Cleaner production of methanol from carbon dioxide over copper and iron supported MCM-41 catalysts using innovative integrated magnetic field-packed bed reactor

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• 作者：Sirapassorn Kiatphuengporn^a ; ^b ; Waleeporn Donphai^a ; ^b ; Pongsakorn Jantaratana^c ; Nevzat Yigit^d ; Karin Fö ; ttinger^d ; Gü ; nther Rupprechter^d ; Metta Chareonpanich^a ; ^b ; ^{fengmtc@ku.ac.th}
• 关键词：Sustainable innovation ; CO2 utilization ; Methanol ; Hydrogenation ; Magnetic field ; Fe-Cu catalyst
• 刊名：Journal of Cleaner Production
• 出版年：2017
• 出版时间：20 January 2017
• 年：2017
• 卷：142
• 期：part_P3
• 页码：1222-1233
• 全文大小：2148 K
• 卷排序：142

文摘

External magnetic field was equipped to a conventional catalytic fixed-bed reactor. Methanol was produced via CO2 hydrogenation over w(Cu)-w(Fe)/MCM-41 catalysts. This integrated magnetic field reactor promoted methanol production at lower temp. The operating temperature could be reduced up to 57.7 °C at the same rate of reaction. Less CO2 emissions by means of temperature saving was obtained from this process.