future application directions are forecasted.
引文
[1]Lu J,Kai X,Yang J,et al.Nano iron oxide impregnated in chitosan bead as a highly efficient sorbent for Cr(Ⅵ)removal from water[J].Carbohydrate Polymers,2017,173:28-36.
[2]高园园,周启星.纳米零价铁在污染土壤修复中的应用与展望[J].农业环境科学学报,2013,32(3):418-425.
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[4]Xue W,Huang D,Zeng G,et al.Nanoscale zero-valent iron coated with rhamnolipid as an effective stabilizer for immobilization of Cd and Pb in river sediments[J]. Journal of Hazardous Materials,2017:S0304389417304491.
[5]刘宏芳,钱天伟,赵东叶.利用稳定的零价纳米铁粒子悬浮液还原固定土壤和地下水中的Re O4-[J].科学通报,2013,(11):972-977.
[6]Li X,Ai L,Jing J.Nanoscale zerovalent iron decorated on graphene nanosheets for Cr(Ⅵ)removal from aqueous solution:Surface corrosion retard induced the enhanced performance[J]. Chemical Engineering Journal,2016,288:789-797.
[7]Sun Z,Zheng S,Ayoko G A,et al. Degradation of simazine from aqueous solutions by diatomite-supported nanosized zero-valent iron composite materials[J]. Journal of Hazardous Materials,2013,263(2):768-777.
[8]Shi L N,Zhang X,Chen Z L. Removal of chromium(Ⅵ)from wastewater using bentonite-supported nanoscale zero-valent iron[J].Water Research,2011,45(2):0-892.
[9]Fu R,Yang Y,Xu Z,et al.The removal of chromium(Ⅵ)and lead(Ⅱ)from groundwater using sepiolite-supported nanoscale zerovalent iron(S-NZVI)[J].Chemosphere,2015,138:726-734.
[10]Rui W,Ting T,Kaibo H,et al.Debromination of polybrominated biphenyls(PBBs)by zero valent metals and iron-based bimetallic particles:Mechanisms,pathways and predicting descriptor[J].Chemical Engineering Journal,2018,351:773-781.
[11]Fang Z,Qiu X,Chen J,et al.Degradation of the polybrominated diphenyl ethers by nanoscale zero-valent metallic particles prepared from steel pickling waste liquor[J]. Desalination,2011,267(1):34-41.
[12]韩文亮,陈海明,陈兴童.改性零价铁降解多溴二苯醚的研究进展[J].环境化学,2017,36(7):1474-1483.
[13]Zhou H,Han J,Baig S A,et al.Dechlorination of 2,4-dichlorophenoxyacetic acid by sodium carboxymethyl cellulose-stabilized Pd/Fe nanoparticles[J]. Journal of Hazardous Materials,2011,198(2):7-12.
[14]周红艺,曾思思,梁思,等.还原脱氯-生物联合降解2,4-二氯苯氧乙酸[J].环境科学,2014,35(9):3430-3435.
[15]Tso C P,Shih Y H.The transformation of hexabromocyclododecane using zerovalent iron nanoparticle aggregates[J].Journal of Hazardous Materials,2014,277:76-83.
[16]Ardekani J G,Hassani Z.Study of the environmental impacts of nitrate pollution and its removal by nanoscale zero-valent iron(NZVI)at the south of Shahre-Kord aquifer(Chaharmahal and Bakhtiari province,Iran)[J]. Arabian Journal of Geosciences,2018,11:708.
[17]Su Y,Adeleye A,Huang Y,et al.Simultaneous removal of cadmium and nitrate in aqueous media by nanoscale zerovalent iron(nZVI)and Au doped nZVI particles[J].Water Research,2014,63(Complete):102-111.
[18]刘桂梅,郭兵毅,曾玉彬.磁性石墨烯负载纳米Fe/Cu去除水中硝酸盐氮[J].水处理技术,2017,43(2):58-62.
[19]董磊,林莉,李青云,等.改性凹凸棒土/纳米铁复合材料与微生物耦合去除地下水硝酸盐氮的研究[J].环境科学研究,2017,30(7):1112-1119.
