Enhanced full-spectrum water splitting by confining plasmonic Au nanoparticles in N-doped TiO2 bowl nanoarrays
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文摘

Utilization of plasmonics in charge generation and separation by resonant energy transfer is well synergized with Schottky junction for enhanced photocatalytic water splitting.

A surfactant-free nanofabrication approach has been developed to confine dense Au nanoparticles in N-doped TiO2 bowl-like nanoarrays, achieving full-spectrum photocatalysis.

The design achieves H2 production rates of 637 μmol g−1 h−1 in full spectrum and 132 μmol g−1 h−1 in visible region, respectively, from pure water based on TiO2.

This work represents a step towards large-scale photocatalyst fabrication and full-spectrum photocatalysis.

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