东营凹陷南部沙河街组砂—泥岩协同成岩作用及其石油地质意义
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摘要
东营凹陷是一个油气资源丰富的陆相断陷盆地,经过40多年的勘探和开发,勘探对象逐渐由构造油气藏转向岩性隐蔽油气藏,由于岩性圈闭含油性预测困难,严重困扰着新增资源的勘探和评价。油气成藏是一个复杂的地质过程,烃类的运移仅仅是泥质烃源岩排出的以无机地层流体向砂岩运移汇聚过程中的特殊幕次。来自泥质烃源岩的孔隙流体对砂岩储层的成岩作用有着重要的影响,可以形成特征性的成岩矿物及其组合。本文对东营凹陷沙河街组沙四上烃源岩、沙三下烃源岩及砂岩的成岩作用进行了详细的分析研究,以期寻找砂泥岩在成岩过程中的流体联系。
首先,本文对比分析了东营凹陷沙河街组沙四上和沙三下两套泥质烃源岩的成岩矿物和地球化学特征。研究发现沙四上烃源岩的成岩碳酸盐矿物以高镁方解石和铁白云石为主,粘土矿物以富含绿泥石为特征,且有大量黄铁矿发育,具有高盐、富硫的成岩环境;沙三下泥质烃源岩的成岩碳酸盐矿物则以方解石为主,粘士矿物主要为伊利石、伊蒙混层和高岭石,黄铁矿仅零星发育,形成于相对低盐度、贫硫的成岩条件。地球化学分析表明沙四上烃源岩相较沙三下更为富含Ca、Mg、Fe、Ba和Sr等元素,且具有更重的C-O同位素组成。据此推测,沙四上烃源岩排出流体应具有更高的Ca、Mg、Fe、Ba、Mn和Sr等元素含量和更重的C-O同位素值。
其次,精细分析了东营凹陷沙河街砂岩的成岩矿物及其组合特征及其空间分布规律。研究发现砂岩碳酸盐矿物的化学成分变化大,在牛18-牛20断层附近及其南侧,碳酸盐胶结物以铁白云石为主,且Sr含量较高：在牛18-牛20断层北侧,则以含铁方解石和方解石为主,仅见少量铁白云石;而在洼陷东部,胶结物则主要为方解石。以胶结物形式出现的粘十矿物成分亦随构造位置变化而变化：在牛18-牛20断层附近及其南侧,以伊利石、高岭石绿泥石和绿蒙混层矿物为主,局部发育有大量的绿泥石和绿蒙混层(如N43井3244m处)；而在牛18-牛20断层北侧,粘土矿物主要为伊利石和高岭石,绿泥石和绿蒙混层矿物仅零星出现；及至洼陷东部,则仅见伊利石和高岭石。
第三,基于成岩矿物分析,提出了两套泥质烃源岩与砂岩间的协同成岩作用关系。近牛18-牛20断层及其南侧,以铁白云石、绿泥石和绿蒙混层矿物为特征的砂岩胶结物反映了富Ca、Mg、Fe等元素的高盐度成岩流体,与沙四上烃源岩的成岩流体具有明显的相似性。而牛18-牛20断层北侧,以含铁方解石为主、绿泥石和绿蒙混层矿物缺乏的砂岩胶结物反映了来自沙三下烃源岩的贡献,因其仍有较高的Sr含量,局部发育铁白云石,推测仍受到沙四上烃源岩的影响。在洼陷东部,砂岩胶结物以方解石、高岭石和伊利石为主,则为沙三下烃源岩成岩流体影响的结果。这一认识与油源对比研究结果亦一致。
第四,初步分析了砂泥岩成岩协同作用发生的空间联系和动力条件。通过典型成岩矿物的流体包裹体分析,发现牛18-牛20断层附近砂岩中包裹体盐度和捕获压力均相对较高,与该区普遍存在的异常高压带有着很好的一致性,可能为成岩流体运移的主要动力。而洼陷东部相对较低,该区亦未见异常压力带形成的勘探证据,成岩流体应以侧向运移和断层沟通为主。成岩流体的运移通道具有多样化,在正常压力区孔隙和微层理面为主要通道,而在异常压力带,断层和微裂隙是主要的运移通道,牛18-牛20断层贯穿了沙三下和沙四上烃源岩,对孔隙流体的运移起到了主要的疏导作用。且研究表明,烃源岩中发育有数量众多的微裂隙,大多被亮晶方解石所充填,而部分为未被充填的空裂隙,对成岩流体的运移具有不容忽视的影响。
The Dongying Depression is one of fault-sag lacustrine basins with enriched petroleum resources. During the last40-year petroleum exploration, the investigating targets became to potential oil pools reserved within lithological interfaces from the structural reservoirs. However, due to the difficulties for the petroleum prediction on this kind of oil-pools, it constrained these potential reservoirs'exploration and evaluation in the future. As for the complexities of oil-gas reserving process, the hydrocarbon migration is merely one step in its process of inorganic fluid from the argillaceous source rock to the reserving sandstone. The pore fluid resulted from the argillaceous source rock affected heavily on the reserving sandstone on its diagenesis of minerals, which could control partially its formation and assemblage essentially. This research targets a fluid effect in the argillaceous-sandstone source rock system based on the investigation of mineral diagenesis from the source rocks of Upper Unit in the fourth Member (ES43) and the Lower Unit in the third Member (ES3) of Shahejie Formation in Dongying Depression.
