Improved performance of hierarchical Fe-ZSM-5 in the direct oxidation of benzene to phenol by N2O
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- 作者：Lulu Lia ; Qinglun Menga ; Junjun Wena ; Jingui Wangb ; Gaomei Tua ; Chunhui Xua ; Fumin Zhanga ; Yijun Zhonga ; Weidong Zhua ; Qiang Xiaoa ; xiaoq@zjnu.edu.cn" class="auth_mail" title="E-mail the corresponding author
- 关键词：Hierarchical zeolite ; Fe-ZSM-5 ; Silane coupling agent ; Benzene oxidation ; Nitrous oxide
- 刊名：Microporous and Mesoporous Materials
- 出版年：2016
- 出版时间：June 2016
- 年：2016
- 卷：227
- 期：Complete
- 页码：252-257
- 全文大小：872 K
文摘
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Hierarchical Fe-ZSM-5 zeolites were hydrothermally synthesized.
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5">A silane coupling agent of 3-glycidoxypropyltrimethoxysilane was used.
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Direct oxidation of benzene to phenol was conducted on the hierarchical Fe-ZSM-5.
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5">The hierarchical Fe-ZSM-5 showed better activity and stability.
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n-Butane uptake experiments indicated the improvement of internal mass-transfer.