Thermodynamic Assessment of the Bi–Ni and Bi–Ni–X (X = Ag, Cu) Systems

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• 作者：Yuling Liu ; Shuhong Liu ; Cong Zhang ; Xingxu Lu…
• 关键词：Bi–Ni ; Bi–Ni–Ag ; Bi–Ni–Cu ; thermodynamic modeling ; CALPHAD
• 刊名：Journal of Electronic Materials
• 出版年：2016
• 出版时间：February 2016
• 年：2016
• 卷：45
• 期：2
• 页码：1041-1056
• 全文大小：2,590 KB
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• 作者单位：Yuling Liu (1)
  Shuhong Liu (1)
  Cong Zhang (1)
  Xingxu Lu (2)
  Chong Chen (1)
  Yong Du (1)
  Dragana Živković (3)
  
  1. State Key Laboratory of Powder Metallurgy, Central South University, Changsha, 410083, Hunan, China
  2. School of Materials Science and Engineering, Central South University, Changsha, 410083, Hunan, China
  3. Technical Faculty, University of Belgrade, VJ 12, 19210, Bor, Serbia
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Optical and Electronic Materials
  Characterization and Evaluation Materials
  Electronics, Microelectronics and Instrumentation
  Solid State Physics and Spectroscopy
  
• 出版者：Springer Boston
• ISSN：1543-186X

文摘

The Bi–Ni system was reassessed by means of the calculation of phase diagrams (CALPHAD) method by considering the latest published experimental data. To maintain the compatibility in higher-order systems, the excess Gibbs energy of the solution phases was modeled with the Redlich–Kister polynomials, and a three-sublattice model, (Bi)_0.3334(Ni,Va)_0.3333(Va,Ni)_0.3333, was used to describe the intermetallic compound BiNi with NiAs-type crystal structure. Compared with the previous thermodynamic description for the Bi–Ni system, noticeable improvements are achieved in the present work. The current thermodynamic parameters can well reproduce the newly published experimental data on thermodynamic properties. Based on the newly obtained parameters for the Bi–Ni system, as well as the thermodynamic descriptions for the Bi-Ag, Ni-Ag, Bi-Cu, and Ni-Cu systems in literature, a thermodynamic database of the Bi–Ni–Ag and Bi–Ni–Cu ternary systems was established by considering the available experimental data. The calculated phase equilibria in these ternary systems are in satisfactory agreement with experimental observations. Keywords Bi–Ni Bi–Ni–Ag Bi–Ni–Cu thermodynamic modeling CALPHAD