Urania foam was successfully prepared for the first time by using sucrose-gel precursor method. Porous urania pellets were successfully prepared for the first time by using citrate gel-combustion method. The foam comprised both meso and macro pores, possessed good crush strength and porosity. Citric acid to nitrate ratio of 0.25 and a compaction pressure of 180 MPa were best suited for the preparation of porous pellets.