Neutron time-of-flight (TOF) methods have been used to measure the neutron spectra produced on thin targets of low-Z (titanium) and high-Z (tantalum) materials at incident deuteron energies of 20 MeV and 29 MeV at 0°. Breakup neutrons at both energies from low-Z targets appear to peak at roughly half of the available kinetic energy, while neutrons from high-Z interactions peak somewhat lower in energy, owing to the increased proton energy due to breakup within the Coulomb field. Furthermore, neutron spectra appear narrower for high-Z targets. These centroids are consistent with recent preliminary proton energy measurements using silicon telescope detectors conducted at LBNL, though there is a notable discrepancy with spectral widths. Prospects for producing a tunable, quasi-monoenergetic neutron facility of 106–108 n/cm2/s at LBNL are promising.