The structure of the neutron rich
pf-shell nuclei
58Ti
36,
60Cr
36 and
62Cr
38 was studied by proton inelastic scattering in inverse kinematics. Large quadrupole deformation lengths of 1.12(16) fm and 1.36(14) fm were obtained for
60Cr and
62Cr, respectively, which confirm the enhanced collectivity in these nuclei. An excited state was observed in
62Cr at 1180(10) keV with tentative assignment of
Jπ=4+. The increase in the
Ex(4+)/Ex(2+) ratio indicates that the nature of collectivity changes from vibrational to rotational in
62Cr and affords evidence for the development of static deformation. The excitation energy of the newly observed 2
+ state in
58Ti (1046(17) keV) shows hindered collectivity. The contrast between the structures of Cr and Ti suggests that the contributions of both protons and neutrons are crucial for the large collectivity in Cr close to
N=40. From the comparison to shell model calculations, the large collectivity is found to originate from the admixture of the
pf- and
gd-shells across the
N=40 sub-shell gap.