缅甸硬玉岩地区钠长石岩的矿物学研究
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摘要
钠长石岩是一种以单一矿物钠长石为主要组成的矿物，在世界上比较少见。产于俯冲带内低温高压环境下的由单矿物构成的硬玉岩通常伴有钠长石岩，目前对于硬玉岩研究的关注度较高，而对于钠长石岩的研究则相对较少，很少有相关论文报导。产于缅甸翡翠矿区的钠长石岩，经常与硬玉岩相伴而生，是良好的研究样品。
缅甸硬玉岩地区钠长石岩的主要矿物成分是钠长石，X射线粉晶衍射结合电子探针分析的结果得到其有序度高，属于低温钠长石，形成温度小于300℃。其次含有硬玉、绿辉石、透辉石等辉石类矿物和钠透闪石、蓝透闪石、镁钠闪石等闪石类矿物，此外还有钠沸石、针钠钙石、含钡和锶的矿物等。钠长石岩沿着解理和裂隙交代硬玉，说明钠长石形成晚于硬玉岩。钠长石岩中的透辉石有两种类型，一类可能是随着被交代的硬玉中的透辉石组分增加而形成的透辉石，另一类是被绿辉石包裹的透辉石残留，其很有可能是早期来自地幔楔或俯冲带岩石中的矿物残留，即异剥钙榴岩类或辉石岩类，可以视作硬玉化绿辉石岩和硬玉化异剥钙榴岩的矿物学证据。钠长石沿着针钠钙石边缘的交代现象，说明钠长石形成于针钠钙石之后。钠沸石、含钡的沸石类矿物和含锶的矿物作为后期矿物出现在钠长石和硬玉颗粒之间。
大量钠长石交代硬玉的现象表明缅甸硬玉岩地区钠长石岩是由富钠流体交代硬玉岩而形成，在交代结构不发育的钠长石岩中，并不能排除钠长石岩直接从流体中结晶而形成。对钠长石岩中流体包裹体的成分和阴阳离子含量进行分析，结果表明钠长石岩中的流体包裹体以H2O为主，四级质谱仪测量结果显示H2O的含量在93.01-98.37mol.%，没有发现类似硬玉岩中富CH4的流体包裹体；其中含量最多的阳离子为Na+，其次为Ca2+和Mg2+，含量最多的阴离子为F﹣和Cl﹣。结合钠长石岩中后期含钡和锶矿物的出现，说明形成钠长石岩的流体与形成硬玉岩的流体有一定的继承关系，流体可能来自硬玉岩之后的残余流体。热液型钠长石岩的存在进一步说明缅甸翡翠矿区钠化热液存在现象的普遍性与穿越性。
通过对不同外观钠长石岩的结构和显微构造进行研究，将缅甸地区的钠长石岩的结构分为两种类型：原生结构和变质变形结构。其中变质重结晶结构包括：晶体结晶定向、机械双晶、亚颗粒、锯齿状高角度缝合边以及恢复结构。钠长石岩通过亚颗粒旋转、颗粒边界迁移等方式将钠长石颗粒细化并定向，形成透明度高的钠长石玉。这些结构的存在说明钠长石岩形成之后经历了持续、强烈的地质力，而这种地质力最有可能的提供者是实皆走滑断裂。
Albitite, a type of rock composed principally of albite, is rare to find.Albitite isfound in several geolocal settings, one of which is in assocation with jadeitite, a rockmade up almost entirely of jadeitic pyroxene and forms under a relatively high-P/Tcondition in the subduction zones. Jadeitites have attracted much attention fromgeologists and gemologists internationally, and many sites of jadeitites have been welldocumented. However, there has been little understanding about the albitites, whichare always associated with jadeitites. The Myanmar jadeite deposit, where someclassic mineral relationships are preserved, is also home to the best samples ofalbitite.
