Enabling practical electrocatalyst-assisted photoelectron-chemical water splitting with earth abundant materials
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- 作者：Xiaogang Yang (1)
Rui Liu (2) (3)
Yumin He (3)
James Thorne (3)
Zhi Zheng (1)
Dunwei Wang (3)
1. Key Laboratory of Micro-Nano Materials for Energy Storage and Conversion of Henan Province and Institute of Surface Micro and Nano Materials ; Xuchang University ; Henan ; 461000 ; China
2. Division of Chemistry and Chemical Engineering ; Joint Center for Artificial Photosynthesis ; California Institute of Technology ; Pasadena ; CA ; 91125 ; USA
3. Department of Chemistry ; Boston College ; Merkert Chemistry Center ; 2609 Beacon St. ; Chestnut Hill ; MA ; 02467 ; USA - 关键词：photoelectrochemical water splitting ; efficiency ; stability ; interface ; earth abundance
- 刊名：Nano Research
- 出版年：2015
- 出版时间：January 2015
- 年：2015
- 卷：8
- 期：1
- 页码：56-81
- 全文大小：3,827 KB
- 参考文献：1. / BP Statistical Review of World Energy. BP Plc, 2014.
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- 刊物主题：Chinese Library of Science
Chemistry
Nanotechnology - 出版者：Tsinghua University Press, co-published with Springer-Verlag GmbH
- ISSN：1998-0000
文摘
Sustainable development and continued prosperity of humanity hinge on the availability of renewable energy sources on a terawatts scale. In the long run, solar energy is the only source that can meet this daunting demand. Widespread utilization of solar energy faces challenges as a result of its diffusive (hence low energy density) and intermittent nature. How to effectively harvest, concentrate, store and redistribute solar energy constitutes a fundamental challenge that the scientific community needs to address. Photoelectrochemical (PEC) water splitting is a process that can directly convert solar energy into chemical energy and store it in chemical bonds, by producing hydrogen as a clean fuel source. It has received significant research attention lately. Here we provide a concise review of the key issues encountered in carrying out PEC water splitting. Our focus is on the balance of considerations such as stability, earth abundance, and efficiency. Particular attention is paid to the combination of photoelectrodes with electrocatalysts, especially on the interfaces between different components.