[20]陈西亮,刘国,高阳阳,等.零价纳米铁炭微电解体系去除水中硝酸盐[J].环境化学,2016,35(8):1670-1675.
[21]Krasae N,Wantala K.Enhanced nitrogen selectivity for nitrate reduction on Cu-nZVI by Ti O2,photocatalysts under UV irradiation[J].Applied Surface Science,2016,380:309-317.
[22]Wang L,Zhou H,Liu J,et al.Effect of humic acid on the nitrate removal by strong base anion exchanger supported nanoscale zerovalent iron composite[J]. Water,Air,&Soil Pollution,2018,229(11):357-366.
[23]Ezzatahmadi Naeim,Ayoko Godwin A Millar,Graeme J,et al.Claysupported nanoscale zero-valent iron composite materials for the remediation of contaminated aqueous solutions:A review[J].Chemical Engineering Journal,2017,312:336-350.
[24]秦泽敏,董黎明,赖花,等.硅酸钙负载零价纳米铁吸附去除水中六价铬[J].硅酸盐通报,2015,34(8):2376-2381.
[25]Ali S W,Mirza M L,Bhatti T M. Removal of Cr(Ⅵ)using iron nanoparticles supported on porous cation-exchange resin[J].Hydrometallurgy,2015,157:82-89.
[26]Joseph N Fiedor,William D Bostick,Robert J Jarabek,et al.Understanding the mechanism of uranium removal from groundwater by zero-valent iron using X-ray photoelectron spectroscopy[J]. Environmental Science&Technology,2015,32(10):1466-1473.
[27]Dutta S,Saha R,Kalita H,et al.Rapid reductive degradation of azo and anthraquinone dyes by nanoscale zero-valent iron[J].Environmental Technology&Innovation,2016,5:176-187.
[28]金晓英,陈征贤,郭飞鹏,等.超声波辅助壳聚糖/零价纳米铁降解酸性品红[J].环境科学学报,2013,33(4):1004-1009.
[29]鲍倩倩,李锦祥,关小红.预磁化强化零价铁除偶氮染料的性能研究[J].环境化学,2017,36(7):1467-1473.
[2]高园园,周启星.纳米零价铁在污染土壤修复中的应用与展望[J].农业环境科学学报,2013,32(3):418-425.
[3]Xie Y Y,Cheng W,Tsang P E,et al.Remediation and phytotoxicity of decabromodiphenyl ether contaminated soil by zero valent iron nanoparticles immobilized in mesopoeous silicamicrospheres[J].Journal of Environmental Management,2016,166:478-483.
[4]Xue W,Huang D,Zeng G,et al.Nanoscale zero-valent iron coated with rhamnolipid as an effective stabilizer for immobilization of Cd and Pb in river sediments[J]. Journal of Hazardous Materials,2017:S0304389417304491.
[5]刘宏芳,钱天伟,赵东叶.利用稳定的零价纳米铁粒子悬浮液还原固定土壤和地下水中的Re O4-[J].科学通报,2013,(11):972-977.
[6]Li X,Ai L,Jing J.Nanoscale zerovalent iron decorated on graphene nanosheets for Cr(Ⅵ)removal from aqueous solution:Surface corrosion retard induced the enhanced performance[J]. Chemical Engineering Journal,2016,288:789-797.
[7]Sun Z,Zheng S,Ayoko G A,et al. Degradation of simazine from aqueous solutions by diatomite-supported nanosized zero-valent iron composite materials[J]. Journal of Hazardous Materials,2013,263(2):768-777.
[8]Shi L N,Zhang X,Chen Z L. Removal of chromium(Ⅵ)from wastewater using bentonite-supported nanoscale zero-valent iron[J].Water Research,2011,45(2):0-892.
[9]Fu R,Yang Y,Xu Z,et al.The removal of chromium(Ⅵ)and lead(Ⅱ)from groundwater using sepiolite-supported nanoscale zerovalent iron(S-NZVI)[J].Chemosphere,2015,138:726-734.
[10]Rui W,Ting T,Kaibo H,et al.Debromination of polybrominated biphenyls(PBBs)by zero valent metals and iron-based bimetallic particles:Mechanisms,pathways and predicting descriptor[J].Chemical Engineering Journal,2018,351:773-781.