Albitite is mainly composed of low-temperature albite, pyroxene minerals such asjadeite, omphacite and dioside and amphibole minerals such as richterite, winchiteand magnesio-riebeckite, natrolite, pectolite, Ba and Sr minerals. Replacement of thejadeite by albite in the albitite along its cleavage and crack indicates that albite formslater than the jadeite. Diopside in the albitite consists of two types: one formed byreplacement of jadeite which contains some components of dioside, the other isinferred to be the residual which was part of the replaced rocks like rodingite orpyroxenite belonging the host serpentine mélange. The latter can be used asmineralogical evidence for confirmation of jadeitized pyroxenite and jadeitizedrondingite.
Replacement of the jadeite by albite indicates the metasomatic origin of albitite.However, we can not exclude the origin of vein crystallization from fluids in thesamples that do not have replacement texture. Micro-Raman spectroscopy,QMS(Quadrupole mass spectrometry) and ion chromatograph were used to detectcomponents in the fluid inclusions, obtain information about additional volatiles andmeasure the bulk cation and anion contents of the fluid inclusions. The fluidinclusions in the albitites are mainly composed of H2O，QMS measurements haveshown that the bulk fluids contain93.01-98.37mol.%H2O. The samples arecharacterized by ionic contents higher than that of in the jadeitites, the most abundantcation being Na+, Ca2+and Mg2+and the most abundant anion are F﹣and Cl﹣.Combined with the Ba and Sr minerals in the albitites, it can be speculated that the albitite-forming fluids might be derived from the residual fluids of the jadeitites.Existence of the albite shows that Na-rich fluids are thorugh and traversing.
Similar to jadeitite, albitite from Myanmar can be classified into two types:undeformed albitite and deformed albitite. The deformed textures include crystallineorientation, mechanical twin, sub-grain, serrated high-angle sutured grain boundariesand recovery textures. Transformation of coarse albitite into the transparentgem-quality albite jade, should have undergone at least two coupled processes ofgrain size reduction and crystallographic orientation. The main processes causingthese are progressive misorientaion of sub-grains and grain-boundary migration. Theexistence of these deformation textures indicate that the most transparent albite jadehas undergone long-lasting and intensive, localized geological forces. It is very likelythat the source of these forces is linked to the major Sagaing stike-slip faults.
缅甸硬玉岩地区钠长石岩的主要矿物成分是钠长石，X射线粉晶衍射结合电子探针分析的结果得到其有序度高，属于低温钠长石，形成温度小于300℃。其次含有硬玉、绿辉石、透辉石等辉石类矿物和钠透闪石、蓝透闪石、镁钠闪石等闪石类矿物，此外还有钠沸石、针钠钙石、含钡和锶的矿物等。钠长石岩沿着解理和裂隙交代硬玉，说明钠长石形成晚于硬玉岩。钠长石岩中的透辉石有两种类型，一类可能是随着被交代的硬玉中的透辉石组分增加而形成的透辉石，另一类是被绿辉石包裹的透辉石残留，其很有可能是早期来自地幔楔或俯冲带岩石中的矿物残留，即异剥钙榴岩类或辉石岩类，可以视作硬玉化绿辉石岩和硬玉化异剥钙榴岩的矿物学证据。钠长石沿着针钠钙石边缘的交代现象，说明钠长石形成于针钠钙石之后。钠沸石、含钡的沸石类矿物和含锶的矿物作为后期矿物出现在钠长石和硬玉颗粒之间。
大量钠长石交代硬玉的现象表明缅甸硬玉岩地区钠长石岩是由富钠流体交代硬玉岩而形成，在交代结构不发育的钠长石岩中，并不能排除钠长石岩直接从流体中结晶而形成。对钠长石岩中流体包裹体的成分和阴阳离子含量进行分析，结果表明钠长石岩中的流体包裹体以H2O为主，四级质谱仪测量结果显示H2O的含量在93.01-98.37mol.%，没有发现类似硬玉岩中富CH4的流体包裹体；其中含量最多的阳离子为Na+，其次为Ca2+和Mg2+，含量最多的阴离子为F﹣和Cl﹣。结合钠长石岩中后期含钡和锶矿物的出现，说明形成钠长石岩的流体与形成硬玉岩的流体有一定的继承关系，流体可能来自硬玉岩之后的残余流体。热液型钠长石岩的存在进一步说明缅甸翡翠矿区钠化热液存在现象的普遍性与穿越性。
通过对不同外观钠长石岩的结构和显微构造进行研究，将缅甸地区的钠长石岩的结构分为两种类型：原生结构和变质变形结构。其中变质重结晶结构包括：晶体结晶定向、机械双晶、亚颗粒、锯齿状高角度缝合边以及恢复结构。钠长石岩通过亚颗粒旋转、颗粒边界迁移等方式将钠长石颗粒细化并定向，形成透明度高的钠长石玉。这些结构的存在说明钠长石岩形成之后经历了持续、强烈的地质力，而这种地质力最有可能的提供者是实皆走滑断裂。
