Efficiency comparison for treatment of amantadine pharmaceutical wastewater by Fenton, ultrasonic, and Fenton/ultrasonic processes

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• 作者：Ping Zeng ; Jijun Du ; Yonghui Song ; Yongqiang Liu…
• 关键词：Amantadine ; Fenton ; Ultrasonic ; Fenton/ultrasonic ; Comparison ; Cavitation
• 刊名：Environmental Earth Sciences
• 出版年：2015
• 出版时间：May 2015
• 年：2015
• 卷：73
• 期：9
• 页码：4979-4987
• 全文大小：856 KB
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• 作者单位：Ping Zeng (1) (2) (3)
  Jijun Du (1)
  Yonghui Song (1) (2)
  Yongqiang Liu (4)
  Ruixia Liu (1) (2)
  Panyue Zhang (5)
  Shuhu Xiao (1) (2)
  
  1. State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Chaoyang District, Beiyuan Road, Dayangfang 8, Beijing, 100012, China
  2. Department of Urban Water Environmental Research, Chinese Research Academy of Environmental Sciences, Beijing, 100012, China
  3. State Environmental Protection Key Laboratory of Microorganism Application and Risk Control (MARC), Tsinghua University, Beijing, 100084, China
  4. Faculty of Engineering and the Environment, University of Southampton, Southampton, SO17 1BJ, UK
  5. Beijing Key Lab for Source Control Technology of Water Pollution, Beijing Forestry University, Beijing, 100083, China
  
• 刊物类别：Earth and Environmental Science
• 刊物主题：None Assigned
• 出版者：Springer Berlin Heidelberg
• ISSN：1866-6299

文摘

Amantadine wastewater is quite recalcitrant to biological treatment because of the quite stable adamantine backbone. To improve amantadine wastewater biodegradability, the combined advanced oxidation process, such as Fenton/ultrasonic process, was proposed to treat amantadine industrial wastewater. The efficiency comparisons for the treatment of amantadine wastewater using Fenton oxidation, ultrasonic process, and Fenton/ultrasonic process were conducted. The results of wastewater treatment with Fenton/ultrasonic process indicated that the TOC removal reached 65.6?%, showing almost 4 times of the degradation rate by individual oxidizing action of hydrogen peroxide. Kinetic study revealed that degradation of amantadine wastewater fitted first order kinetics for the three processes under investigation. The synergistic index (f) for the combined process was calculated as 2.24, indicating an obvious synergy effect. The energy consumption for hydrodynamic cavitation-based process has been analyzed on the basis of cavitational yield. Fenton and combined processes reduced the toxicity of wastewater by 50 and 55?%, respectively, while ultrasonic process showed no obvious effect on toxicity reduction. The monitoring of treated wastewater by EEM and GC–MS showed that the Fenton/ultrasonic process effectively removed the organic matters in the wastewater, especially the biodegradation-resistant matters containing benzene ring.