高铁酸盐去除废水中重金属及其他污染物的研究进展
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摘要
重金属的污染严重威胁着水生态环境和人类健康,需要研发更加高效、绿色的水处理药剂。高铁酸钾作为新一代的水处理药剂,以其独特的氧化和混凝效果已经得到了众多研究者的深入研究。文章综述了高铁酸盐的制备方法、高铁酸钾在水处理中对重金属的去除研究以及在处理其他污染物方面的应用。
The pollution of heavy metals is a particularly serious threat to the ecological environment of water and human health. Therefore,the research and development on more efficient and environment-friendly water treatment agents are needed. Potassium ferrate, as a new generation of water treatment agents,has been investigated in depth by a great number of researchers, due to its unique oxidation and coagulation effects. The preparation method of potassium ferrate, the research on the removal of heavy metals in water treatment and the application in dealing with other pollutants are summarized.
The pollution of heavy metals is a particularly serious threat to the ecological environment of water and human health. Therefore,the research and development on more efficient and environment-friendly water treatment agents are needed. Potassium ferrate, as a new generation of water treatment agents,has been investigated in depth by a great number of researchers, due to its unique oxidation and coagulation effects. The preparation method of potassium ferrate, the research on the removal of heavy metals in water treatment and the application in dealing with other pollutants are summarized.
引文
[1]秦海利.高铁酸钾对废水中亚甲基蓝和重金属离子的处理研究[D].绵阳:绵阳师范学院,2016.
[2] Begum A, Amin N,Kaneco S. Selected elemental composition of the muscle tissue of three species of fish:tilapia niltica cirrhina ntrigala and clarius batrachus from fresh water Dhanmondi Lake in Bangledesh[J]. Food Chemistry,2005,93(3):439-443.
[3]葛俊森,梁渠.水中重金属危害现状及处理方法[J].江苏化工,2007,35(5):44-46.
[4] Jiang Jiaqian. Advances in the development and application of ferrate(Ⅵ)for water and wastewater treatment[J]. Journal of Chemical Technology and Biotechnology,2014,89(2):165-177.
[5]王东升,李文涛,杨晓芳.高铁酸盐:一种绿色的多功能水处理剂[J].应用化学,2016,33(11):1221-1233.
[6]孙旭辉,李文超,李冰.高铁酸盐的制备、性质及在水处理中的应用[J].东北电力大学学报,2015,35(4):33-39.
[7] Macova Z,Bouzek K,Hives J,et al. Research progress in the electrochemical synthesis of Ferrate(Ⅵ)[J]. Electrochimica Acta,2009,54(10):2673-2683.
[8]汪德家.高铁酸钾在水处理中的应用与研究[D].上海:同济大学,2005.
[9]何文丽,桂和荣,苑志华,等.高铁酸钾混凝去除矿井水中的铅、镉、铁、锰[J].工业水处理,2009,29(10):83-86.
[10]苑志华,桂和荣,何文丽,等.高铁酸钾去除重金属的模拟试验研究[J].水处理技术,2009,35(5):67-71.
[11]柴立元,王云燕,邓荣,等.水环境中铬的存在形态及迁移转化规律[J].工业安全与环保,2006,32(8):1-3.
[12]崔建国,刘幼琼,李娜.高铁酸钾同时降解微污染水中苯酚和Cr(Ⅵ)的研究[J].中国环境科学,2011,31(9):1461-1465.
[13]王萍,王世亮,刘少卿,等.砷的发生、形态、污染源及地球化学循环[J].环境科学与技术,2010,33(7):90-97.
[14]许杉.沉积物中砷的赋存形态及其环境化学特征[D].北京:中国地质大学(北京),2012.
[15] Fan M,Brown R C,Huang C P. Preliminary studies of the oxidation of Arsenic(Ⅲ)by potassium ferrate[J]. International Journal of Environment&Pollution,2003,18(1):91-96.
[16] Lee Y,Um I H,Yoon J. Arsenic(Ⅲ)oxidation by Iron(Ⅵ)(Ferrate)and subsequent removal of Arsenic(Ⅴ)by Iron(Ⅲ)coagulation[J].Environmental Science&Technology,2003,37(24):5750-5756.
[17] Goff H,Murmann R K. Mechanism of isotopic oxygen exchange and reduction of Ferrate(Ⅵ)ion(Fe O42-)[J]. Journal of the American Chemical Society,2002,93(23):94-95.
[18]孙玉林.废水中Cr(Ⅵ)、As(Ⅴ)处理技术及其污染去除机理[D].济南:山东建筑大学,2015.
[19]蒋国民.高铁酸钾的制备及其处理含砷废水的研究[D].长沙:中南大学,2010.
[20] Lim M,Kim M J. Effectiveness of potassium ferrate(K2Fe O4)for si multaneous removal of heavy metals and natural organic matters from river water[J]. Water,Air,&Soil Pollution,2010,211(1):313-322.
[21]王颖馨,周雪婷,卜洪龙,等.高铁酸钾的制备及其对水中As(Ⅲ)、Pb(Ⅱ)的去除效能研究[J].华南师范大学学报:自然科学版,2015,47(4):80-87.
