Phonon-assisted relaxation in a frustrated antiferromagnet
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文摘
A thermally activated magnetic relaxation is observed using neutron spin-echo in the pyrochlore slab (kagomé bilayer) compound in a restricted temperature range, , above a cross-over to a low temperature relaxation regime with a weaker temperature dependence. The activation energy of the thermally activated relaxation, of the order of 7 meV, coincides with the energy of a phonon mode observed with neutron and Raman spectroscopy, indicating a phonon-assisted regime. The experimental observation of phonon-assisted process gives additional insight to the importance of spin–phonon coupling in frustrated magnets with regard to the models mostly based on purely magnetic interactions.

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