The results showed that the heavy metal concentrations in foliar dust were high, particularly for Cd and Pb. Concentrations of Cd ranged from 6.2 to 12.8 mg kg−1, while concentrations of Pb ranged from 434.0 to 512.0 mg kg−1. The amount of foliar dust retained by the four tree species increased with time for 20 d following a rain event. The amount of foliar dust collected from different locations in the city was significantly different. Specifically, the heavy metal and sulfur pollution index in the different locations decreased in this order: Power Station (PS) > Electronic Industry Area (EIA) > Commercial and Traffic Area (CTA) > Residential Areas (RA) > Control Area (CA). These data suggest that the foliar dust can remove appreciable amounts of Cd, Cr, Cu, Pb, Zn, and S – 0.040 t, 1.63 t, 2.70 t, 1.84 t, 5.54 t, and 19.52 t, respectively – from the atmosphere in the study area. This information can provide health-related impetus and guidance for the work of urban planners and those involved in environment protection.