Reductions in Emissions of Carbonaceous Particulate Matter and Polycyclic Aromatic Hydrocarbons from Combustion of Biomass Pellets in Comparison with Raw Fuel Burning

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• 作者：Guofeng Shen ; Shu Tao ; Siye Wei ; Yanyan Zhang ; Rong Wang ; Bin Wang ; Wei Li ; Huizhong Shen ; Ye Huang ; Yuanchen Chen ; Han Chen ; Yifeng Yang ; Wei Wang ; Wen Wei ; Xilong Wang ; Wenxing Liu ; Xuejun Wang ; Staci L. Massey Simonich
• 刊名：Environmental Science & Technology (ES&T)
• 出版年：2012
• 出版时间：June 5, 2012
• 年：2012
• 卷：46
• 期：11
• 页码：6409-6416
• 全文大小：272K
• 年卷期：v.46,no.11(June 5, 2012)
• ISSN：1520-5851

文摘

Biomass pellets are emerging as a cleaner alternative to traditional biomass fuels. The potential benefits of using biomass pellets include improving energy utilization efficiency and reducing emissions of air pollutants. To assess the environmental, climate, and health significance of replacing traditional fuels with biomass pellets, it is critical to measure the emission factors (EFs) of various pollutants from pellet burning. However, only a few field measurements have been conducted on the emissions of carbon monoxide (CO), particulate matter (PM), and polycyclic aromatic hydrocarbons (PAHs) from the combustion of pellets. In this study, pine wood and corn straw pellets were burned in a pellet burner (2.6 kW), and the EFs of CO, organic carbon, elemental carbon, PM, and PAHs (EF_CO, EF_OC, EF_EC, EF_PM, and EF_PAH) were determined. The average EF_CO, EF_OC, EF_EC, and EF_PM were 1520 卤 1170, 8.68 卤 11.4, 11.2 卤 8.7, and 188 卤 87 mg/MJ for corn straw pellets and 266 卤 137, 5.74 卤 7.17, 2.02 卤 1.57, and 71.0 卤 54.0 mg/MJ for pine wood pellets, respectively. Total carbonaceous carbon constituted 8 to 14% of the PM mass emitted. The measured values of EF_PAH for the two pellets were 1.02 卤 0.64 and 0.506 卤 0.360 mg/MJ, respectively. The secondary side air supply in the pellet burner did not change the EFs of most pollutants significantly (p > 0.05). The only exceptions were EF_OC and EF_PM for pine wood pellets because of reduced combustion temperatures with the increased air supply. In comparison with EFs for the raw pine wood and corn straw, EF_CO, EF_OC, EF_EC, and EF_PM for pellets were significantly lower than those for raw fuels (p < 0.05). However, the differences in EF_PAH were not significant (p > 0.05). Based on the measured EFs and thermal efficiencies, it was estimated that 95, 98, 98, 88, and 71% reductions in the total emissions of CO, OC, EC, PM, and PAHs could be achieved by replacing the raw biomass fuels combusted in traditional cooking stoves with pellets burned in modern pellet burners.