Dynamics in pure and substituted volborthite kagome-like compounds
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文摘
Volborthite Cu3V2O7(OH)2·2H2O is a natural frustrated antiferromagnet with a kagomé-like magnetic lattice decorated by spins. Our μSR results confirm the existence of a dynamical plateau below 2 K, as initially demonstrated in [Phys. Rev. Lett. 91 (2003) 207603] despite sensible quantitative differences in the relaxation rate values. Thanks to additional low temperature SQUID and NMR data we show that this plateau occurs concurrently with a freezing transition. Moreover, we revisited the effect of diluting the magnetic lattice for small dilution rates between 1 % and 15 % . Comparison is made with the well studied kagomé bilayer compounds. The ground state of volborthite appears to be far less stable with respect to dilution.

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