A novel quinone-based polymer electrode for high performance lithium-ion batteries

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• 作者：Jian Xie 谢健 ; Zilong Wang 王子龙 ; Peiyang Gu 顾培洋 ; Yi Zhao 赵毅…
• 关键词：lithium battery ; electrode ; polymer ; carbonyl ; thioether
• 刊名：Science China Materials
• 出版年：2016
• 出版时间：January 2016
• 年：2016
• 卷：59
• 期：1
• 页码：6-11
• 全文大小：795 KB
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• 作者单位：Jian Xie 谢健 (1)
  Zilong Wang 王子龙 (1)
  Peiyang Gu 顾培洋 (1)
  Yi Zhao 赵毅 (1)
  Zhichuan J. Xu 徐梽川 (1)
  Qichun Zhang 张其春 (1) (2)
  
  1. School of Materials Science and Engineering, Nanyang Technological University, Singapore, 639798, Singapore
  2. Division of Chemistry and Biological Chemistry, School of Physical and Mathematics Science, Nanyang Technological University, Singapore, 637371, Singapore
  
• 刊物类别：Materials Science, general; Chemistry/Food Science, general;
• 刊物主题：Materials Science, general; Chemistry/Food Science, general;
• 出版者：Science China Press
• ISSN：2199-4501

文摘

Designing of high electrochemical performance organic electrode materials has attracted tremendous attention. Recent investigations revealed that quinone-based polymers along with the stable thioether bonds could achieve a high specific capacity and a good cycling stability simultaneously. In this study, we synthesized a novel ladder-structured polymer poly(2,3-dithiino-1,4- benzoquinone) (PDB) through a simple two-step polymerization. The electrochemical performance indicated that PDB could achieve a high reversible specific capacity of 681 mAh g−1 with 98.4% capacity retention after 100 cycles. A good rate performance was also achieved with a fast recovery of the capacity after testing at different current densities. Ultra-long cycling performance of PDB was also investigated. The promising results of PDB provided us more confidence to continue searching for high performance polymers through the modification of organic structures. Keywords lithium battery electrode polymer carbonyl thioether