Energy efficient sorption enhanced-chemical looping methane reforming process for high-purity H2 production: Experimental proof-of-concept
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- 作者：Andy Antzaraa ; Eleni Heracleousb ; c ; Angeliki A. Lemonidoua ; c ; alemonidou@cheng.auth.gr" class="auth_mail" title="E-mail the corresponding author
- 关键词：Oxygen transfer materials ; CO2 sorbents ; Ca&ndash ; Ni looping ; Sorption enhanced chemical looping steam methane reforming ; High-purity hydrogen ; High energy efficiency
- 刊名：Applied Energy
- 出版年：2016
- 出版时间：15 October 2016
- 年：2016
- 卷：180
- 期：Complete
- 页码：457-471
- 全文大小：3497 K
文摘
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Experimental demonstration of low-energy sorption enhanced chemical looping methane reforming.
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NiO/ZrO2 is easily reduced by CH4 even in the presence of steam and exhibits high reforming activity.
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CaO/CaZrO3 demonstrates high capacity and remarkable stability in multiple cycles.
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Ni reoxidation can cover substantial part of the heat for sorbent calcination.