Mined retired coefficient of haze (COH) data to estimate black carbon (BC) trends. Determined COH-BC relationship with two reinstated COH monitors and aethalometers. BC concentrations decreased markedly between 1965 and 2000 across the U.S. BC decreased from 13 to 2 μg m−3 in New Jersey and 4 to 1 μg m−3 in California. Declining BC concentrations contrast increasing energy use and CO2 emissions.