Intimately coupled hybrid of graphitic carbon nitride nanoflakelets with reduced graphene oxide for supporting Pd nanoparticles: A stable nanocatalyst with high catalytic activity towards formic acid and methanol electrooxidation
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- 作者：Wenyao Zhanga ; Qiushi Yaob ; Xiaodong Wua ; Yongsheng Fua ; fuyongsheng0925@163.com" class="auth_mail" title="E-mail the corresponding author ; Kaiming Dengb ; kmdeng@njust.edu.cn" class="auth_mail" title="E-mail the corresponding author ; Xin Wanga ; wangx@njust.edu.cn" class="auth_mail" title="E-mail the corresponding author ; wxin48@163.com" class="auth_mail" title="E-mail the corresponding author
- 关键词：graphene ; graphitic carbon nitride nanoflakelets ; electrocatalysis ; formic acid oxidation ; methanol oxidation
- 刊名：Electrochimica Acta
- 出版年：2016
- 出版时间：10 May 2016
- 年：2016
- 卷：200
- 期：Complete
- 页码：131-141
- 全文大小：2977 K
文摘
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Intimately coupled hybrid of g-C3N4 nanoflakelets with rGO is fabricated via an in situ chemical synthesis approach.
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The detailed forming process of CNNF-G composite is carefully investigated.
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The Pd-CNNF-G composite exhibits exceptional catalytic activity and durability.
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The real fuel cells have been assembled to evaluate the performance of the electrocatalysts.
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The effects of g-C3N4 nanoflakelets on Pd atom were investigated by DFT computations.