[22] Lan B,Wang Y,Wang X,et al. Aqueous Arsenic(As)and antimony(Sb)removal by potassium ferrate[J]. Chemical Engineering Journal,2016,292:389-397.
[23] Sailo L,Pachuau L,Yang J K,et al. Efficient use of Ferrate(Ⅵ)for the remediation of wastewater contaminated with metal complexes[J]. Environmental Engineering Research,2015,20(1):89-97.
[24] Pachuau L,Lee S M,Tiwari D. Ferrate(Ⅵ)in wastewater treatment contaminated with metal(Ⅱ)-iminodiacetic acid complexed species[J]. Chemical Engineering Journal,2013,230(16):141-148.
[25] Tiwari D,Sailo L,Pachuau L. Remediation of aquatic environment contaminated with the iminodiacetic acid metal complexes using ferrate(Ⅵ)[J]. Separation&Purification Technology,2014,132(3):77-83.
[26] Lee S M,Tiwari D. Application of ferrate(Ⅵ)in the treatment of industrial wastes containing metal-complexed cyanides:a green treatment[J]. Journal of Environmental Sciences,2009,21(10):1347-1352.
[27]吴晓荣.高铁酸钾联合聚合硫酸铁对除磷试验的研究[D].太原:太原理工大学,2012.
[28] Jing Zhang,Liang Zhu,Zhenyu Shi,et al. Rapid removal of organic pollutants by activation sulfite with ferrate[J]. Chemosphere,2017,186:576-579.
[29] Mingbao Feng,Leslie Cizmas,Zunyao Wang,et al. Synergistic effect of aqueous removal of fluoroquinolones by a combined use of peroxymonosulfate and ferrate(Ⅵ)[J]. Chemosphere,2017,177:144-148.
[30] Sharma V K, Zboril R, Varma R S. Ferrates:greener oxidants with multimodal action in water treatment technologies[J]. Accounts of Chemical Research,2015,48(2):182-191.
[31] Malik S N, Ghosh P C, Vaidya A N,et al. Comparison of coagulation,ozone and ferrate treatment processes for color,COD and toxicity removal from complex textile wastewater[J]. Water Science&Technology,2017,76(5):1001-1010.
[32] Wu C,Jin L,Zhang P,et al. Effects of potassium ferrate oxidation on sludge disintegration,dewaterability and anaerobic biodegradation[J]. International Biodeterioration&Biodegradation,2015,102:137-142.
[33] Gombos E,Barkács K,Felfoldi T,et al. Removal of organic matters in wastewater treatment by ferrate(Ⅵ)-technology[J]. Microchemical Journal,2013,107(3):115-120.
[34]朱开金,李敏,任晓莉,等. Si O32+作用下Ag2+对K2Fe O4氧化焦化废水的有效催化[J].工业水处理,2018,38(2):59-62.
[35]刘菲,赵胜勇,王晓毅.高铁酸钾氧化处理废水中邻氯苯酚的研究[J].工业用水与废水,2018,49(2):29-31.
[36] Mager T R,Landes J D,Moon D M,et al. An overview on production and application of ferrate(Ⅵ)for chemical oxidation,coagulation and disinfection of water and wastewater[J]. Journal of Environmental Chemical Engineering,2017,5(2):1828-1842.
[2] Begum A, Amin N,Kaneco S. Selected elemental composition of the muscle tissue of three species of fish:tilapia niltica cirrhina ntrigala and clarius batrachus from fresh water Dhanmondi Lake in Bangledesh[J]. Food Chemistry,2005,93(3):439-443.
[3]葛俊森,梁渠.水中重金属危害现状及处理方法[J].江苏化工,2007,35(5):44-46.
[4] Jiang Jiaqian. Advances in the development and application of ferrate(Ⅵ)for water and wastewater treatment[J]. Journal of Chemical Technology and Biotechnology,2014,89(2):165-177.
[5]王东升,李文涛,杨晓芳.高铁酸盐:一种绿色的多功能水处理剂[J].应用化学,2016,33(11):1221-1233.
[6]孙旭辉,李文超,李冰.高铁酸盐的制备、性质及在水处理中的应用[J].东北电力大学学报,2015,35(4):33-39.
[7] Macova Z,Bouzek K,Hives J,et al. Research progress in the electrochemical synthesis of Ferrate(Ⅵ)[J]. Electrochimica Acta,2009,54(10):2673-2683.
[8]汪德家.高铁酸钾在水处理中的应用与研究[D].上海:同济大学,2005.
[9]何文丽,桂和荣,苑志华,等.高铁酸钾混凝去除矿井水中的铅、镉、铁、锰[J].工业水处理,2009,29(10):83-86.
[10]苑志华,桂和荣,何文丽,等.高铁酸钾去除重金属的模拟试验研究[J].水处理技术,2009,35(5):67-71.
[11]柴立元,王云燕,邓荣,等.水环境中铬的存在形态及迁移转化规律[J].工业安全与环保,2006,32(8):1-3.
[12]崔建国,刘幼琼,李娜.高铁酸钾同时降解微污染水中苯酚和Cr(Ⅵ)的研究[J].中国环境科学,2011,31(9):1461-1465.