The first, comparisons on the diagenetic mineral and bulk-rock geochemical features have been made from the core samples of Units ES43and ES31in Dongying Depression. The diagenetic carbonate minerals in Unit ES43developed characteristically with highly contents of high-Mg calcite and ferrous dolomite; its clay minerals enriched with chlorite, and abundant of pyrite as well, which indicate a depositing environment of salinity with enriched element sulfur. Whereas, the carbonate minerals in the Unit ES31contain mainly mineral calcite; and its clay include minerals of illite, illite-kaolinite mixture, and kaolinite with few of pyrite, which means an environmental condition with low concentrations of salinity and sulfur. Geochemical data reveal that the source rock of ES4shows relatively high concentrations in elements of Mg, Ca, Fe, Ba, Sr, and heavy isotopic compositions of carbon and oxygen as well. These could deduce that the diagenitic fluid expelled from the source rock of Unit ES43with the same geochemical characters.
The second, this research analyzed the type of minerals, its assemblage and it spatial distribution of Unit ES31. The geochemical compositions of carbonate minerals in this Unit changed identifiably in different regions. The cement minerals contain mainly ferrodolomite with high content of element Sr near the fault Niu18-Niu20and southward nearby. In the northern side of Niu18-Niu20, it changed to be high content of ferroan calcite and calcite minerals with few of ferrodolomite; however, it developed merely in calcite in the eastern area of Dongying Depression. Significantly, the cemented clay-mineral composition displayed also changing distributions in different areas. In the Fault Niu18-Niu20and its southern side nearby, the cemented clay minerals are composited mainly of illite, kaolinite, chlorite, and chlorite-smectite mixture occasionally yielding with abundant minerals of chlorite and chlorite-smectite mixture elsewhere (e.g.,3244m depth in the Well N43); In the northern side of Fault Niu18-Niu20, it changes to be high content of illite and kaolinite minerals, but with sparse of chloritand chlorite-smectite; but it yielded merely the minerals of illite and kaolinite in the eastern area of Dongying Depression.
The third, this research recognized two relationships involving in the synergistic diagenesis between argillaceous and sandstone rocks under analysis of diagenetic minerals in this area. In the sandstone reservoir in the Fault Niu18-Niu20and nearby, the sandstone cements containing mainly with the minerals of ferrodolomite, chlorite, and chlorite-smectite mixture are result of the salinity fluid input with enriched elements of Ca, Mg, and Fe, which excluded from the Unit ES43with similar geochemical compositions. Whereas, the sandstone cements in the northern side of Fault Niu18-Niu20, which enriched with ferroan calcite but without chlorite and chlorite-smectite mixture, reflect the influences from the diagenetic fluid input of source rock in Unit ES31. Meanwhile, the relatively high content of element Sr in this sandstone cement means that it is still under the fluid effects from the Unit ES43. In the eastern side of Dongying Depression, the sandstone cement characteristically with high mineral contains of calcite, kaolinite and illite was the results of diagenetic fluid input from the source rock of Unit ES31. These conclusions are consistent with the results from researches of source rocks in this area before.
The fourth, this research discussed further the spatial relationships and its dynamic drive between the source rock and sandstone reservoir. The analysis on the inclusion textures in the sandstone cements reveals that high salinity and captured temperature occurred near the Fault Niu18-Niu20, which supported very well the evidence of high-pressure occurrence observed in this area before. This relative high pressure might be the driving force for the diagenetic fluid migration around. In the eastern side of the Dongying Depression, the analyses of sandstone inclusion texture found no evidence for the anomaly of high-pressure occurrence even from the exploration data before. We excluded that the driving force should migrated by the lateral system within rocks and by the channel connections in the fault belts. The migrating channel system of the diagenetic fluid varied by different connecting systems in this area. It generally transported by the pore system and/or the microlaminar system in normal pressure condition; however, it could migrate by the macro and/or micro-crack systems in the fault belt and rocks. The fault belt of Niu18-Niu20was a primary migrating channel for the diagenetic fluid transportation and release, which perfectly cut deeply downward through the source-rock beds of Unit ES31and ES34. Furthermore, this research observed also that abundant micro-crack system developed in the argillaceous source rock, which mostly filled by the sparry calcite; however, the remaining unfilled cracks should significantly to be connecting channel system for the diagenetic fluid migration.
