Utilization of plasmonics in charge generation and separation by resonant energy transfer is well synergized with Schottky junction for enhanced photocatalytic water splitting.
A surfactant-free nanofabrication approach has been developed to confine dense Au nanoparticles in N-doped TiO2 bowl-like nanoarrays, achieving full-spectrum photocatalysis.
The design achieves H2 production rates of 637 μmol g−1 h−1 in full spectrum and 132 μmol g−1 h−1 in visible region, respectively, from pure water based on TiO2.
This work represents a step towards large-scale photocatalyst fabrication and full-spectrum photocatalysis.