Synthesis, characterization of a new photosensitive compound [Ru(bpy)2 (TPAD)](PF6)2 and its application for photocatalytic hydrogen production
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- 作者：Hui-Qin Zhenga ; b ; Yi-Ping Guoc ; Ming-Cai Yinb ; 1 ; mcyin@zzu.edu.cn" class="auth_mail" title="E-mail the corresponding author ; Yao-Ting Fanb ; yt.fan@zzu.edu.cn" class="auth_mail" title="E-mail the corresponding author ; ytfan1207@163.com" class="auth_mail" title="E-mail the corresponding author
- 关键词：Triphenylamine derivative ; Ruthenium(II) photosensitive complex ; TiO2 photosensitive catalyst ; Photo-catalytic hydrogen production
- 刊名：Chemical Physics Letters
- 出版年：2016
- 出版时间：1 June 2016
- 年：2016
- 卷：653
- 期：Complete
- 页码：17-23
- 全文大小：2016 K
文摘
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A new photosensitive compound [Ru(bpy)2(TPAD)](PF6)2 (PS1) was synthesized.
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PS1 was characterized by elemental analysis, 1H NMR, MS spectra, UV, PL and CV.
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Photocatalyst PS1/0.5 wt% Pt/TiO2 was prepared and characterized by SEM and XRD.
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The photocatalytic hydrogen-evolving conditions were optimized.
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The total amount of hydrogen evolution reached to 9500 μmol·(g·catalyst)−1 within 5.5 h.