首先,本文对比分析了东营凹陷沙河街组沙四上和沙三下两套泥质烃源岩的成岩矿物和地球化学特征。研究发现沙四上烃源岩的成岩碳酸盐矿物以高镁方解石和铁白云石为主,粘土矿物以富含绿泥石为特征,且有大量黄铁矿发育,具有高盐、富硫的成岩环境;沙三下泥质烃源岩的成岩碳酸盐矿物则以方解石为主,粘士矿物主要为伊利石、伊蒙混层和高岭石,黄铁矿仅零星发育,形成于相对低盐度、贫硫的成岩条件。地球化学分析表明沙四上烃源岩相较沙三下更为富含Ca、Mg、Fe、Ba和Sr等元素,且具有更重的C-O同位素组成。据此推测,沙四上烃源岩排出流体应具有更高的Ca、Mg、Fe、Ba、Mn和Sr等元素含量和更重的C-O同位素值。
其次,精细分析了东营凹陷沙河街砂岩的成岩矿物及其组合特征及其空间分布规律。研究发现砂岩碳酸盐矿物的化学成分变化大,在牛18-牛20断层附近及其南侧,碳酸盐胶结物以铁白云石为主,且Sr含量较高：在牛18-牛20断层北侧,则以含铁方解石和方解石为主,仅见少量铁白云石;而在洼陷东部,胶结物则主要为方解石。以胶结物形式出现的粘十矿物成分亦随构造位置变化而变化：在牛18-牛20断层附近及其南侧,以伊利石、高岭石绿泥石和绿蒙混层矿物为主,局部发育有大量的绿泥石和绿蒙混层(如N43井3244m处)；而在牛18-牛20断层北侧,粘土矿物主要为伊利石和高岭石,绿泥石和绿蒙混层矿物仅零星出现；及至洼陷东部,则仅见伊利石和高岭石。
第三,基于成岩矿物分析,提出了两套泥质烃源岩与砂岩间的协同成岩作用关系。近牛18-牛20断层及其南侧,以铁白云石、绿泥石和绿蒙混层矿物为特征的砂岩胶结物反映了富Ca、Mg、Fe等元素的高盐度成岩流体,与沙四上烃源岩的成岩流体具有明显的相似性。而牛18-牛20断层北侧,以含铁方解石为主、绿泥石和绿蒙混层矿物缺乏的砂岩胶结物反映了来自沙三下烃源岩的贡献,因其仍有较高的Sr含量,局部发育铁白云石,推测仍受到沙四上烃源岩的影响。在洼陷东部,砂岩胶结物以方解石、高岭石和伊利石为主,则为沙三下烃源岩成岩流体影响的结果。这一认识与油源对比研究结果亦一致。
第四,初步分析了砂泥岩成岩协同作用发生的空间联系和动力条件。通过典型成岩矿物的流体包裹体分析,发现牛18-牛20断层附近砂岩中包裹体盐度和捕获压力均相对较高,与该区普遍存在的异常高压带有着很好的一致性,可能为成岩流体运移的主要动力。而洼陷东部相对较低,该区亦未见异常压力带形成的勘探证据,成岩流体应以侧向运移和断层沟通为主。成岩流体的运移通道具有多样化,在正常压力区孔隙和微层理面为主要通道,而在异常压力带,断层和微裂隙是主要的运移通道,牛18-牛20断层贯穿了沙三下和沙四上烃源岩,对孔隙流体的运移起到了主要的疏导作用。且研究表明,烃源岩中发育有数量众多的微裂隙,大多被亮晶方解石所充填,而部分为未被充填的空裂隙,对成岩流体的运移具有不容忽视的影响。
The Dongying Depression is one of fault-sag lacustrine basins with enriched petroleum resources. During the last40-year petroleum exploration, the investigating targets became to potential oil pools reserved within lithological interfaces from the structural reservoirs. However, due to the difficulties for the petroleum prediction on this kind of oil-pools, it constrained these potential reservoirs'exploration and evaluation in the future. As for the complexities of oil-gas reserving process, the hydrocarbon migration is merely one step in its process of inorganic fluid from the argillaceous source rock to the reserving sandstone. The pore fluid resulted from the argillaceous source rock affected heavily on the reserving sandstone on its diagenesis of minerals, which could control partially its formation and assemblage essentially. This research targets a fluid effect in the argillaceous-sandstone source rock system based on the investigation of mineral diagenesis from the source rocks of Upper Unit in the fourth Member (ES43) and the Lower Unit in the third Member (ES3) of Shahejie Formation in Dongying Depression.
