Influences of fireworks on chemical characteristics of atmospheric fine and coarse particles during Taiwan's Lantern Festival

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• 作者：Hsieh-Hung Tsai ; Li-Hsing Chien ; Chung-Shin Yuan ; Yuan-Chung Lin ; Yi-Hsiu Jen ; Iau-Ren Ie
• 关键词：Firework displays ; Air quality monitoring ; Physicochemical properties ; Principal component analysis (PCA) ; CMB receptor modeling
• 刊名：Atmospheric Environment
• 出版年：2012
• 出版时间：December, 2012
• 年：2012
• 卷：62
• 期：Complete
• 页码：256-264
• 全文大小：1207 K

文摘

In recent years, the celebration activities of various folk-custom festivals have been getting more and more attention from the citizens in Taiwan. Festivities throughout the whole island are traditionally accompanied by loud and brightly colored firework displays. Among these activities, the firework displays during Taiwan's Lantern Festival in Kaohsiung harbor is one of the largest festivals in Taiwan each year. Therefore, it is of importance to investigate the influence of fireworks displays on the ambient air quality during the Taiwan's Lantern Festival. Field measurements of atmospheric particulate matter (PM) were conducted on February 9th-11th, 2009 during Taiwan's Lantern Festival in Kaohsiung City. Moreover, three kinds of fireworks powders obtained from the same manufacturing factory producing Kaohsiung Lantern Festival fireworks were burned in a self-designed combustion chamber to determine the physicochemical properties of the fireworks' particles and to establish the source profile of firework burning. Several metallic elements of PM during the firework display periods were notably higher than those during the non-firework periods. The concentrations of Mg, K, Pb, and Sr in PM_2.5 during the firework periods were 10 times higher than those during the non-firework periods. Additionally, the Cl^?/Na⁺ ratio was approximately 3 during the firework display periods as Cl^? came from the chlorine content of the firework powder. Moreover, the OC/EC ratio increased up to 2.8. Results obtained from PCA and CMB receptor modeling showed that major sources of atmospheric particles during the firework display periods in Kaohsiung harbor were fireworks, vehicular exhausts, soil dusts and marine sprays. Particularly, on February 10th, the firework displays contributed approximately 25.2 % and 16.6 % of PM₁₀ at two downwind sampling sites, respectively.