CoIrx/γ-Al2O3 catalysts were synthesized by impregnation method.
CoIrx/γ-Al2O3 materials catalyzed hydrogen generation from N2H4·H2O decomposition.
CoIr0.081/γ-Al2O3 catalyst exhibited highest activity and 100% H2 selectivity.
Optimal catalytic activity was achieved due to formation of Co–Ir alloy on γ-Al2O3.