[13]王萍,王世亮,刘少卿,等.砷的发生、形态、污染源及地球化学循环[J].环境科学与技术,2010,33(7):90-97.
[14]许杉.沉积物中砷的赋存形态及其环境化学特征[D].北京:中国地质大学(北京),2012.
[15] Fan M,Brown R C,Huang C P. Preliminary studies of the oxidation of Arsenic(Ⅲ)by potassium ferrate[J]. International Journal of Environment&Pollution,2003,18(1):91-96.
[16] Lee Y,Um I H,Yoon J. Arsenic(Ⅲ)oxidation by Iron(Ⅵ)(Ferrate)and subsequent removal of Arsenic(Ⅴ)by Iron(Ⅲ)coagulation[J].Environmental Science&Technology,2003,37(24):5750-5756.
[17] Goff H,Murmann R K. Mechanism of isotopic oxygen exchange and reduction of Ferrate(Ⅵ)ion(Fe O42-)[J]. Journal of the American Chemical Society,2002,93(23):94-95.
[18]孙玉林.废水中Cr(Ⅵ)、As(Ⅴ)处理技术及其污染去除机理[D].济南:山东建筑大学,2015.
[19]蒋国民.高铁酸钾的制备及其处理含砷废水的研究[D].长沙:中南大学,2010.
[20] Lim M,Kim M J. Effectiveness of potassium ferrate(K2Fe O4)for si multaneous removal of heavy metals and natural organic matters from river water[J]. Water,Air,&Soil Pollution,2010,211(1):313-322.
[21]王颖馨,周雪婷,卜洪龙,等.高铁酸钾的制备及其对水中As(Ⅲ)、Pb(Ⅱ)的去除效能研究[J].华南师范大学学报:自然科学版,2015,47(4):80-87.
[22] Lan B,Wang Y,Wang X,et al. Aqueous Arsenic(As)and antimony(Sb)removal by potassium ferrate[J]. Chemical Engineering Journal,2016,292:389-397.
[23] Sailo L,Pachuau L,Yang J K,et al. Efficient use of Ferrate(Ⅵ)for the remediation of wastewater contaminated with metal complexes[J]. Environmental Engineering Research,2015,20(1):89-97.
[24] Pachuau L,Lee S M,Tiwari D. Ferrate(Ⅵ)in wastewater treatment contaminated with metal(Ⅱ)-iminodiacetic acid complexed species[J]. Chemical Engineering Journal,2013,230(16):141-148.
[25] Tiwari D,Sailo L,Pachuau L. Remediation of aquatic environment contaminated with the iminodiacetic acid metal complexes using ferrate(Ⅵ)[J]. Separation&Purification Technology,2014,132(3):77-83.
[26] Lee S M,Tiwari D. Application of ferrate(Ⅵ)in the treatment of industrial wastes containing metal-complexed cyanides:a green treatment[J]. Journal of Environmental Sciences,2009,21(10):1347-1352.
[27]吴晓荣.高铁酸钾联合聚合硫酸铁对除磷试验的研究[D].太原:太原理工大学,2012.
[28] Jing Zhang,Liang Zhu,Zhenyu Shi,et al. Rapid removal of organic pollutants by activation sulfite with ferrate[J]. Chemosphere,2017,186:576-579.
[29] Mingbao Feng,Leslie Cizmas,Zunyao Wang,et al. Synergistic effect of aqueous removal of fluoroquinolones by a combined use of peroxymonosulfate and ferrate(Ⅵ)[J]. Chemosphere,2017,177:144-148.
[30] Sharma V K, Zboril R, Varma R S. Ferrates:greener oxidants with multimodal action in water treatment technologies[J]. Accounts of Chemical Research,2015,48(2):182-191.
[31] Malik S N, Ghosh P C, Vaidya A N,et al. Comparison of coagulation,ozone and ferrate treatment processes for color,COD and toxicity removal from complex textile wastewater[J]. Water Science&Technology,2017,76(5):1001-1010.
[32] Wu C,Jin L,Zhang P,et al. Effects of potassium ferrate oxidation on sludge disintegration,dewaterability and anaerobic biodegradation[J]. International Biodeterioration&Biodegradation,2015,102:137-142.
[33] Gombos E,Barkács K,Felfoldi T,et al. Removal of organic matters in wastewater treatment by ferrate(Ⅵ)-technology[J]. Microchemical Journal,2013,107(3):115-120.
[34]朱开金,李敏,任晓莉,等. Si O32+作用下Ag2+对K2Fe O4氧化焦化废水的有效催化[J].工业水处理,2018,38(2):59-62.
[35]刘菲,赵胜勇,王晓毅.高铁酸钾氧化处理废水中邻氯苯酚的研究[J].工业用水与废水,2018,49(2):29-31.
[36] Mager T R,Landes J D,Moon D M,et al. An overview on production and application of ferrate(Ⅵ)for chemical oxidation,coagulation and disinfection of water and wastewater[J]. Journal of Environmental Chemical Engineering,2017,5(2):1828-1842.
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