Solution-processed high-k oxide dielectric via deep ultraviolet and rapid thermal annealing for high-performance MoS<sub>2sub> FETs
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文摘
So far most of MoS<sub>2sub>-based devices have been demonstrated on oxide gate dielectrics (e.g., SiO<sub>2sub>, Al<sub>2sub>O<sub>3sub>, HfO<sub>2sub>, etc) deposited by vacuum process or on polymer gate dielectrics. In this study, we report electrical characteristics of multilayer MoS<sub>2sub> transistors fabricated on solution-processed high-k AlO<sub>xsub> gate dielectric via deep ultraviolet (DUV) activation in combination with rapid thermal annealing process at 250&thinsp;°C. The solution-processed AlO<sub>xsub> sol&ndash;gel film exhibited low leakage current of about 1.49&thinsp;μA&thinsp;cm<sup>&minus;2sup> at 1&thinsp;MV&thinsp;cm<sup>&minus;1sup> and a relative dielectric constant (k) of &sim;6.1 at 1&thinsp;kHz. The fabricated MoS<sub>2sub>-FETs exhibit median field-effect mobility of &sim;23.3&thinsp;cm<sup>2sup>&thinsp;V<sup>&minus;1sup>s<sup>&minus;1sup>, threshold voltage of &sim;&thinsp;0.79&thinsp;V, subthreshold slope of &sim;0.30&thinsp;V&thinsp;dec<sup>&minus;1sup>, and on/off current ratio of &sim;10<sup>7sup>. The electrical performance can be further improved by optimizing the AlO<sub>xsub> sol&ndash;gel film as well as the device structure, and the result implies that the solution-processed high-k AlO<sub>xsub> is promising for TMDC&ndash;based device applications.

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