tert-Butylcarbazole-based Schiff bases and difluoroboron complex were synthesized.
rong class="boldFont">TPMProng> and rong class="boldFont">TPMArong> without any tradition gelation group could form organogels.
Appropriate π-π interaction between π-skeleton with tert-butyl leads to the gelation.
rong class="boldFont">TPOBrong> showed reversible piezofluorochromism.
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