Functional NZVI coupled with ultrasound as a novel and green system was proposed.
The functional NZVI was fabricated via a facile, one-step and eco-friendly method.
The new system achieved a significant synergy in decolorization of cationic dyes.
As reductant, dispersant and capping agent, tea polyphenol is eco-friendly.
The findings offer insight into nanoremediation with practical green approach.