Effects of finite laser pulse width on two-dimensional electronic spectroscopy

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• 作者：Xuan Leng^a ; ^b ; ^c ; Shuai Yue^a ; ^c ; Yu-Xiang Weng^a ; ^c ; ^{yxweng@aphy.iphy.ac.cn} ; Kai Song^b ; ^c ; Qiang Shi^b ; ^c ; ¹ ; ^{qshi@iccas.ac.cn}
• 关键词：Two-dimensional electronic spectroscopy ; Hierarchical equations of motion ; Optical response functions ; Finite laser pulse width
• 刊名：Chemical Physics Letters
• 出版年：2017
• 出版时间：January 2017
• 年：2017
• 卷：667
• 期：Complete
• 页码：79-86
• 全文大小：2307 K
• 卷排序：667

文摘

The laser pulses are included explicitly in two-dimensional electronic spectra simulation. Effects of the finite laser pulse width are examined. Two-color two-dimensional electronic spectra are simulated. To observe quantum beats, the related excitonic states should be excited simultaneously.