Burnout of soot particles in a two-stage burner with a JP-8 surrogate fuel
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- 作者：Carlos A. Echavarria ; Isabel C. Jaramillo ; Adel F. Sarofim ; JoAnn S. Lighty ; jlighty@utah.edu ;
- 关键词：Soot size distribution ; JP-8 ; m-Xylene flames ; n-Dodecane flames ; Soot oxidation
- 刊名：Combustion and Flame
- 出版年：2012
- 出版时间：July, 2012
- 年：2012
- 卷：159
- 期：7
- 页码：2441-2448
- 全文大小：849 K
文摘
This work focuses on the understanding of the oxidation of soot particles which were the result of using a JP-8 surrogate fuel in a two-stage burner. The two-stage system consists of an initial premixed burner where soot was generated with an air/fuel mixture, specifically a JP-8 surrogate (m-xylene and n-dodecane), under a variety of conditions. Downstream, the soot-laden combustion gases were passed through a second, flat-flame burner where soot was burned out under fuel-lean or slightly fuel-rich conditions. Soot oxidation in the secondary burner was determined by investigating particle size distribution (PSD), flame temperature, gas-phase composition, soot surface area, and soot morphology and nanostructure as a function of the height above the second burner (HAB). Measurements of soot size distribution and number concentration as a function of the HAB under fuel lean (¦µoverall = 0.8) and slightly rich (¦µoverall = 1.14) conditions showed a decrease in particle mean diameter and a significant increase in number concentration in the region where O2 concentration decreased. In this region, the effectiveness factor for O2 was found to be 1, indicating the potential for internal oxygen diffusion and burning. This caused both the breakup of the bridges cementing primary particles and the rupture of the primary particles. Higher in the burner, where modeling suggested the presence of OH*, soot oxidation was attributed to OH* mechanisms which are faster as compared to O2 oxidation.