A green template-assisted synthesis of hierarchical TS-1 with excellent catalytic activity and recyclability for the oxidation of 2,3,6-trimethylphenol

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• 作者：Xiang Gao ; Jianguo An ; Jinlou Gu ; Liang Li ; Yongsheng Li ; ^{ysli@ecust.edu.cn}
• 关键词：Zeolites ; Hierarchical TS-1 ; Ammonium-modified chitosan ; Selective oxidation ; Recyclability
• 刊名：Microporous and Mesoporous Materials
• 出版年：2017
• 出版时间：February 2017
• 年：2017
• 卷：239
• 期：Complete
• 页码：381-389
• 全文大小：3681 K
• 卷排序：239

文摘

A low-cost product from exoskeleton of crustaceans, HTCC, was first used to synthesize hierarchical TS-1 as mesoporogen. The hierarchical TS-1 zeolite possesses large external surface areas and mesoporous volumes. The hierarchical TS-1 presents high activity and selectivity for the oxidation of TMP under mild conditions.