The first, comparisons on the diagenetic mineral and bulk-rock geochemical features have been made from the core samples of Units ES43and ES31in Dongying Depression. The diagenetic carbonate minerals in Unit ES43developed characteristically with highly contents of high-Mg calcite and ferrous dolomite; its clay minerals enriched with chlorite, and abundant of pyrite as well, which indicate a depositing environment of salinity with enriched element sulfur. Whereas, the carbonate minerals in the Unit ES31contain mainly mineral calcite; and its clay include minerals of illite, illite-kaolinite mixture, and kaolinite with few of pyrite, which means an environmental condition with low concentrations of salinity and sulfur. Geochemical data reveal that the source rock of ES4shows relatively high concentrations in elements of Mg, Ca, Fe, Ba, Sr, and heavy isotopic compositions of carbon and oxygen as well. These could deduce that the diagenitic fluid expelled from the source rock of Unit ES43with the same geochemical characters.
The second, this research analyzed the type of minerals, its assemblage and it spatial distribution of Unit ES31. The geochemical compositions of carbonate minerals in this Unit changed identifiably in different regions. The cement minerals contain mainly ferrodolomite with high content of element Sr near the fault Niu18-Niu20and southward nearby. In the northern side of Niu18-Niu20, it changed to be high content of ferroan calcite and calcite minerals with few of ferrodolomite; however, it developed merely in calcite in the eastern area of Dongying Depression. Significantly, the cemented clay-mineral composition displayed also changing distributions in different areas. In the Fault Niu18-Niu20and its southern side nearby, the cemented clay minerals are composited mainly of illite, kaolinite, chlorite, and chlorite-smectite mixture occasionally yielding with abundant minerals of chlorite and chlorite-smectite mixture elsewhere (e.g.,3244m depth in the Well N43); In the northern side of Fault Niu18-Niu20, it changes to be high content of illite and kaolinite minerals, but with sparse of chloritand chlorite-smectite; but it yielded merely the minerals of illite and kaolinite in the eastern area of Dongying Depression.
The third, this research recognized two relationships involving in the synergistic diagenesis between argillaceous and sandstone rocks under analysis of diagenetic minerals in this area. In the sandstone reservoir in the Fault Niu18-Niu20and nearby, the sandstone cements containing mainly with the minerals of ferrodolomite, chlorite, and chlorite-smectite mixture are result of the salinity fluid input with enriched elements of Ca, Mg, and Fe, which excluded from the Unit ES43with similar geochemical compositions. Whereas, the sandstone cements in the northern side of Fault Niu18-Niu20, which enriched with ferroan calcite but without chlorite and chlorite-smectite mixture, reflect the influences from the diagenetic fluid input of source rock in Unit ES31. Meanwhile, the relatively high content of element Sr in this sandstone cement means that it is still under the fluid effects from the Unit ES43. In the eastern side of Dongying Depression, the sandstone cement characteristically with high mineral contains of calcite, kaolinite and illite was the results of diagenetic fluid input from the source rock of Unit ES31. These conclusions are consistent with the results from researches of source rocks in this area before.
The fourth, this research discussed further the spatial relationships and its dynamic drive between the source rock and sandstone reservoir. The analysis on the inclusion textures in the sandstone cements reveals that high salinity and captured temperature occurred near the Fault Niu18-Niu20, which supported very well the evidence of high-pressure occurrence observed in this area before. This relative high pressure might be the driving force for the diagenetic fluid migration around. In the eastern side of the Dongying Depression, the analyses of sandstone inclusion texture found no evidence for the anomaly of high-pressure occurrence even from the exploration data before. We excluded that the driving force should migrated by the lateral system within rocks and by the channel connections in the fault belts. The migrating channel system of the diagenetic fluid varied by different connecting systems in this area. It generally transported by the pore system and/or the microlaminar system in normal pressure condition; however, it could migrate by the macro and/or micro-crack systems in the fault belt and rocks. The fault belt of Niu18-Niu20was a primary migrating channel for the diagenetic fluid transportation and release, which perfectly cut deeply downward through the source-rock beds of Unit ES31and ES34. Furthermore, this research observed also that abundant micro-crack system developed in the argillaceous source rock, which mostly filled by the sparry calcite; however, the remaining unfilled cracks should significantly to be connecting channel system for the diagenetic fluid migration.
引文
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