[11]Fang Z,Qiu X,Chen J,et al.Degradation of the polybrominated diphenyl ethers by nanoscale zero-valent metallic particles prepared from steel pickling waste liquor[J]. Desalination,2011,267(1):34-41.
[12]韩文亮,陈海明,陈兴童.改性零价铁降解多溴二苯醚的研究进展[J].环境化学,2017,36(7):1474-1483.
[13]Zhou H,Han J,Baig S A,et al.Dechlorination of 2,4-dichlorophenoxyacetic acid by sodium carboxymethyl cellulose-stabilized Pd/Fe nanoparticles[J]. Journal of Hazardous Materials,2011,198(2):7-12.
[14]周红艺,曾思思,梁思,等.还原脱氯-生物联合降解2,4-二氯苯氧乙酸[J].环境科学,2014,35(9):3430-3435.
[15]Tso C P,Shih Y H.The transformation of hexabromocyclododecane using zerovalent iron nanoparticle aggregates[J].Journal of Hazardous Materials,2014,277:76-83.
[16]Ardekani J G,Hassani Z.Study of the environmental impacts of nitrate pollution and its removal by nanoscale zero-valent iron(NZVI)at the south of Shahre-Kord aquifer(Chaharmahal and Bakhtiari province,Iran)[J]. Arabian Journal of Geosciences,2018,11:708.
[17]Su Y,Adeleye A,Huang Y,et al.Simultaneous removal of cadmium and nitrate in aqueous media by nanoscale zerovalent iron(nZVI)and Au doped nZVI particles[J].Water Research,2014,63(Complete):102-111.
[18]刘桂梅,郭兵毅,曾玉彬.磁性石墨烯负载纳米Fe/Cu去除水中硝酸盐氮[J].水处理技术,2017,43(2):58-62.
[19]董磊,林莉,李青云,等.改性凹凸棒土/纳米铁复合材料与微生物耦合去除地下水硝酸盐氮的研究[J].环境科学研究,2017,30(7):1112-1119.
[20]陈西亮,刘国,高阳阳,等.零价纳米铁炭微电解体系去除水中硝酸盐[J].环境化学,2016,35(8):1670-1675.
[21]Krasae N,Wantala K.Enhanced nitrogen selectivity for nitrate reduction on Cu-nZVI by Ti O2,photocatalysts under UV irradiation[J].Applied Surface Science,2016,380:309-317.
[22]Wang L,Zhou H,Liu J,et al.Effect of humic acid on the nitrate removal by strong base anion exchanger supported nanoscale zerovalent iron composite[J]. Water,Air,&Soil Pollution,2018,229(11):357-366.
[23]Ezzatahmadi Naeim,Ayoko Godwin A Millar,Graeme J,et al.Claysupported nanoscale zero-valent iron composite materials for the remediation of contaminated aqueous solutions:A review[J].Chemical Engineering Journal,2017,312:336-350.
[24]秦泽敏,董黎明,赖花,等.硅酸钙负载零价纳米铁吸附去除水中六价铬[J].硅酸盐通报,2015,34(8):2376-2381.
[25]Ali S W,Mirza M L,Bhatti T M. Removal of Cr(Ⅵ)using iron nanoparticles supported on porous cation-exchange resin[J].Hydrometallurgy,2015,157:82-89.
[26]Joseph N Fiedor,William D Bostick,Robert J Jarabek,et al.Understanding the mechanism of uranium removal from groundwater by zero-valent iron using X-ray photoelectron spectroscopy[J]. Environmental Science&Technology,2015,32(10):1466-1473.
[27]Dutta S,Saha R,Kalita H,et al.Rapid reductive degradation of azo and anthraquinone dyes by nanoscale zero-valent iron[J].Environmental Technology&Innovation,2016,5:176-187.
[28]金晓英,陈征贤,郭飞鹏,等.超声波辅助壳聚糖/零价纳米铁降解酸性品红[J].环境科学学报,2013,33(4):1004-1009.
[29]鲍倩倩,李锦祥,关小红.预磁化强化零价铁除偶氮染料的性能研究[J].环境化学,2017,36(7):1467-1473.
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