Albitite, a type of rock composed principally of albite, is rare to find.Albitite isfound in several geolocal settings, one of which is in assocation with jadeitite, a rockmade up almost entirely of jadeitic pyroxene and forms under a relatively high-P/Tcondition in the subduction zones. Jadeitites have attracted much attention fromgeologists and gemologists internationally, and many sites of jadeitites have been welldocumented. However, there has been little understanding about the albitites, whichare always associated with jadeitites. The Myanmar jadeite deposit, where someclassic mineral relationships are preserved, is also home to the best samples ofalbitite.
Albitite is mainly composed of low-temperature albite, pyroxene minerals such asjadeite, omphacite and dioside and amphibole minerals such as richterite, winchiteand magnesio-riebeckite, natrolite, pectolite, Ba and Sr minerals. Replacement of thejadeite by albite in the albitite along its cleavage and crack indicates that albite formslater than the jadeite. Diopside in the albitite consists of two types: one formed byreplacement of jadeite which contains some components of dioside, the other isinferred to be the residual which was part of the replaced rocks like rodingite orpyroxenite belonging the host serpentine mélange. The latter can be used asmineralogical evidence for confirmation of jadeitized pyroxenite and jadeitizedrondingite.
Replacement of the jadeite by albite indicates the metasomatic origin of albitite.However, we can not exclude the origin of vein crystallization from fluids in thesamples that do not have replacement texture. Micro-Raman spectroscopy,QMS(Quadrupole mass spectrometry) and ion chromatograph were used to detectcomponents in the fluid inclusions, obtain information about additional volatiles andmeasure the bulk cation and anion contents of the fluid inclusions. The fluidinclusions in the albitites are mainly composed of H2O，QMS measurements haveshown that the bulk fluids contain93.01-98.37mol.%H2O. The samples arecharacterized by ionic contents higher than that of in the jadeitites, the most abundantcation being Na+, Ca2+and Mg2+and the most abundant anion are F﹣and Cl﹣.Combined with the Ba and Sr minerals in the albitites, it can be speculated that the albitite-forming fluids might be derived from the residual fluids of the jadeitites.Existence of the albite shows that Na-rich fluids are thorugh and traversing.
Similar to jadeitite, albitite from Myanmar can be classified into two types:undeformed albitite and deformed albitite. The deformed textures include crystallineorientation, mechanical twin, sub-grain, serrated high-angle sutured grain boundariesand recovery textures. Transformation of coarse albitite into the transparentgem-quality albite jade, should have undergone at least two coupled processes ofgrain size reduction and crystallographic orientation. The main processes causingthese are progressive misorientaion of sub-grains and grain-boundary migration. Theexistence of these deformation textures indicate that the most transparent albite jadehas undergone long-lasting and intensive, localized geological forces. It is very likelythat the source of these forces is linked to the major Sagaing stike-slip faults.
引文
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