Two-Dimensional Modeling of Volatile Organic Compounds Adsorption onto Beaded Activated Carbon

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• 作者：Dereje Tamiru Tefera ; Masoud Jahandar Lashaki ; Mohammadreza Fayaz ; Zaher Hashisho ; John H. Philips ; James E. Anderson ; Mark Nichols
• 刊名：Environmental Science & Technology
• 出版年：2013
• 出版时间：October 15, 2013
• 年：2013
• 卷：47
• 期：20
• 页码：11700-11710
• 全文大小：570K
• 年卷期：v.47,no.20(October 15, 2013)
• ISSN：1520-5851

文摘

A two-dimensional heterogeneous computational fluid dynamics model was developed and validated to study the mass, heat, and momentum transport in a fixed-bed cylindrical adsorber during the adsorption of volatile organic compounds (VOCs) from a gas stream onto a fixed bed of beaded activated carbon (BAC). Experimental validation tests revealed that the model predicted the breakthrough curves for the studied VOCs (acetone, benzene, toluene, and 1,2,4-trimethylbenzene) as well as the pressure drop and temperature during benzene adsorption with a mean relative absolute error of 2.6, 11.8, and 0.8%, respectively. Effects of varying adsorption process variables such as carrier gas temperature, superficial velocity, VOC loading, particle size, and channelling were investigated. The results obtained from this study are encouraging because they show that the model was able to accurately simulate the transport processes in an adsorber and can potentially be used for enhancing absorber design and operation.