Laser ablation of Al–Ni alloys and multilayers
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  • 作者:Johannes Roth ; Hans-Rainer Trebin ; Alexander Kiselev
  • 刊名:Applied Physics A: Materials Science & Processing
  • 出版年:2016
  • 出版时间:May 2016
  • 年:2016
  • 卷:122
  • 期:5
  • 全文大小:6,258 KB
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  • 作者单位:Johannes Roth (1)
    Hans-Rainer Trebin (1)
    Alexander Kiselev (1)
    Dennis-Michael Rapp (1) (2)

    1. Institut für Funktionelle Materie und Quantentechnologien, Universität Stuttgart, Stuttgart, Germany
    2. Institut für Materialprüfung, Werkstoffkunde und Festigkeitslehre, Universität Stuttgart, Stuttgart, Germany
  • 刊物类别:Physics and Astronomy
  • 刊物主题:Physics
    Condensed Matter
    Optical and Electronic Materials
    Nanotechnology
    Characterization and Evaluation Materials
    Surfaces and Interfaces and Thin Films
    Operating Procedures and Materials Treatment
  • 出版者:Springer Berlin / Heidelberg
  • ISSN:1432-0630
文摘
Laser ablation of Al–Ni alloys and multilayers has been studied by molecular dynamics simulations. The method was combined with a two-temperature model to describe the interaction between the laser beam, the electrons, and the atoms. As a first step, electronic parameters for the alloys had to be found and the model developed originally for pure metals had to be generalized to multilayers. The modifications were verified by computing melting depths and ablation thresholds for pure Al and Ni. Here known data could be reproduced. The improved model was applied to the alloys \(\mathrm{Al}_3\mathrm{Ni}\), AlNi and \(\mathrm{AlNi}_3\). While melting depths and ablation thresholds for AlNi behave unspectacular, sharp drops at high fluences are observed for \(\mathrm{Al}_3\mathrm{Ni}\) and \(\mathrm{AlNi}_3\). In both cases, the reason is a change in ablation mechanism from phase explosion to vaporization. Furthermore, a phase transition occurs in \(\mathrm{Al}_3\mathrm{Ni}\). Finally, Al layers of various thicknesses on a Ni substrate have been simulated. Above threshold, 8 nm Al films are ablated as a whole while 24 nm Al films are only partially removed. Below threshold, alloying with a mixture gradient has been observed in the thin layer system.

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